Identification and characterization of aging products in the glyoxal/ammonium sulfate system – Implications for light-absorbing material in atmospheric aerosols

Atmospheric Chemistry and Physics

Volumn 12, Issue 14, 2012, Pages 6323-6333

  Kampf, C J ^a   Jakob, R ^a   Hoffmann, T ^a  

^a JOHANNES GUTENBERG UNIVERSITY   (Germany)

Author keywords

[No Author keywords available]

Indexed keywords

ABSORPTION COEFFICIENT; AEROSOL PROPERTY; AGING; AMMONIUM SULFATE; IDENTIFICATION METHOD;

EID: 84864228355     PISSN: 16807316     EISSN: 16807324     Source Type: Journal    
DOI: 10.5194/acp-12-6323-2012     Document Type: Article

References (44)

1. Altieri, K. E., Seitzinger, S. P., Carlton, A. G., Turpin, B. J., Klein, G. C., and Marshall, A. G.: Oligomers formed through in-cloud methylglyoxal reactions: Chemical composition, properties, and mechanisms investigated by ultra-high resolution FT-ICR mass spectrometry, Atmos. Environ., 42, 1476-1490, 2008.
2. Bones, D. L., Henricksen, D. K., Mang, S. A., Gonsior, M., Bateman, A. P., Nguyen, T. B., Cooper, W. J., and Nizkorodov, S. A.: Appearance of strong absorbers and fluorophores in limonene-O3 secondary organic aerosol due to NH4+-mediated chemical aging over long time scales, J. Geophys. Res., 115, D05023, doi:10.1029/2009JD012864, 2010.
3. Carlton, A. G., Turpin, B. J., Altieri, K. E., Seitzinger, S., Reff, A., Lim, H. J., and Ervens, B.: Atmospheric oxalic acid and SOA production from glyoxal: Results of aqueous photooxidation experiments, Atmos. Environ., 41, 7588-7602, 2007. (Pubitemid 350064570)
4. Chiswell, B., Lions, F., and Morris, B. S.: Bidentate chelate compounds. III. Metal complexes of some pyridyl-imidazole derivatives, Inorg. Chem., 3, 110-114, 1964.
5. Cho, J. R., Cho, S. G., Goh, E. M., and Kim, J. K: Preparation method of 2,2'-bi-1H-imidazole using glyoxal and an ammonium salt, United States Patent, 6713631, 2003.
6. Clarisse, L., Clerbaux, C., Dentener, F., Hurtmans, D., and Coheur, F.: Global ammonia distribution derived from infrared satellite observations, Nat. Geosci., 2, 479-483, doi:10.1038/ngeo551, 2009.
7. Debus, H.: Uber die Einwirkung des Ammoniaks auf Glyoxal, Liebigs Ann. Chem., 107, 199-208, 1858.
8. De Haan, D. O., Corrigan, A. L., Smith, K.W., Stroik, D. R., Turley, J. J., Lee, F. E., Tolbert, M. A., Jimenez, J. L., Cordova, K. E., and Ferrell, G. R.: Secondary organic aerosol-forming reactions of glyoxal with amino acids, Environ. Sci. Technol., 43, 2818-2824, 2009a.
9. De Haan, D. O., Tolbert, M. A., and Jimenez, J. L.: Atmospheric condensed-phase reactions of glyoxal with methylamine, Geophys. Res. Lett., 36, L11819, doi:10.1029/2009GL037441, 2009b.
10. De Haan, D. O., Hawkins, L. N., Kononenko, J. A., Turley, J. J., Corrigan, A. L., Tolbert, M. A., and Jimenez, J. L.: Formation of Nitrogen-Containing Oligomers by Methylglyoxal and Amines in Simulated Evaporating Cloud Droplets, Environ. Sci. Technol., 45, 984-991, 2011.
11. Ervens, B., Turpin, B. J., and Weber, R. J.: Secondary organic aerosol formation in cloud droplets and aqueous particles (aqSOA): a review of laboratory, field and model studies, Atmos. Chem. Phys., 11, 11069-11102, doi:10.5194/acp-11-11069-2011, 2011.
12. Fieselmann, B. F., Hendrickson, D. N., and Stucky, G. D: Synthesis, electron paramagnetic resonance, and magnetic studies of binuclear bis(-5-cyclopentadienyl)titanium(III) compounds with bridging pyrazolate, biimidazolate, and bibenzimidazolate anions, Inorg. Chem., 17, 2078-2084, 1978.
13. Galloway, M. M., Chhabra, P. S., Chan, A. W. H., Surratt, J. D., Flagan, R. C., Seinfeld, J. H., and Keutsch, F. N.: Glyoxal uptake on ammonium sulphate seed aerosol: reaction products and reversibility of uptake under dark and irradiated conditions, Atmos. Chem. Phys., 9, 3331-3345, doi:10.5194/acp-9-3331- 2009, 2009.
