Lateral size-dependent spontaneous and stimulated emission properties in colloidal CdSe nanoplatelets

ACS Nano

Volumn 9, Issue 5, 2015, Pages 5041-5050

  Olutas, Murat ^a,b   Guzelturk, Burak ^a   Kelestemur, Yusuf ^a   Yeltik, Aydan ^a   Delikanli, Savas ^a   Demir, Hilmi Volkan ^a,c  

^a BILKENT UNIVERSITY   (Turkey)

^b ABANT IZZET BAYSAL UNIVERSITY   (Turkey)

^c NANYANG TECHNOLOGICAL UNIVERSITY   (Singapore)

Author keywords

amplified spontaneous emission; colloidal quantum wells; giant two photon absorption cross section; lateral size; photoluminescence quantum efficiency; semiconductor nanoplatelets; stimulated emission

Indexed keywords

DECAY (ORGANIC); OPTOELECTRONIC DEVICES; PHOTOLUMINESCENCE; PHOTONS; SEMICONDUCTOR QUANTUM DOTS; SEMICONDUCTOR QUANTUM WELLS; SPONTANEOUS EMISSION; STIMULATED EMISSION; TWO PHOTON PROCESSES;

AMPLIFIED SPONTANEOUS EMISSIONS; COLLOIDAL QUANTUM WELLS; LATERAL SIZES; NANO-PLATELETS; PHOTOLUMINESCENCE QUANTUM EFFICIENCY; TWO-PHOTON ABSORPTION CROSS SECTION;

QUANTUM EFFICIENCY;

EID: 84930679068     PISSN: 19360851     EISSN: 1936086X     Source Type: Journal    
DOI: 10.1021/acsnano.5b01927     Document Type: Article

References (53)

