Formation of light absorbing organo-nitrogen species from evaporation of droplets containing glyoxal and ammonium sulfate

Environmental Science and Technology

Volumn 47, Issue 22, 2013, Pages 12819-12826

  Lee, Alex K Y ^a   Zhao, Ran ^a   Li, Richard ^a   Liggio, John ^b   Li, Shao Meng ^b   Abbatt, Jonathan P D ^a  

^a UNIVERSITY OF TORONTO   (Canada)

^b ENVIRONMENT CANADA   (Canada)

Author keywords

[No Author keywords available]

Indexed keywords

ABSORBING MATERIALS; AEROSOL CHEMISTRY; AEROSOL MASS SPECTROMETRY; AMMONIUM SULFATE; AQUEOUS DROPLETS; DROPLET EVAPORATION; INORGANIC-ORGANIC; ORDERS OF MAGNITUDE;

AEROSOLS; ATMOSPHERIC CHEMISTRY; MASS SPECTROMETRY; NITROGEN; SALTS; VOLATILE ORGANIC COMPOUNDS;

DROPS;

AMMONIUM SULFATE; GLYOXAL; ORGANONITROGEN DERIVATIVE; SULFATE; CARBON; ION; NITROGEN; ORGANIC COMPOUND; SOLUTION AND SOLUBILITY; WATER;

AEROSOL; AMMONIUM SULFATE; AQUEOUS SOLUTION; EVAPORATION; LIGHT AVAILABILITY; REACTION KINETICS; TIMESCALE;

ARTICLE; EVAPORATION; MASS SPECTROMETRY; ATMOSPHERE; CHEMISTRY; LIGHT; RADIATION ABSORPTION; SOLUTION AND SOLUBILITY; TIME; VOLATILIZATION;

ABSORPTION, RADIATION; AMMONIUM SULFATE; ATMOSPHERE; CARBON; GLYOXAL; IONS; LIGHT; MASS SPECTROMETRY; NITROGEN; ORGANIC CHEMICALS; SOLUTIONS; TIME FACTORS; VOLATILIZATION; WATER;

EID: 84888251923     PISSN: 0013936X     EISSN: 15205851     Source Type: Journal    
DOI: 10.1021/es402687w     Document Type: Article

References (39)

