Oxidative degradation of organic pollutants in aqueous solution using zero valent copper under aerobic atmosphere condition

Journal of Hazardous Materials

Volumn 275, Issue , 2014, Pages 193-199

  Wen, Gang ^a   Wang, Sheng Jun ^b,c   Ma, Jun ^b   Huang, Ting Lin ^a   Liu, Zheng Qian ^d   Zhao, Lei ^b   Xu, Jin Lan ^a  

^a XI'AN UNIVERSITY OF ARCHITECTURE AND TECHNOLOGY   (China)

^b HARBIN INSTITUTE OF TECHNOLOGY   (China)

^c Beijing General Municipal Engineering Design and Research Institute   (China)

^d HUAZHONG UNIVERSITY OF SCIENCE AND TECHNOLOGY   (China)

Author keywords

Hydroxyl radical; Mechanism; Organic pollutants; Oxidative degradation; Zero valent copper

Indexed keywords

DEGRADATION; MECHANISMS; ORGANIC POLLUTANTS; SOLUTIONS;

CONCURRENT REDUCTION; FENTON-LIKE REACTIONS; HYDROXYL RADICALS; MECHANISM INVESTIGATION; OXIDATION CAPACITY; OXIDATIVE DEGRADATION; PSEUDO-FIRST ORDER KINETICS; ZERO-VALENT COPPERS;

COPPER;

ALUMINUM; COPPER; HYDROGEN PEROXIDE; HYDROXYL RADICAL; OXYGEN; PHTHALIC ACID DIETHYL ESTER; TERT BUTYL ALCOHOL; UNCLASSIFIED DRUG; ZERO VALENT COPPER; PHTHALIC ACID DERIVATIVE; SOLUTION AND SOLUBILITY; WATER POLLUTANT;

ALUMINUM; AQUEOUS SOLUTION; HYDROXYL RADICAL; ORGANIC POLLUTANT; OXIDATION; PH; REACTION KINETICS;

AQUEOUS SOLUTION; ARTICLE; DEGRADATION KINETICS; DISSOLUTION; FENTON REACTION; ORGANIC POLLUTANT; OXIDATION; PH; POLLUTANT; CHEMISTRY; OXIDATION REDUCTION REACTION; SOLUTION AND SOLUBILITY; WATER POLLUTANT;

COPPER; HYDROGEN PEROXIDE; HYDROGEN-ION CONCENTRATION; HYDROXYL RADICAL; OXIDATION-REDUCTION; OXYGEN; PHTHALIC ACIDS; SOLUTIONS; WATER POLLUTANTS, CHEMICAL;

EID: 84901198905     PISSN: 03043894     EISSN: 18733336     Source Type: Journal    
DOI: 10.1016/j.jhazmat.2014.05.002     Document Type: Article

References (37)

