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Volumn 112, Issue 11, 2000, Pages 4910-4922

Approximate calculation of femtosecond pump-probe spectra monitoring nonadiabatic excited-state dynamics

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EID: 0001014447     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.481045     Document Type: Article
Times cited : (25)

References (47)
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    • The mixed terms E†A and A†E have been omitted since they vanish in standard pump-probe experiments, which average over the phase of the electric field
    • The mixed terms E†A and A†E have been omitted since they vanish in standard pump-probe experiments, which average over the phase of the electric field.
  • 35
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    • In all calculations, approximate and exact nonperturbative data have been scaled by multiplication with a constant factor, which was usually chosen such that the signals coincide at the maximal delay time
    • In all calculations, approximate and exact nonperturbative data have been scaled by multiplication with a constant factor, which was usually chosen such that the signals coincide at the maximal delay time.
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    • note
    • Unlike the probing of the system as a function of the delay time and probe frequency, the interaction with the pump pulse needs to be calculated only a single time. It is therefore not a time-consuming task and can be readily performed exactly. Within the Franck-Condon approximation, finite pump pulses and overlapping laser fields have been described in Ref. 16.


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