1. Murray, C. B.; Norris, D. J.; Bawendi, M. G. Synthesis and Characterization of Nearly Monodisperse CdE (E = S, Se, Te) Semiconductor Nanocrystallites J. Am. Chem. Soc. 1993, 115, 8706-8715
2. Colvin, V. L.; Schlamp, M. C.; Alivisatos, A. P. Light-Emitting Diodes Made from Cadmium Selenide Nanocrystals and a Semiconducting Polymer Nature 1994, 370, 354-357
3. Klimov, V. I.; Mikhailosvsky, A. A.; Xu, S.; Malko, A.; Hollingsworth, J. A.; Leatherdale, C. A.; Eisler, H. J.; Bawendi, M. G. Optical Gain and Stimulated Emission in Nanocrystal Quantum Dots Science 2000, 290, 314-317
4. Semonin, O. E.; Luther, J. M.; Choi, S.; Chen, H.-Y.; Gao, J.; Nozik, A. J.; Beard, M. C. Peak External Photocurrent Quantum Efficiency Exceeding 100% via MEG in a Quantum Dot Solar Cell Science 2011, 334, 1530-1533
5. Dai, X.; Zhang, Z.; Jin, Y.; Niu, Y.; Cao, H.; Liang, X.; Chen, L.; Wang, J.; Peng, X. Solution-Processed, High-Performance Light-Emitting Diodes Based on Quantum Dots Nature 2014, 515, 96-99
6. Lim, J.; Jeong, B. G.; Park, M.; Kim, J. K.; Pietryga, J. M.; Park, Y.-S.; Klimov, V. I.; Lee, C.; Lee, D. C.; Bae, W. K. Influence of Shell Thickness on the Performance of Light-Emitting Devices Based on CdSe/Zn1-X CdX S Core/Shell Heterostructured Quantum Dots Adv. Mater. 2014, 26, 8034-8040
7. Norris, D.; Bawendi, M. Measurement and Assignment of the Size-Dependent Optical Spectrum in CdSe Quantum Dots Phys. Rev. B 1996, 53, 16338-16346
8. Yu, W. W.; Qu, L.; Guo, W.; Peng, X. Experimental Determination of the Extinction Coefficient of CdTe, CdSe, and CdS Nanocrystals Chem. Mater. 2003, 15, 2854-2860
9. Robel, I.; Gresback, R.; Kortshagen, U.; Schaller, R. D.; Klimov, V. I. Universal Size-Dependent Trend in Auger Recombination in Direct-Gap and Indirect-Gap Semiconductor Nanocrystals Phys. Rev. Lett. 2009, 102, 177404
10. Jasieniak, J.; Smith, L.; van Embden, J.; Mulvaney, P.; Califano, M. Re-examination of the Size-Dependent Absorption Properties of CdSe Quantum Dots J. Phys. Chem. C 2009, 113, 19468-19474
11. Leistikow, M.; Johansen, J.; Kettelarij, A.; Lodahl, P.; Vos, W. Size-Dependent Oscillator Strength and Quantum Efficiency of CdSe Quantum Dots Controlled via the Local Density of States Phys. Rev. B 2009, 79, 045301
12. Gong, K.; Zeng, Y.; Kelley, D. F. Extinction Coefficients, Oscillator Strengths, and Radiative Lifetimes of CdSe, CdTe, and CdTe/CdSe Nanocrystals J. Phys. Chem. C 2013, 117, 20268-20279
13. Kambhampati, P. Hot Exciton Relaxation Dynamics in Semiconductor Quantum Dots: Radiationless Transitions on the Nanoscale J. Phys. Chem. C 2011, 115, 22089-22109
14. Kambhampati, P. Multiexcitons in Semiconductor Nanocrystals: A Platform for Optoelectronics at High Carrier Concentration J. Phys. Chem. Lett. 2012, 3, 1182-1190
15. Kambhampati, P. Unraveling the Structure and Dynamics of Excitons in Semiconductor Quantum Dots Acc. Chem. Res. 2011, 44, 1-13
16. Ithurria, S.; Dubertret, B. Quasi 2D Colloidal CdSe Platelets with Thicknesses Controlled at the Atomic Level J. Am. Chem. Soc. 2008, 130, 16504-16505
17. Ithurria, S.; Tessier, M. D.; Mahler, B.; Lobo, R. P. S. M.; Dubertret, B.; Efros, A. L. Colloidal Nanoplatelets with Two-Dimensional Electronic Structure Nat. Mater. 2011, 10, 936-941
18. Biadala, L.; Liu, F.; Tessier, M. D.; Yakovlev, D. R.; Dubertret, B.; Bayer, M. Recombination Dynamics of Band Edge Excitons in Quasi-Two-Dimensional CdSe Nanoplatelets Nano Lett. 2014, 14, 1134-1139
