Electrochemical degradation of nitrobenzene by anodic oxidation on the constructed TiO2-NTs/SnO2-Sb/PbO2 electrode

Chemosphere

Volumn 113, Issue , 2014, Pages 48-55

  Chen, Yong ^a,b   Li, Hongyi ^b,c   Liu, Weijing ^a   Tu, Yong ^a   Zhang, Yaohui ^a   Han, Weiqing ^b   Wang, Lianjun ^b  

^a Jiangsu Provincial Academy of Environmental Science   (China)

^b NANJING UNIVERSITY OF SCIENCE AND TECHNOLOGY   (China)

^c NANJING INSTITUTE OF TECHNOLOGY   (China)

Author keywords

Electrochemical oxidation; Enhanced mechanism; Hydroxyl radicals; Nitrobenzene

Indexed keywords

ANODIC OXIDATION; ANTIMONY COMPOUNDS; ELECTROCHEMICAL OXIDATION; LEAD OXIDE; NITROBENZENE; REACTION INTERMEDIATES; TITANIUM DIOXIDE;

COMBUSTION EFFICIENCIES; DEGRADATION INTERMEDIATES; ELECTROCHEMICAL DEGRADATION; ELECTROCHEMICAL PERFORMANCE; ELECTRODEPOSITION PROCESS; HYDROXYL RADICALS; NITROBENZENE OXIDATION; PSEUDO-FIRST ORDER REACTIONS;

ELECTROCHEMICAL ELECTRODES;

ANTIMONY; LEAD; LEAD DIOXIDE; NANOTUBE; NITROBENZENE; TIN OXIDE; TITANIUM DIOXIDE; UNCLASSIFIED DRUG;

BENZENE; BIOACCUMULATION; BIODEGRADATION; COMBUSTION; ELECTROCHEMICAL METHOD; ELECTRODE; HYDROXYL RADICAL; OXIDATION; OXIDE;

ARTICLE; CHEMICAL REACTION; CHEMICAL STRUCTURE; COMBUSTION; CRYSTAL; DEGRADATION; ELECTROCHEMISTRY; ELECTRODE; ELECTROLYSIS; KINETICS; MASS FRAGMENTOGRAPHY; MORPHOLOGY; OXIDATION; REACTION ANALYSIS;

CONSTRUCTED PBO(2) ELECTRODE; ELECTROCHEMICAL OXIDATION; ENHANCED MECHANISM; HYDROXYL RADICALS; NITROBENZENE;

ANTIMONY; ELECTROCHEMICAL TECHNIQUES; ELECTRODES; ENVIRONMENTAL REMEDIATION; GAS CHROMATOGRAPHY-MASS SPECTROMETRY; KINETICS; LEAD; NANOTUBES; NITROBENZENES; OXIDATION-REDUCTION; TIN COMPOUNDS; TITANIUM; WASTE WATER; WATER PURIFICATION;

EID: 84904671747     PISSN: 00456535     EISSN: 18791298     Source Type: Journal    
DOI: 10.1016/j.chemosphere.2014.03.122     Document Type: Article

References (34)