1. Blando, J. D.; Turpin, B. J. Secondary organic aerosol formation in cloud and fog droplets: a literature evaluation of plausibility Atmos. Environ. 2000, 34, 1623-1632
2. Lim, Y. B.; Tan, Y.; Perri, M. J.; Seitzinger, S. P.; Turpin, B. J. Aqueous chemistry and its role in secondary organic aerosol (SOA) formation Atmos. Chem. Phys. 2010, 10, 10521-10539
3. Ervens, B.; Volkamer, R. Glyoxal processing by aerosol multiphase chemistry: towards a kinetic modeling framework of secondary organic aerosol formation in aqueous particles Atmos. Chem. Phys. 2010, 10, 8219-8244
4. Lee, A. K. Y.; Hayden, K. L.; Herckes, P.; Leaitch, W. R.; Liggio, J.; Macdonald, A. M.; Abbatt, J. P. D. Characterization of aerosol and cloud water at a mountain site during WACS 2010: secondary organic aerosol formation through oxidative cloud processing Atmos. Chem. Phys. 2012, 12, 7103-7116
5. Kroll, J. H.; Ng, N. L.; Murphy, S. M.; Varutbangkul, V.; Flagan, R. C.; Seinfeld, J. H. Chamber studies of secondary organic aerosol growth by reactive uptake of simple carbonyl compounds J. Geophys. Res.-Atmos. 2005, 110, D23207
6. Ip, H. S. S.; Huang, X. H. H.; Yu, J. Z. Effective Henry's law constants of glyoxal, glyoxylic acid, and glycolic acid Geophys. Res. Lett. 2009, 36, L01802
7. Aiken, A. C.; Decarlo, P. F.; Kroll, J. H.; Worsnop, D. R.; Huffman, J. A.; Docherty, K. S.; Ulbrich, I. M.; Mohr, C.; Kimmel, J. R.; Sueper, D.; Sun, Y.; Zhang, Q.; Trimborn, A.; Northway, M.; Ziemann, P. J.; Canagaratna, M. R.; Onasch, T. B.; Alfarra, M. R.; Prevot, A. S. H.; Dommen, J.; Duplissy, J.; Metzger, A.; Baltensperger, U.; Jimenez, J. L. O/C and OM/OC ratios of primary, secondary, and ambient organic aerosols with high-resolution time-of-flight aerosol mass spectrometry Environ. Sci. Technol. 2008, 42, 4478-4485
8. Ng, N. L.; Canagaratna, M. R.; Zhang, Q.; Jimenez, J. L.; Tian, J.; Ulbrich, I. M.; Kroll, J. H.; Docherty, K. S.; Chhabra, P. S.; Bahreini, R.; Murphy, S. M.; Seinfeld, J. H.; Hildebrandt, L.; Donahue, N. M.; DeCarlo, P. F.; Lanz, V. A.; Prevot, A. S. H.; Dinar, E.; Rudich, Y.; Worsnop, D. R. Organic aerosol components observed in Northern Hemispheric datasets from Aerosol Mass Spectrometry Atmos. Chem. Phys. 2010, 10, 4625-4641
9. Lee, A. K. Y.; Herckes, P.; Leaitch, W. R.; Macdonald, A. M.; Abbatt, J. P. D. Aqueous OH oxidation of ambient organic aerosol and cloud water organics: Formation of highly oxidized products Geophys. Res. Lett. 2011, 38, L11805
10. Lee, A. K. Y.; Zhao, R.; Gao, S. S.; Abbatt, J. P. D. Aqueous-phase OH oxidation of glyoxal: application of a novel analytical approach employing aerosol mass spectrometry and complementary off-line techniques RID E-7380-2011 J. Phys. Chem. A 2011, 115, 10517-10526
11. Waxman, E. M.; Dzepina, K.; Ervens, B.; Lee-Taylor, J.; Aumont, B.; Jimenez, J. L.; Madronich, S.; Volkamer, R. Secondary organic aerosol formation from semi-and intermediate-volatility organic compounds and glyoxal: Relevance of O/C as a tracer for aqueous multiphase chemistry Geophys. Res. Lett. 2013, 40, 978-982
12. Loeffler, K. W.; Koehler, C. A.; Paul, N. M.; De Haan, D. O. Oligomer formation in evaporating aqueous glyoxal and methyl glyoxal solutions Environ. Sci. Technol. 2006, 40, 6318-6323
13. De Haan, D. O.; Corrigan, A. L.; Tolbert, M. A.; Jimenez, J. L.; Wood, S. E.; Turley, J. J. Secondary organic aerosol formation by self-reactions of methylglyoxal and glyoxal in evaporating droplets Environ. Sci. Technol. 2009, 43, 8184-8190
14. Schwier, A. N.; Sareen, N.; Mitroo, D.; Shapiro, E. L.; McNeill, V. F. Glyoxal-methylglyoxal cross-reactions in secondary organic aerosol formation Environ. Sci. Technol. 2010, 44, 6174-6182
15. Peng, C.; Chan, M.; Chan, C. The hygroscopic properties of dicarboxylic and multifunctional acids: Measurements and UNIFAC predictions Environ. Sci. Technol. 2001, 35, 4495-4501
16. Choi, M.; Chan, C. The effects of organic species on the hygroscopic behaviors of inorganic aerosols Environ. Sci. Technol. 2002, 36, 2422-2428
17. Galloway, M. M.; Chhabra, P. S.; Chan, A. W. H.; Surratt, J. D.; Flagan, R. C.; Seinfeld, J. H.; Keutsch, F. N. Glyoxal uptake on ammonium sulphate seed aerosol: reaction products and reversibility of uptake under dark and irradiated conditions Atmos. Chem. Phys. 2009, 9, 3331-3345
18. +) J. Phys. Chem. A 2009, 113, 231-237
19. Shapiro, E. L.; Szprengiel, J.; Sareen, N.; Jen, C. N.; Giordano, M. R.; McNeill, V. F. Light-absorbing secondary organic material formed by glyoxal in aqueous aerosol mimics Atmos. Chem. Phys. 2009, 9, 2289-2300
