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Volumn 282, Issue 5392, 1998, Pages 1305-1309

Large-scale nitrogen oxide plumes in the tropopause region and implications for ozone

Author keywords

[No Author keywords available]

Indexed keywords

NITROGEN OXIDE;

EID: 0032514883     PISSN: 00368075     EISSN: None     Source Type: Journal    
DOI: 10.1126/science.282.5392.1305     Document Type: Article
Times cited : (73)

References (32)
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    • note
    • x concentration averaged over all measurements between December 1995 to May 1996 of 172 pptv, this represents a difference of about 20%.
  • 22
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    • note
    • ECMWF (European Centre for Medium-Range Weather Forecast) model at T213/L31 resolution - that is, with 31 vertical layers and 0.75° by 0.75° horizontal resolution.
  • 29
    • 3643111474 scopus 로고    scopus 로고
    • note
    • x samples that show an average increase relative to the background of at least 0.1 ppbv. The background level during a plume event was simply obtained by linear interpolation between the concentrations adjacent to the plume (Fig. 1). Given the (true air) speed of the aircraft of 250 m/s, four samples correspond to a flight leg of 120 km. A difference of 0.1 ppbv is well above the noise of the measurement (11) and represents a significant increase above background levels of typically 70 to 200 pptv (Table 1).
  • 30
    • 3643138572 scopus 로고    scopus 로고
    • note
    • Using a higher PV value of 4 PVU for the tropopause definition, the fraction of samples obtained within plumes is 10.4% and 1.6% for the tropospheric and stratospheric samples, respectively. Thus, the probability to observe a large-scale plume rapidly decreases in the stratosphere.
  • 32
    • 3643125023 scopus 로고    scopus 로고
    • note
    • The NOXAR project was funded by the Swiss Federal Civil Aviation Authority (BAZL). We thank Swissair for the generous support and ECO Physics Inc. for the design of the instrumentation and the assistance during the measurements. We also acknowledge H. Wernli and M. Bourqui for the trajectory calculations and R. Luethi for providing data from his archive of satellite images, which were both of great help for the interpretation of the measurements.


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