Controlling an electron-transfer reaction at a metal surface by manipulating reactant motion and orientation

Angewandte Chemie - International Edition

Volumn 53, Issue 50, 2014, Pages 13690-13694

  Bartels, Nils ^a   Krüger, Bastian C ^a   Auerbach, Daniel J ^b   Wodtke, Alec M ^a,b   Schäfer, Tim ^a  

^a UNIVERSITY OF GÖTTINGEN   (Germany)

^b MAX PLANCK INSTITUTE FOR BIOPHYSICAL CHEMISTRY   (Germany)

Author keywords

Electron transfer; NO; Surface scattering; Vibrational relaxation; Vibrationally excited molecules

Indexed keywords

DEGREES OF FREEDOM (MECHANICS); ELECTRON TRANSITIONS; MOLECULAR ORIENTATION; MOLECULES; NOBELIUM; OPTICAL PUMPING; SINGLE CRYSTALS; SURFACE SCATTERING;

CONTROL PARAMETERS; ELECTRON TRANSFER; ELECTRON-TRANSFER REACTIONS; REACTANT MOTIONS; SIMPLE MODELING; VIBRATIONAL ENERGIES; VIBRATIONAL RELAXATION; VIBRATIONALLY EXCITED;

SURFACE REACTIONS;

METAL;

CHEMISTRY; ELECTRON; SURFACE PROPERTY;

ELECTRONS; METALS; SURFACE PROPERTIES;

EID: 84918789270     PISSN: 14337851     EISSN: 15213773     Source Type: Journal    
DOI: 10.1002/anie.201407051     Document Type: Article

References (30)

1. a) I. A. Balabin, J.N. Onuchic, Science 2000, 290, 114-117
2. b) P. F. Barbara, T. J. Meyer, M. A. Ratner, J. Phys. Chem. 1996, 100, 13148-13168
3. c) V. Balzani in Electron Transfer in Chemistry (Ed.: V. Balzani), Wiley-VCH, Weinheim, 2008, pp. I-lxxx
4. d) K. B. Yoon, Chem. Rev. 1993, 93, 321-339.
5. J. D. White, J. Chen, D. Matsiev, D. J. Auerbach, A. M. Wodtke, J. Chem. Phys. 2006, 124, 064702.
6. a) Y. Huang, C. T. Rettner, D. J. Auerbach, A. M. Wodtke, Science 2000, 290, 111-114
7. b) R. Cooper, C Bartels, A. Kandratsenka, I. Rahinov, N. Shenvi, K. Golibrzuch, Z. S. Li, D. J. Auerbach, J. C. Tully, A. M. Wodtke, Angew. Chem. Int. Ed. 2012, 51, 4954-4958
8. Angew. Chem. 2012, 124, 5038-5042
9. c) J. D. White, J. Chen, D. Matsiev, D. J. Auerbach, A. M. Wodtke, Nature 2005, 433, 503-505
10. d) N. H. Nahler, J. D. White, J. LaRue, D. J. Auerbach, A. M. Wodtke, Science 2008, 321, 1191-1194
11. e) J. LaRue, T. Schäfer, D. Matsiev, L. Velarde, N. H. Nahler, D. J. Auerbach, A. M. Wodtke, Phys. Chem. Chem. Phys. 2011, 13, 97-99
12. f) J. L. LaRue, T. Schäfer, D. Matsiev, L. Velarde, N H. Nahler, D. J. Auerbach, A. M. Wodtke, J. Phys. Chem. A 2011, 115, 14306-14314
13. g) C T. Rettner, F. Fabre, J. Kimman, D. J. Auerbach, Phys. Rev. Lett. 1985, 55, 1904-1907.
14. a) N Shenvi, S. Roy, J. C Tully, Science 2009, 326, 829-832
15. b) S. Roy, N Shenvi, J. C Tully, J. Phys. Chem. C 2009, 113, 16311-16320
16. c) D. M. Newns, Surf. Sci. 1986, 171, 600-614
17. d) J. W Gadzuk, J. Chem. Phys. 1983, 79, 6341-6348
18. e) S. Monturet, P. Saalfrank, Phys. Rev. B 2010, 82, 075404.
19. a) N Bartels, B. C Krüger, S. Meyer, A. M. Wodtke, T Schäfer, J. Phys. Chem. Lett. 2013, 4, 2367-2370
20. b) N Bartels, K. Golibrzuch, C. Bartels, L. Chen, D. J. Auerbach, A. M. Wodtke, T. Schäfer, Proc. Natl. Acad. Sci. USA 2013, 110, 17738-17743
21. c) K. Golibrzuch, P R. Shirhatti, J. Altschäffel, I. Rahinov, D. J. Auerbach, A. M. Wodtke, C Bartels, J. Phys. Chem. A 2013, 117, 8750-8760
22. d) K. Golibrzuch, PR. Shirhatti, I. Rahinov, D. J. Auerbach, A. M. Wodtke, C. Bartels, Phys. Chem. Chem. Phys. 2014, 16, 7602-7610
23. e) K. Golibrzuch, P. R. Shirhatti, I. Rahinov, A. Kandratsenka, D. J. Auerbach, A. M. Wodtke, C Bartels, J. Chem. Phys. 2014, 140, 044701
24. f) T Schäfer, N Bartels, N Hocke, X. M. Yang, A. M. Wodtke, Chem. Phys. Lett. 2012, 535, 1-11.
25. a) M. Silva, R. Jongma, R. W Field, A. M. Wodtke, Annu. Rev. Phys. Chem. 2001, 52, 811-852
26. b) C. Kittrell, E. Abramson, J. L. Kinsey, S. A. Mcdonald, D. E. Reisner, R. W. Field, D. H. Katayama, J. Chem. Phys. 1981, 75, 2056-2059.
27. a) J. Bulthuis, J. J. Vanleuken, S. Stolte, J. Chem. Soc. Faraday Trans. 1995, 91, 205-214
28. b) J. Chen, D. Matsiev, J. D. White, M. Murphy, A. M. Wodtke, Chem. Phys. 2004, 301, 161-172.
29. A. W. Kleyn, T. C. M. Horn, Phys. Rep. 1991, 199, 191-230.
30. N. Bartels, K. Golibrzuch, C. Bartels, L. Chen, D. J. Auerbach, A. M. Wodtke, T. Schäfer, J. Chem. Phys. 2014, 140, 054710.