20. Yu, G.; Bayer, A. R.; Galloway, M. M.; Korshavn, K. J.; Fry, C. G.; Keutsch, F. N. Glyoxal in aqueous ammonium sulfate solutions: products, kinetics and hydration effects Environ. Sci. Technol. 2011, 45, 6336-6342
21. Kampf, C. J.; Jakob, R.; Hoffmann, T. Identification and characterization of aging products in the glyoxal/ammonium sulfate system-implications for light-absorbing material in atmospheric aerosols Atmos. Chem. Phys. 2012, 12, 6323-6333
22. Trainic, M.; Riziq, A. A.; Lavi, A.; Rudich, Y. Role of interfacial water in the heterogeneous uptake of glyoxal by mixed glycine and ammonium sulfate aerosols J. Phys. Chem. A 2012, 116, 5948-5957
23. Woo, J. L.; Kim, D. D.; Schwier, A. N.; Li, R.; McNeil, V. F. Aqueous aerosol SOA formation: Impact on aerosol physical properties Faraday Discuss. 2013, 10.1039/C3FD00032J
24. Nguyen, T. B.; Lee, P. B.; Updyke, K. M.; Bones, D. L.; Laskin, J.; Laskin, A.; Nizkorodov, S. A. Formation of nitrogen-and sulfur-containing light-absorbing compounds accelerated by evaporation of water from secondary organic aerosols J. Geophys. Res.-Atmos. 2012, 117, D01207
25. De Haan, D. O.; Hawkins, L. N.; Kononenko, J. A.; Turley, J. J.; Corrigan, A. L.; Tolbert, M. A.; Jimenez, J. L. Formation of nitrogen-containing oligomers by methylglyoxal and amines in simulated evaporating cloud droplets Environ. Sci. Technol. 2011, 45, 984-991
26. Canagaratna, M. R.; Jayne, J. T.; Jimenez, J. L.; Allan, J. D.; Alfarra, M. R.; Zhang, Q.; Onasch, T. B.; Drewnick, F.; Coe, H.; Middlebrook, A.; Delia, A.; Williams, L. R.; Trimborn, A. M.; Northway, M. J.; DeCarlo, P. F.; Kolb, C. E.; Davidovits, P.; Worsnop, D. R. Chemical and microphysical characterization of ambient aerosols with the aerodyne aerosol mass spectrometer Mass Spectrom. Rev. 2007, 26, 185-222
27. Allan, J.; Delia, A.; Coe, H.; Bower, K.; Alfarra, M.; Jimenez, J.; Middlebrook, A.; Drewnick, F.; Onasch, T.; Canagaratna, M.; Jayne, J.; Worsnop, D. A generalised method for the extraction of chemically resolved mass spectra from aerodyne aerosol mass spectrometer data J. Aerosol Sci. 2004, 35, 909-922
28. Wang, Z. Comprehensive Organic Name Reactions and Reagents; John Wiley & Sons: U.K., 2009.
29. 2O at 298.15 K J. Phys. Chem. A 1998, 102, 2155-2171
30. Andreae, M. O.; Gelencser, A. Black carbon or brown carbon? The nature of light-absorbing carbonaceous aerosols Atmos. Chem. Phys. 2006, 6, 3131-3148
31. Hoffer, A.; Gelencser, A.; Guyon, P.; Kiss, G.; Schmid, O.; Frank, G. P.; Artaxo, P.; Andreae, M. O. Optical properties of humic-like substances (HULIS) in biomass-burning aerosols Atmos. Chem. Phys. 2006, 6, 3563-3570
32. Lukacs, H.; Gelencser, A.; Hammer, S.; Puxbaum, H.; Pio, C.; Legrand, M.; Kasper-Giebl, A.; Handler, M.; Limbeck, A.; Simpson, D.; Preunkert, S. Seasonal trends and possible sources of brown carbon based on 2-year aerosol measurements at six sites in Europe J. Geophys. Res.-Atmos. 2007, 112, D23S18
33. Hecobian, A.; Zhang, X.; Zheng, M.; Frank, N.; Edgerton, E. S.; Weber, R. J. Water-Soluble Organic Aerosol material and the light-absorption characteristics of aqueous extracts measured over the Southeastern United States Atmos. Chem. Phys. 2010, 10, 5965-5977
34. Jaoui, M.; Edney, E. O.; Kleindienst, T. E.; Lewandowski, M.; Offenberg, J. H.; Surratt, J. D.; Seinfeld, J. H. Formation of secondary organic aerosol from irradiated alpha-pinene/toluene/NOx mixtures and the effect of isoprene and sulfur dioxide J. Geophys. Res.-Atmos. 2008, 113, D09303
35. Bones, D. L.; Henricksen, D. K.; Mang, S. A.; Gonsior, M.; Bateman, A. P.; Nguyen, T. B.; Cooper, W. J.; Nizkorodov, S. A. Appearance of strong absorbers and fluorophores in limonene-O-3 secondary organic aerosol due to NH4+-mediated chemical aging over long time scales J. Geophys. Res.-Atmos. 2010, 115, D05203
36. Limbeck, A.; Kulmala, M.; Puxbaum, H. Secondary organic aerosol formation in the atmosphere via heterogeneous reaction of gaseous isoprene on acidic particles Geophys. Res. Lett. 2003, 30, 1996
37. De Haan, D. O.; Corrigan, A. L.; Smith, K. W.; Stroik, D. R.; Turley, J. J.; Lee, F. E.; Tolbert, M. A.; Jimenez, J. L.; Cordova, K. E.; Ferrell, G. R. Secondary organic aerosol-forming reactions of glyoxal with amino acids Environ. Sci. Technol. 2009, 43, 2818-2824
38. Sareen, N.; Schwier, A. N.; Shapiro, E. L.; Mitroo, D.; McNeill, V. F. Secondary organic material formed by methylglyoxal in aqueous aerosol mimics Atmos. Chem. Phys. 2010, 10, 997-1016
39. Zhang, X.; Lin, Y.; Surratt, J. D.; Zotter, P.; Prevot, A. S. H.; Weber, R. J. Light-absorbing soluble organic aerosol in Los Angeles and Atlanta: A contrast in secondary organic aerosol Geophys. Res. Lett. 2011, 38, L21810