1. Andrade L.S., Ruotolo L.A.M., Rocha-Filho R.C., Bocchi N., Biaggio S.R., Iniesta J., Garcia-Garcia V., Montiel V. On the performance of Fe and Fe, F doped Ti-Pt/PbO2 electrodes in the electrooxidation of the Blue Reactive 19 dye in simulated textile wastewater. Chemosphere 2007, 66:2035-2043.
2. 2 electrodes doped with Ru and Pt. Electrochim. Acta 2009, 54:5230-5238.
3. Bhatkhandea D.S., Pangarkara V.G., Beenackers A.A.C.M. Photocatalytic degradation of nitrobenzene using titanium dioxide and concentrated solar radiation: chemical effects and scaleup. Water Res. 2003, 37:1223-1230.
4. Blood P.J., Brown I.J., Sotiropoulos S. Electrodeposition of lead dioxide on carbon substrates from a high internal phase emulsion (HIPE). J. Appl. Electrochem. 2004, 34:1-7.
5. 2+ and UVA light on the electrochemical degradation of nitrobenzene using an oxygen-diffusion cathode. New J. Chem. 2004, 28:314-322.
6. Cañizares P., Lobato J., Paz R., Rodrigo M.A., Saez C. Advanced oxidation processes for the treatment of olive-oil mills wastewater. Chemosphere 2007, 67:832-838.
7. 2 anodes. Electrochim. Acta 2009, 54:2595-2602.
8. 2 evolution with low Ir content. J. Phys. Chem. B 2001, 105:4623-4628.
9. 2-Sb electrodes by electrodeposition. J. Electroanal. Chem. 2010, 648:119-127.
10. Chen Y., Hong L., Han W., Wang L., Sun X., Li J. Treatment of high explosive production wastewater containing RDX by combined electrocatalytic reaction and anoxic-oxic biodegradation. Chem. Eng. J. 2011, 168:1256-1262.
11. Comninellis Ch. Electrocatalysis in the electrochemical conversion/combustion of organic pollutants for waste water treatment. Electrochim. Acta 1994, 39:1857-1862.
12. Comninellis Ch., Vercesi G.P. Characterization of DSA-type oxygen evolving electrodes: choice of a coating. J. Appl. Electrochem. 1991, 21:335-345.
13. 2 nanotubes. Nano Lett. 2006, 6:1080-1082.
14. Hyde M.E., Jacobs R.M.J., Compton R.G. An AFM study of the correlation of lead dioxide electrocatalytic activity with observed morphology. J. Phys. Chem. B 2004, 108:6381-6390.
15. 2 electrodes doped with different rare earth oxides. Electrochim. Acta 2007, 53:2048-2054.
16. Liu Y., Liu H., Li Y. Comparative study of the electrocatalytic oxidation and mechanism of nitrophenols at Bi-doped lead dioxide anodes. Appl. Catal. B: Environ. 2008, 84:297-302.
17. Martinez-Huitle C.A., Ferro S., De Battisti A. Electrochemical incineration of oxalic acid: role of electrode material. Electrochim. Acta 2004, 49:4027-4034.
18. Miwa D.W., Malpass G.R.P., Machado S.A.S., Motheo A.J. Electrochemical degradation of carbaryl on oxide electrodes. Water Res. 2006, 40:3281-3289.
19. 2 nanotube arrays via anodization of titanium thin films. Adv. Funct. Mater. 2005, 15:1291-1296.
20. Pacheco M.J., Morao A., Lopes A., Ciriaco L., Goncalves I. Degradation of phenols using boron-doped diamond electrodes: a method for quantifying the extent of combustion. Electrochim. Acta 2007, 53:629-636.
21. Panizza M., Cerisola G. Direct and mediated anodic oxidation of organic pollutants. Chem. Rev. 2009, 109:6541-6569.
22. Panizza M., Kapalka A., Comninellis C. Oxidation of organic pollutants on BDD anodes using modulated current electrolysis. Electrochim. Acta 2008, 53:2289-2295.
23. Samet Y., Agengui L., Abdelhedi R. Electrochemical degradation of chlorpyrifos pesticide in aqueous solutions by anodic oxidation at boron-doped diamond electrodes. Chem. Eng. J. 2010, 161:167-172.
24. 2 as high oxidation power anodes. J. Electroanal. Chem. 2008, 613:151-159.
25. State Environmental Protection Administration of China Water and Wastewater Analytical Methods 2002, China Environmental Press, Beijing, (in Chinese). fourth ed.
26. Tai C., Peng J.F., Liu J.F., Jiang G.B., Zou H. Determination of hydroxyl radicals in advanced oxidation processes with dimethyl sulfoxide trapping and liquid chromatography. Anal. Chim. Acta 2004, 527:73-80.
27. 2-based oxide electrodes. J. Electroanal. Chem. 2010, 649:9-15.
28. Torres R.A., Torres W., Peringer P., Pulgarin C. Electrochemical degradation of p-substituted phenols of industrial interest on Pt electrodes. Attempt of a structure-reactivity relationship assessment. Chemosphere 2003, 50:97-104.
29. Un U.T., Altay U., Koparal A.S., Ogutveren U.B. Complete treatment of olive mill wastewaters by electrooxidation. Chem. Eng. J. 2008, 139:445-452.
30. Velichenko A.B., Amadelli R., Baranova E.A., Girenko D.V., Danilov F.I. Electrodeposition of Co-doped lead dioxide and its physicochemical properties. J. Electroanal. Chem. 2002, 527:56-64.
31. 2 electrode for the degradation of 2,4-dichlorophenol in aqueous solution. Chemosphere 2010, 79:987-996.
32. Xia K., Xie F., Ma Y. Degradation of nitrobenzene in aqueous solution by dual-pulse ultrasound enhanced electrochemical process. Ultrason. Sonochem. 2014, 21:549-553.
33. Zhao G., Zhang Y., Lei Y., Lv B., Gao J., Zhang Y., Li D. Fabrication and electrochemical treatment application of a novel lead dioxide anode with superhydrophobic surfaces, high oxygen evolution potential, and oxidation capability. Environ. Sci. Technol. 2010, 44:1754-1759.
34. Zhu X., Shi S., Wei J., Lv F., Zhao H., Kong J., He Q., Ni J. Electrochemical oxidation characteristics of p-substituted phenols using a boron-doped diamond electrode. Environ. Sci. Technol. 2007, 41:6541-6546.