Dimeric [Mo2S12]2- Cluster: A Molecular Analogue of MoS2 Edges for Superior Hydrogen-Evolution Electrocatalysis

Angewandte Chemie - International Edition

Volumn 54, Issue 50, 2015, Pages 15181-15185

  Huang, Zhongjie ^a   Luo, Wenjia ^b   Ma, Lu ^a   Yu, Mingzhe ^a   Ren, Xiaodi ^a   He, Mingfu ^a   Polen, Shane ^a   Click, Kevin ^a   Garrett, Benjamin ^a   Lu, Jun ^d   Amine, Khalil ^d   Hadad, Christopher ^a   Chen, Weilin ^c   Asthagiri, Aravind ^b   Wu, Yiying ^a  

^a OHIO STATE UNIVERSITY   (United States)

^b The Ohio State University   (United States)

^c NORTHEAST NORMAL UNIVERSITY   (China)

^d ARGONNE NATIONAL LABORATORY   (United States)

Author keywords

electrocatalysis; hydrogen adsorption energy; hydrogen evolution; molecular analogues; molybdenum sulfide

Indexed keywords

BIOMIMETICS; CATALYSIS; CATALYSTS; ELECTROCATALYSIS; FREE ENERGY; HYDROGEN; LIGANDS; MOLYBDENUM COMPOUNDS; SULFUR COMPOUNDS;

ATTRACTIVE STRATEGIES; CATALYTIC MECHANISMS; ELECTROCHEMICAL TEST; HYDROGEN ADSORPTION; HYDROGEN EVOLUTION; HYDROGEN EVOLUTION REACTIONS; MOLECULAR ANALOGUES; MOLYBDENUM SULFIDE;

GAS ADSORPTION;

EID: 84955204546     PISSN: 14337851     EISSN: 15213773     Source Type: Journal    
DOI: 10.1002/anie.201507529     Document Type: Article

References (38)