19. Tessier, M. D.; Spinicelli, P.; Dupont, D.; Patriarche, G.; Ithurria, S.; Dubertret, B. Efficient Exciton Concentrators Built from Colloidal Core/Crown CdSe/CdS Semiconductor Nanoplatelets Nano Lett. 2014, 14, 207-213
20. Kunneman, L. T.; Tessier, M. D.; Heuclin, H.; Dubertret, B.; Aulin, Y. V.; Grozema, F. C.; Schins, J. M.; Siebbeles, L. D. A. Bimolecular Auger Recombination of Electron-Hole Pairs in Two-Dimensional CdSe and CdSe/CdZnS Core/Shell Nanoplatelets J. Phys. Chem. Lett. 2013, 4, 3574-3578
21. Mahler, B.; Nadal, B.; Bouet, C.; Patriarche, G.; Dubertret, B. Core/Shell Colloidal Semiconductor Nanoplatelets J. Am. Chem. Soc. 2012, 134, 18591-18598
22. Pelton, M.; Ithurria, S.; Schaller, R. D.; Dolzhnikov, D. S.; Talapin, D. V. Carrier Cooling in Colloidal Quantum Wells Nano Lett. 2012, 12, 6158-6163
23. Achtstein, A. W.; Schliwa, A.; Prudnikau, A.; Hardzei, M.; Artemyev, M. V.; Thomsen, C.; Woggon, U. Electronic Structure and Exciton-Phonon Interaction in Two-Dimensional Colloidal CdSe Nanosheets Nano Lett. 2012, 12, 3151-3157
24. Chen, Z.; Nadal, B.; Mahler, B.; Aubin, H.; Dubertret, B. Quasi-2D Colloidal Semiconductor Nanoplatelets for Narrow Electroluminescence Adv. Funct. Mater. 2014, 24, 295-302
25. She, C.; Fedin, I.; Dolzhnikov, D. S.; Demortière, A.; Schaller, R. D.; Pelton, M.; Talapin, D. V. Low-Threshold Stimulated Emission Using Colloidal Quantum Wells Nano Lett. 2014, 14, 2772-2777
26. Guzelturk, B.; Kelestemur, Y.; Olutas, M.; Delikanli, S.; Demir, H. V. Amplified Spontaneous Emission and Lasing in Colloidal Nanoplatelets ACS Nano 2014, 8, 6599-6605
27. Grim, J. Q.; Christodoulou, S.; Di Stasio, F.; Krahne, R.; Cingolani, R.; Manna, L.; Moreels, I. Continuous-Wave Biexciton Lasing at Room Temperature Using Solution-Processed Quantum Wells Nat. Nanotechnol. 2014, 9, 891-895
28. Guzelturk, B.; Kelestemur, Y.; Gungor, K.; Yeltik, A.; Akgul, M. Z.; Wang, Y.; Chen, R.; Dang, C.; Sun, H.; Demir, H. V. Stable and Low-Threshold Optical Gain in CdSe/CdS Quantum Dots: An All-Colloidal Frequency Up-Converted Laser Adv. Mater. 2015, 27, 2741-2746
29. Achtstein, A. W.; Prudnikau, A. V.; Ermolenko, M. V.; Gurinovich, L. I.; Gaponenko, S. V.; Woggon, U.; Baranov, A. V.; Leonov, M. Y.; Rukhlenko, I. D.; Federov, A. V. et al. Electroabsorption by 0D, 1D, and 2D Nanocrystals: A Comparative Study of CdSe Colloidal Quantum Dots, Nanorods and Nanoplatelets ACS Nano 2014, 8, 7678-7686
30. Abecassis, B.; Tessier, M. D.; Davidson, P.; Dubertret, B. Self-Assembly of CdSe Nanoplatelets into Giant Micrometer-Scale Needles Emitting Polarized Light Nano Lett. 2014, 14, 710-715
31. Guzelturk, B.; Erden, O.; Olutaş, M.; Kelestemur, Y.; Demir, H. V. Stacking in Colloidal Nanoplatelets: Tuning Excitonic Properties ACS Nano 2014, 8, 12524-12533
32. Guzelturk, B.; Olutas, M.; Delikanli, S.; Kelestemur, Y.; Erden, O.; Demir, H. V. Nonradiative Energy Transfer in Colloidal CdSe Nanoplatelet Films Nanoscale 2015, 7, 2545-2551
33. Pedetti, S.; Ithurria, S.; Heuclin, H.; Patriarche, G.; Dubertret, B. Type-II CdSe/CdTe Core/Crown Semiconductor Nanoplatelets J. Am. Chem. Soc. 2014, 136, 16430-16438
34. Prudnikau, A.; Chuvilin, A.; Artemyev, M. CdSe-CdS Nanoheteroplatelets with Efficient Photoexcitation of Central CdSe Region through Epitaxially Grown CdS Wings J. Am. Chem. Soc. 2013, 135, 14476-14479
35. Ithurria, S.; Talapin, D. V. Colloidal Atomic Layer Deposition (c-ALD) Using Self-Limiting Reactions at Nanocrystal Surface Coupled to Phase Transfer between Polar and Nonpolar Media J. Am. Chem. Soc. 2012, 134, 18585-18590
