Oxidation of aquatic pollutants by ferrous-oxalate complexes under dark aerobic conditions

Journal of Hazardous Materials

Volumn 274, Issue , 2014, Pages 79-86

  Lee, Jaesang ^a   Kim, Jungwon ^b   Choi, Wonyong ^c  

^a Korea University   (South Korea)

^b Hallym University   (South Korea)

^c Pohang University of Science and Technology (POSTECH)   (South Korea)

Author keywords

Dark aerobic reaction; Ferrous oxalate complexes; OH radicals; Oxidation; Water treatment

Indexed keywords

DEGRADATION; ELECTROLYTIC REDUCTION; FREE RADICALS; IRON; OXIDATION; OXYGEN; RATE CONSTANTS; WATER POLLUTION; WATER TREATMENT;

4-CHLOROPHENOL (4-CP); AEROBIC REACTION; DEGRADATION KINETICS; DEGREE OF DEGRADATION; FERROUS-OXALATE COMPLEXES; OH RADICAL; OXIDATIVE DEGRADATION; TWO-ELECTRON REDUCTION;

OXALIC ACID;

4 CHLOROPHENOL; ACETIC ACID; CITRIC ACID; EDETIC ACID; HYDROGEN PEROXIDE; IRON COMPLEX; MALONIC ACID; OXALIC ACID DERIVATIVE; OXYGEN; WATER; ACETIC ACID DERIVATIVE; FERROUS ION; HYDROXYL RADICAL; MALONIC ACID DERIVATIVE; WATER POLLUTANT;

CHLOROPHENOL; DEGRADATION; HYDROXYL RADICAL; IRON; LIGAND; OXALATE; OXIC CONDITIONS; OXIDATION; PH; REACTION KINETICS; REACTION RATE; WATER TREATMENT;

ARTICLE; DEGRADATION KINETICS; ELECTRON; OXIDATION; PH; WATER POLLUTANT; CHEMISTRY; OXIDATION REDUCTION REACTION; PROCEDURES; WATER MANAGEMENT;

ACETATES; CITRIC ACID; EDETIC ACID; FERROUS COMPOUNDS; HYDROGEN PEROXIDE; HYDROXYL RADICAL; MALONATES; OXALATES; OXIDATION-REDUCTION; OXYGEN; WATER POLLUTANTS, CHEMICAL; WATER PURIFICATION;

EID: 84899680584     PISSN: 03043894     EISSN: 18733336     Source Type: Journal    
DOI: 10.1016/j.jhazmat.2014.03.056     Document Type: Article

References (45)