1. J. K. Nørskov, T. Bligaard, A. Logadottir, J. R. Kitchin, J. G. Chen, S. Pandelov, U. Stimming, J. Electrochem. Soc. 2005, 152, J 23 -J 26;
2. T. F. Jaramillo, K. P. Jorgensen, J. Bonde, J. H. Nielsen, S. Horch, I. Chorkendorff, Science 2007, 317, 100-102.
3. B. Hinnemann, P. G. Moses, J. Bonde, K. P. Jorgensen, J. H. Nielsen, S. Horch, I. Chorkendorff, J. K. Norskov, J. Am. Chem. Soc. 2005, 127, 5308-5309.
4. H. I. Karunadasa, E. Montalvo, Y. Sun, M. Majda, J. R. Long, C. J. Chang, Science 2012, 335, 698-702.
5. J. Kibsgaard, T. F. Jaramillo, F. Besenbacher, Nat. Chem. 2014, 6, 248-253.
6. Y. Li, H. Wang, L. Xie, Y. Liang, G. Hong, H. Dai, J. Am. Chem. Soc. 2011, 133, 7296-7299;
7. D. Merki, X. Hu, Energy Environ. Sci. 2011, 4, 3878-3888;
8. J. Kibsgaard, Z. Chen, B. N. Reinecke, T. F. Jaramillo, Nat. Mater. 2012, 11, 963-969;
9. M. A. Lukowski, A. S. Daniel, F. Meng, A. Forticaux, L. Li, S. Jin, J. Am. Chem. Soc. 2013, 135, 10274-10277;
10. H. Wang, Z. Lu, S. Xu, D. Kong, J. Cha, G. Zheng, P. Hsu, K. Yan, D. Bradshaw, F. Prinz, Y. Cui, Proc. Natl. Acad. Sci. USA 2013, 110, 19701-19706;
11. T. Wang, L. Liu, Z. Zhu, P. Papakonstantinou, J. Hu, H. Liu, M. Li, Energy Environ. Sci. 2013, 6, 625-633;
12. J. Xie, J. Zhang, S. Li, F. Grote, X. Zhang, H. Zhang, R. Wang, Y. Lei, B. Pan, Y. Xie, J. Am. Chem. Soc. 2013, 135, 17881-17888;
13. J. D. Benck, T. R. Hellstern, J. Kibsgaard, P. Chakthranont, T. F. Jaramillo, ACS Catal. 2014, 4, 3957-3971;
14. M. Gao, M. Chan, Y. Sun, Nat. Commun. 2015, 6, 7493;
15. M. Gao, J. Liang, Y. Zheng, Y. Xu, J. Jiang, Q. Gao, J. Li, S. Yu, Nat. Commun. 2015, 6, 5982.
16. A. Müller, W.-O. Nolte, B. Krebs, Angew. Chem. Int. Ed. Engl. 1978, 17, 279-279;
17. Angew. Chem. 1978, 90, 286-287;
18. A. Müller, S. Sarkar, R. G. Bhattacharyya, S. Pohl, M. Dartmann, Angew. Chem. Int. Ed. Engl. 1978, 17, 535-535;
19. Angew. Chem. 1978, 90, 564-565;
20. A. Müller, R. G. Bhattacharyya, B. Pfefferkorn, Chem. Ber. 1979, 112, 778-780;
21. A. Müller, E. Krickemeyer, A. Hadjikyriacou, D. Coucouvanis, in Inorg. Synth., Wiley, Hoboken, 2007, pp. 47-51.
22. H. Fukumoto, Y. Yonezawa, Thin Solid Films 1998, 327, 748-751.
23. B. E. Conway, B. V. Tilak, Electrochim. Acta 2002, 47, 3571-3594.
24. T. Wang, J. Zhuo, K. Du, B. Chen, Z. Zhu, Y. Shao, M. Li, Adv. Mater. 2014, 26, 3761-3766.
25. M. S. Faber, R. Dziedzic, M. A. Lukowski, N. S. Kaiser, Q. Ding, S. Jin, J. Am. Chem. Soc. 2014, 136, 10053-10061;
26. Y. Zheng, Y. Jiao, Y. H. Zhu, L. H. Li, Y. Han, Y. Chen, A. J. Du, M. Jaroniec, S. Z. Qiao, Nat. Commun. 2014, 5, 3783.
27. T. F. Jaramillo, J. Bonde, J. Zhang, B.-L. Ooi, K. Andersson, J. Ulstrup, I. Chorkendorff, J. Phys. Chem. C 2008, 112, 17492-17498.
28. Z. Chen, D. Cummins, B. N. Reinecke, E. Clark, M. K. Sunkara, T. F. Jaramillo, Nano Lett. 2011, 11, 4168-4175;
29. J. Xie, H. Zhang, S. Li, R. Wang, X. Sun, M. Zhou, J. Zhou, X. Lou, Y. Xie, Adv. Mater. 2013, 25, 5807-5813;
30. D. Li, U. Maiti, J. Lim, D. Choi, W. Lee, Y. Oh, G. Lee, S. Kim, Nano. Lett. 2014, 14, 1228-1233;
31. H. Wang, Z. Lu, D. Kong, J. Sun, T. Hymel, Y. Cui, ACS Nano 2014, 8, 4940-4947;
32. J. D. Benck, Z. Chen, L. Y. Kuritzky, A. J. Forman, T. F. Jaramillo, ACS Catal. 2012, 2, 1916-1923.
33. J. Greeley, T. F. Jaramillo, J. Bonde, I. B. Chorkendorff, J. K. Norskov, Nat. Mater. 2006, 5, 909-913;
34. J. K. Nørskov, T. Bligaard, J. Rossmeisl, C. H. Christensen, Nat. Chem. 2009, 1, 37-46.
35. Y. Huang, R. J. Nielsen, W. A. Goddard, M. P. Soriaga, J. Am. Chem. Soc. 2015, 137, 6692-6698;
36. B. Lassalle-Kaiser, D. Merki, H. Vrubel, S. Gul, V. K. Yachandra, X. Hu, J. Yano, J. Am. Chem. Soc. 2015, 137, 314-321;
37. A. M. Appel, D. L. DuBois, M. R. DuBois, J. Am. Chem. Soc. 2005, 127, 12717-12726.
38. Y. Hou, B. L. Abrams, P. C. K. Vesborg, M. E. Bjorketun, K. Herbst, L. Bech, A. M. Setti, C. D. Damsgaard, T. Pedersen, O. Hansen, J. Rossmeisl, S. Dahl, J. K. Norskov, I. Chorkendorff, Nat. Mater. 2011, 10, 434-438.