36. Kunneman, L. T.; Schins, J. M.; Pedetti, S.; Heuclin, H.; Grozema, F. C.; Houtepen, A. J.; Dubertret, B.; Siebbeles, L. D. A. Nature and Decay Pathways of Photoexcited States in CdSe and CdSe/CdS Nanoplatelets Nano Lett. 2014, 14, 7039-7045
37. Tessier, M. D.; Mahler, B.; Nadal, B.; Heuclin, H.; Pedetti, S.; Dubertret, B. Spectroscopy of Colloidal Semiconductor Core/Shell Nanoplatelets with High Quantum Yield Nano Lett. 2013, 13, 3321-3328
38. Kelestemur, Y.; Olutas, M.; Delikanli, S.; Guzelturk, B.; Akgul, M. Z.; Demir, H. V. Type-II Colloidal Quantum Wells: CdSe/CdTe Core/Crown Heteronanoplatelets J. Phys. Chem. C 2015, 119, 2177-2185
39. Naeem, A.; Masia, F.; Christodoulou, S.; Moreels, I.; Borri, P.; Langbein, W. Giant Exciton Oscillator Strength and Radiatively Limited Dephasing in Two-Dimensional Platelets Phys. Rev. B 2015, 91, 121302(R)
40. Tessier, M. D.; Biadala, L.; Bouet, C.; Ithurria, S.; Abecassis, B.; Dubertret, B. Phonon Line Emission Revealed by Self-Assembly of Colloidal Nanoplatelets ACS Nano 2013, 3332-3340
41. Tessier, M. D.; Javaux, C.; Maksimovic, I.; Loriette, V.; Dubertret, B. Spectroscopy of Single CdSe Nanoplatelets ACS Nano 2012, 6, 6751-6758
42. Feldmann, J.; Peter, G.; Gobel, E. O. Linewidth Dependence of Radiative Exciton Lifetimes in Quantum Wells Phys. Rev. Lett. 1987, 59, 2337-2340
43. Ithurria, S.; Bousquet, G.; Dubertret, B. Continuous Transition from 3D to 1D Confinement Observed during the Formation of CdSe Nanoplatelets J. Am. Chem. Soc. 2011, 133, 3070-3077
44. Hines, D. A.; Kamat, P. V. Quantum Dot Surface Chemistry: Ligand Effects and Electron Transfer Reactions J. Phys. Chem. C 2013, 117, 14418-14426
45. Knowles, K. E.; Mcarthur, E. A.; Weiss, E. A. A Multi-Timescale Map of Radiative and Nonradiative Decay Pathways for Excitons in CdSe Quantum Dots ACS Nano 2011, 5, 2026-2035
46. Vietmeyer, F.; Tchelidze, T.; Tsou, V.; Janko, B.; Kuno, M. Electric Field-Induced Emission Enhancement and Modulation in Individual CdSe Nanowires ACS Nano 2012, 6, 9133-9140
47. Kambhampati, P. On the Kinetics and Thermodynamics of Excitons at the Surface of Semiconductor Nanocrystals: Are There Surface Excitons? Chem. Phys. 2015, 446, 92-107
48. Mooney, J.; Krause, M. M.; Kambhampati, P. Connecting the Dots: The Kinetics and Thermodynamics of Hot, Cold, and Surface-Trapped Excitons in Semiconductor Nanocrystals J. Phys. Chem. C 2014, 118, 7730-7739
49. Cihan, A. F.; Kelestemur, Y.; Guzelturk, B.; Yerli, O.; Kurum, U.; Yaglioglu, H. G.; Elmali, A.; Demir, H. V. Attractive versus Repulsive Excitonic Interactions of Colloidal Quantum Dots Control Blue- to Red-Shifting (and Non-Shifting) Amplified Spontaneous Emission J. Phys. Chem. Lett. 2013, 4, 4146-4152
50. Kelestemur, Y.; Cihan, A. F.; Guzelturk, B.; Demir, H. V. Type-Tunable Amplified Spontaneous Emission from Core-Seeded CdSe/CdS Nanorods Controlled by Exciton-Exciton Interaction Nanoscale 2014, 6, 8509-8514
51. Guzelturk, B.; Kelestemur, Y.; Akgul, M. Z.; Sharma, V. K.; Demir, H. V. Ultralow Threshold One-Photon- and Two-Photon-Pumped Optical Gain Media of Blue-Emitting Colloidal Quantum Dot Films J. Phys. Chem. Lett. 2014, 5, 2214-2218
52. Xing, G.; Liao, Y.; Wu, X.; Chakrabortty, S.; Liu, X.; Yeow, E. K. L.; Chan, Y.; Sum, T. C. Ultralow-Threshold Two-Photon Pumped Amplified Spontaneous Emission and Lasing from Seeded CdSe/CdS Nanorod Heterostructures ACS Nano 2012, 6, 10835-10844
53. Raymond, J. E.; Bhaskar, A.; Goodson, T.; Makiuchi, N.; Ogawa, K.; Kobuke, Y. Synthesis and Two-Photon Absorption Enhancement of Porphyrin Macrocycles J. Am. Chem. Soc. 2008, 130, 17212-17213