1. Balmer M.E., Sulzberger B. Atrazine degradation in irradiated iron/oxalate systems: effects of pH and oxalate. Environ. Sci. Technol. 1999, 33:2418-2424.
2. Liu G., Zheng S., Xing X., Li Y., Yin D., Ding Y. Fe(III)-oxalate complexes mediated photolysis of aqueous alkylphenol ethoxylates under simulated sunlight conditions. Chemosphere 2010, 78:402-408.
3. Ou X., Quan X., Chen S., Zhang F., Zhao Y. Photocatalytic reaction by Fe(III)-citrate complex and its effect on the photodegradation of atrazine in aqueous solution. J. Photochem. Photobiol. A 2008, 197:382-388.
4. Abida O., Kolar M., Jirkovsky J., Mailhot G. Degradation of 4-chlorophenol in aqueous solution photoinduced by Fe(III)-citrate complex. Photochem. Photobiol. Sci. 2012, 11:794-802.
5. Chen Y., Liu Z., Wang Z., Xue M., Zhu X., Tao T. Photodegradation of propranolol by Fe(III)-citrate complexes: kinetics, mechanism and effect of environmental media. J. Hazard. Mater. 2011, 194:202-208.
6. Zhang C., Wang L., Pan G., Wu F., Deng N., Mailhot G., Mestankova H., Bolte M. Degradation of atrazine photoinduced by Fe(III)-pyruvate complexes in the aqueous solution. J. Hazard. Mater. 2009, 169:772-779.
7. II-tiron complex: reaction kinetics and mechanisms. Environ. Sci. Technol. 2013, 47:11023-11031.
8. Hakala J.A., Chin Y.-P. Abiotic reduction of pendimethalin and trifluralin in controlled and natural systems containing Fe(II) and dissolved organic matter. J. Agric. Food Chem. 2010, 58:12840-12846.
9. Naka D., Kim D., Strathmann T.J. Abiotic reduction of nitroaromatic compounds by aqueous iron(II)-catechol complexes. Environ. Sci. Technol. 2006, 40:3006-3012.
10. Naka D., Kim D., Carbonaro R.F., Strathmann T.J. Abiotic reduction of nitroaromatic contaminants by iron(II) complexes with organothiol ligands. Environ. Toxicol. Chem. 2008, 27:1257-1266.
11. Kim D., Strathmann T.J. Role of organically complexed iron(II) species in the reductive transformation of RDX in anoxic environments. Environ. Sci. Technol. 2007, 41:1257-1264.
12. Sanchez I., Stüber F., Font J., Fortuny A., Fabregat A., Bengoa C. Elimination of phenol and aromatic compounds by zero valent iron and EDTA at low temperature and atmospheric pressure. Chemosphere 2007, 68:338-344.
13. Zhou T., Lim T.-T., Li Y., Lu X., Wong F.-S. The role and fate of EDTA in ultrasound-enhanced zero-valent iron/air system. Chemosphere 2010, 78:576-582.
14. Zhou T., Lim T.-T., Lu X., Li Y., Wong F.-S. Simultaneous degradation of 4CP and EDTA in a heterogeneous ultrasound/fenton like system at ambient circumstance. Sep. Purif. Technol. 2009, 68:367-374.
15. Noradoun C.E., Mekmaysy C.S., Hutcheson R.M., Cheng I.F. Detoxification of malathion a chemical warfare agent analog using oxygen activation at room temperature and pressure. Green Chem. 2005, 7:426-430.
16. Luther G.W., Shellenbarger P.A., Brendel P.J. Dissolved organic Fe(III) and Fe(II) complexes in salt marsh porewaters. Geochim. Cosmochim. Acta 1996, 60:951-960.
17. Lovley D.R., Holmes D.E., Nevin K.P. Dissimilatory Fe(III) and Mn(IV) reduction. Adv. Microb. Physiol. 2004, 49:219-286.
18. Chin Y.-P., Traina S.J., Swank C.R., Backhus D. Abundance and properties of dissolved organic matter in pore waters of a freshwater wetland. Limnol. Oceanogr. 1998, 43:1287-1296.
19. Pirkanniemi K., Metsärinne S., Sillanpää M. Degradation of EDTA and novel complexing agents in pulp and paper mill process and waste waters by Fenton's reagent. J. Hazard. Mater. 2007, 147:556-561.
20. Shimada M., Akamtsu Y., Tokimatsu T., Mii K., Hattori T. Possible biochemical roles of oxalic acid as a low molecular weight compound involved in brown-rot and white-rot wood decays. J. Biotechnol. 1997, 53:103-113.
21. Fortune W.B., Mellon M.G. Determination of iron with o-phenanthroline: a spectrophotometric study. Ind. Eng. Chem. Anal. Ed. 1938, 10:60-64.
22. CRC Handbook of Chemistry and Physics 1996, 10-189. CRC Press Inc., New York, NY. 77th ed. R.L. David (Ed.).