1. Schwarzenbach R.P., Escher B.I., Fenner K., Hofstetter T.B., Johnson C.A., von Gunten U., Wehrli B. The challenge of micropollutants in aquatic systems. Science 2006, 313:1072-1077.
2. Alexander M. Biodegradation of organic chemicals. Environ. Sci. Technol. 1985, 19:106-111.
3. Pera-Titus M., García-Molina V., Banos M.A., Giménez J., Esplugas S. Degradation of chlorophenols by means of advanced oxidation processes: a general review. Appl. Catal., B: Environ. 2004, 47:219-256.
4. Saritha P., Aparna C., Himabindu V., Anjaneyulu Y. Comparison of various advanced oxidation processes for the degradation of 4-chloro-2 nitrophenol. J. Hazard. Mater. 2007, 149:609-614.
5. Joseph C.G., Li Puma G., Bono A., Krishnaiah D. Sonophotocatalysis in advanced oxidation process: a short review. Ultrason. Sonochem. 2009, 16:583-589.
6. Noradoun C.E., Cheng I.F. EDTA degradation induced by oxygen activation in a zero valent iron/air/water system. Environ. Sci. Technol. 2005, 39:7158-7163.
7. Keenan C.R., Sedlak D.L. Factors affecting the yield of oxidants from the reaction of nanoparticulate zero-valent iron and oxygen. Environ. Sci. Technol. 2008, 42:1262-1267.
8. Stieber M., Putschew A., Jekel M. Treatment of pharmaceuticals and diagnostic agents using zero-valent iron-kinetic studies and assessment of transformation products assay. Environ. Sci. Technol. 2011, 45:4944-4950.
9. Bokare A.D., Choi W. Zero-valent aluminum for oxidative degradation of aqueous organic pollutants. Environ. Sci. Technol. 2009, 43:7130-7135.
10. Liu W., Zhang H., Cao B., Lin K., Gan J. Oxidative removal of bisphenol A using zero valent aluminum-acid system. Water Res. 2011, 45:1872-1878.
11. 2/acid system. J. Chem. Technol. Biotechnol. 2013, 88:2181-2187.
12. Zhang H., Cao B., Liu W., Lin K., Feng J. Oxidative removal of acetaminophen using zero valent aluminum-acid system: efficacy, influencing factors, and reaction mechanism. J. Environ. Sci. 2012, 24:314-319.
13. Keenan C.R., Sedlak D.L. Ligand-enhanced reactive oxidant generation by nanoparticulate zero-valent iron and oxygen. Environ. Sci. Technol. 2008, 42:6936-6941.
14. Fan J.H., Ma L.M. The pretreatment by the Fe-Cu process for enhancing biological degradability of the mixed wastewater. J. Hazard. Mater. 2009, 164:1392-1397.
15. 2 at normal temperature and pressure. Chem. Eng. J. 2014, 236:274-284.
16. Liu X., Fan J.H., Ma L.M. Oxidative degradation of EDTA in aqueous solution by the bimetallic Fe-Cu. Water Air Soil Pollut. 2013, 224:1-11.
17. Lee C., Sedlak D.L. Enhanced formation of oxidants from bimetallic nickel-iron nanoparticles in the presence of oxygen. Environ. Sci. Technol. 2008, 42:8528-8533.
18. Huang C.C., Lo S.L., Lien H.L. Zero-valent copper nanoparticles for effective dechlorination of dichloromethane using sodium borohydride as a reductant. Chem. Eng. J. 2012, 203:95-100.
19. Lin C.J., Lo S.L., Liou Y.H. Degradation of aqueous carbon tetrachloride by nanoscale zero-valent copper on a cation resin. Chemosphere 2005, 59:1299-1307.
20. Chand R., Ince N.H., Gogate P.R., Bremner D.H. Phenol degradation using 20, 300 and 520kHz ultrasonic reactors with hydrogen peroxide, ozone and zero valent metals. Sep. Purif. Technol. 2009, 67:103-109.
21. Stumm W., Morgan J.J. Aquatic chemistry: chemical equilibria and rates in natural waters 2012, John Wiley & Sons, New York.
22. APHA Standard Methods for the Examination of Water and Wastewater 1998, American Public Health Association, Washington, DC.
23. 2. J. Hazard. Mater. 2011, 195:371-377.
24. Bader H., Sturzenegger V., Hoigne J. Photometric method for the determination of low concentrations of hydrogen peroxide by the peroxidase catalyzed oxidation of N,N-diethyl-p-phenylenediamine (DPD). Water Res. 1988, 22:1109-1115.
25. Wen G., Pan Z.H., Ma J., Liu Z.Q., Zhao L., Li J.J. Reuse of sewage sludge as a catalyst in ozonation-efficiency for the removal of oxalic acid and the control of bromate formation. J. Hazard. Mater. 2012, 239-240:381-388.
26. Wen G., Wang S.J., Ma J., Huang T.L., Liu Z.Q., Zhao L., Su J.F. Enhanced ozonation degradation of di-n-butyl phthalate by zero-valent zinc in aqueous solution: performance and mechanism. J. Hazard. Mater. 2014, 265:69-78.
27. Moffett J.W., Zika R.G., Petasne R.G. Evaluation of bathocuproine for the spectro-photometric determination of copper(I) in copper redox studies with applications in studies of natural waters. Anal. Chim. Acta 1985, 175:171-179.
28. Liang L., Sun W., Guan X., Huang Y., Choi W., Bao H., Li L., Jiang Z. Weak magnetic field significantly enhances selenite removal kinetics by zero valent iron. Water Res. 2013, 49:371-380.
29. Neta P., Huie R.E., Ross A.B. Rate constants for reactions of inorganic radicals in aqueous solution. J. Phys. Chem. Ref. Data 1988, 17:1027-1284.
30. Welham N., Malatt K., Vukcevic S. The effect of solution speciation on iron-sulphur-arsenic-chloride systems at 298K. Hydrometallurgy 2000, 57:209-223.
31. Lewis E.A., Tolman W.B. Reactivity of dioxygen-copper systems. Chem. Rev. 2004, 104:1047-1076.
32. Eberhardt M.K., Ramirez G., Ayala E. Does the reaction of copper(I) with hydrogen peroxide give hydroxyl radicals? A study of aromatic hydroxylation. J. Org. Chem. 1989, 54:5922-5926.
33. 2+ aq. J. Am. Chem. Soc. 1988, 110:4293-4297.
34. Moffett J.W., Zika R.G. Reaction kinetics of hydrogen peroxide with copper and iron in seawater. Environ. Sci. Technol. 1987, 21:804-810.
35. Moffett J.W., Zika R.G. Oxidation kinetics of Cu(I) in seawater: implications for its existence in the marine environment. Mar. Chem. 1983, 13:239-251.
36. Chelikani P., Fita I., Loewen P. Diversity of structures and properties among catalases. Cell. Mol. Life Sci. 2004, 61:192-208.
37. Ma J., Graham N.J. Degradation of atrazine by manganese-catalysed ozonation-influence of radical scavengers. Water Res. 2000, 34:3822-3828.