23. Sawyer D.T., Valentine J.S. How super is superoxide?. Acc. Chem. Res. 1981, 14:393-400.
24. Rose A.L., Waite T.D. Kinetic model for Fe(II) oxidation in seawater in the absence and presence of natural organic matter. Environ. Sci. Technol. 2002, 36:433-444.
25. II: influence of organic ligands and natural organic matter. Environ. Sci. Technol. 2002, 36:5172-5183.
26. Park J.S.B., Wood P.M., Davies M.J., Gilbert B.C., Whitwood A.C. A kinetic and ESR investigation of iron(II) oxalate oxidation by hydrogen peroxide and dioxygen as a source of hydroxyl radicals. Free Rad. Res. 1997, 27:447-458.
27. Hyde S.M., Wood P.M. A mechanism for production of hydroxyl radicals by the brown-rot fungus coniophora puteana: Fe(III) reduction by cellobiose dehydrogenase and Fe(II) oxidation at a distance from the hyphae. Microbiology 1997, 143:259-266.
28. Wardman P. Reduction potentials of one electron couples involving free radicals in aqueous solution. J. Phys. Chem. Ref. Data 1989, 18:1637-1755.
29. 2 surface on anoxic photocatalytic degradation of organic compounds. Chem. Commun. 2008, 756-758.
30. Kim J., Choi W. Hydrogen producing water treatment through solar photocatalysis. Energy Environ. Sci. 2010, 3:1042-1045.
31. Lingane J.J. Interpretation of the polarographic waves of complex metal ions. Chem. Rev. 1941, 29:1-35.
32. Chandra I., Jeffrey M.I. A fundamental study of ferric oxalate for dissolving gold in thiosulfate solutions. Hydrometallurgy 2005, 77:191-201.
33. -) in aqueous solution. J. Phys. Chem. Ref. Data 1988, 17:513-886.
34. Gözmen B., Oturan M.A., Oturan N., Erbatur O. Indirect electrochemical treatment of bisphenol A in water via electrochemically generated Fenton's reagent. Environ. Sci. Technol. 2003, 37:3716-3723.
35. Zimbron J.A., Reardon K.F. Hydroxyl free radical reactivity toward aqueous chlorinated phenols. Water Res. 2005, 39:865-869.
36. Lopez A., Kiwi J. Modeling the performance of an innovative membrane-based reactor. abatement of azo dye (orange II) up to biocompatibility. Ind. Eng. Chem. Res. 2001, 40:1852-1858.
37. Mabury S.A., Crosby D.G. The relationship of hydroxyl reactivity to pesticide persistence. Aquatic and Surface Photochemistry 1994, 149-162. CRC Press Inc., Boca Raton, FL. G.R. Helz, R.G. Zepp, D.G. Crosby (Eds.).
38. Wink D.A., Nims R.W., Desrosiers M.F., Ford P.C., Keefer L.K. A kinetic investigation of intermediates formed during the fenton reagent mediated degradation of N-nitrosodimethylamine: evidence for an oxidative pathway not involving hydroxyl radical. Chem. Res. Toxicol. 1991, 4:510-512.
39. Motohashi N., Saito Y. Competitive measurement of rate constants for hydroxyl radical reactions using radiolytic hydroxylation of benzoate. Chem. Pharm. Bull. 1993, 41:1842-1845.
40. Dwibedy P., Dey G.R., Naik D.B., Kishore K. Rate constants for the reaction of OH radicals with some amino polycarboxylic acids. Int. J. Chem. Kinet. 2000, 32:99-104.
41. Gutteridge J.M.C., Halliwell B. The deoxyribose assay: an assay both for 'free' hydroxyl radical and for site-specific hydroxyl radical production. Biochem. J. 1988, 253:932-933.
42. Ervens B., Gligorovski S., Herrmann H. Temperature-dependent rate constants for hydroxyl radical reactions with organic compounds in aqueous solutions. Phys. Chem. Chem. Phys. 2003, 5:1811-1824.
43. Dükkanci M., Gündüz G. Ultrasonic degradation of oxalic acid in aqueous solutions. Ultrason. Sonochem. 2006, 13:517-522.
44. An T., Li G., Zhu X., Fu J., Sheng G., Kun Z. Photoelectrocatalytic degradation of oxalic acid in aqueous phase with a novel three-dimensional electrode-hollow quartz tube photoelectrocatalytic reactor. Appl. Catal., A: Gen. 2005, 279:247-256.
45. Bravo D., Braissant O., Solokhina A., Clerc M., Daniels A.U., Verrecchia E., Junier P. Use of an isothermal microcalorimetry assay to characterize microbial oxalotrophic activity. FEMS Microbiol. Ecol. 2011, 78:266-274.