14. Hastings, W. P., Koehler, C. A., Bailey, E. L., and De Haan, D. O.: Secondary organic aerosol formation by glyoxal hydration and oligomer formation: Humidity effects and equilibrium shifts during analysis, Environ. Sci. Technol., 39, 22, 8728-8735, 2005. (Pubitemid 41636140)
15. Holmes, F., Jones, K. M., and Torrible, E. G.: Complex-forming agents similar to 2,2'-bipyridyl. Part I. Some Ligands containing imidazole, J. Chem. Soc., 4790-4794, 1961.
16. Hallquist, M., Wenger, J. C., Baltensperger, U., Rudich, Y., Simpson, D., Claeys, M., Dommen, J., Donahue, N. M., George, C., Goldstein, A. H., Hamilton, J. F., Herrmann, H., Hoffmann, T., Iinuma, Y., Jang, M., Jenkin, M. E., Jimenez, J. L., Kiendler-Scharr, A., Maenhaut, W., McFiggans, G., Mentel, T. F., Monod, A., Prevot, A. S. H., Seinfeld, J. H., Surratt, J. D., Szmigielski, R., andWildt, J.: The formation, properties and impact of secondary organic aerosol: current and emerging issues, Atmos. Chem. Phys., 9, 5155-5236, doi:10.5194/acp-9-5155-2009, 2009.
17. Jimenez, J. L., Canagaratna, M. R., Donahue, N. M., Prevot, A. S. H., Zhang, Q., Kroll, J. H., DeCarlo, P. F., Allan, J. D., Coe, H., Ng, N. L., Aiken, A. C., Docherty, K. S., Ulbrich, I. M., Grieshop, A. P., Robinson, A. L., Duplissy, J., Smith, J. D., Wilson, K. R., Lanz, V. A., Hueglin, C., Sun, Y. L., Tian, J., Laaksonen, A., Raatikainen, T., Rautiainen, J., Vaattovaara, P., Ehn, M., Kulmala, M., Tomlinson, J. M., Collins, D. R., Cubison, M. J., Dunlea, E. J., Huffman, J. A., Onasch, T. B., Alfarra, M. R., Williams, P. I., Bower, K., Kondo, Y., Schneider, J., Drewnick, F., Borrmann, S., Weimer, S., Demerjian, K., Salcedo, D., Cottrell, L., Griffin, R., Takami, A., Miyoshi, T., Hatakeyama, S., Shimono, A., Sun, J. Y., Zhang, Y. M., Dzepina, K., Kimmel, J. R., Sueper, D., Jayne, J. T., Herndon, S. C., Trimborn, A. M., Williams, L. R., Wood, E. C., Middlebrook, A. M., Kolb, C. E., Baltensperger, U., and Worsnop, D. R.: Evolution of Organic Aerosols in the Atmosphere, Science, 326, 1525-1529, 2009.
18. Kalberer, M., Paulsen, D., Sax, M., Steinbacher, M., Dommen, J., Prevot, A. S. H., Fisseha, R., Weingartner, E., Frankevich, V., Zenobi, R., and Baltensperger, U.: Identification of polymers as major components of atmospheric organic aerosols, Science, 303, 1659-1662, 2004. (Pubitemid 38338322)
19. Kua, J., Krizner H. E., and De Haan, D. O.: Thermodynamics and Kinetics of Imidazole Formation from Glyoxal, Methylamine, and Formaldehyde: A Computational Study, J. Phys. Chem. A, 115, 1667-1675, 2011.
20. Kulshrestha, U. C., Saxena, A., Kumar, N., Kumari, K. M., and Srivastava, S. S.: Chemical composition and association of sizedifferentiated aerosols at a suburban site in a semi-arid tract of India, J. Atmos. Chem., 29, 109-118, 1998. (Pubitemid 28142903)
21. Liggio, J., Li, S. M., and McLaren, R.: Heterogeneous reactions of glyoxal on particulate matter: Identification of acetals and sulfate esters, Environ. Sci. Technol., 39, 1532-1541, 2005a. (Pubitemid 40387706)
22. Liggio, J., Li, S. M., and McLaren, R.: Reactive uptake of glyoxal by particulate matter, J. Geophys. Res. Atmos., 110, D10304, doi:10.1029/ 2004JD005113, 2005 (Pubitemid 40919776)
23. Lim, Y. B., Tan, Y., Perri, M. J., Seitzinger, S. P., and Turpin, B. J.: Aqueous chemistry and its role in secondary organic aerosol (SOA) formation, Atmos. Chem. Phys., 10 10521-10539, doi:10.5194/acp-10-10521-2010, 2010.
24. Loeffler, K. W., Koehler, C. A., Paul, N. M., and De Haan, D. O.: Oligomer formation in evaporating aqueous glyoxal and methyl glyoxal solutions, Environ. Sci. Technol., 40, 6318-6323, 2006. (Pubitemid 44630895)
25. Mao, F., Mano, N., and Heller, A.: Long tethers binding redox centers to polymer backbones enhance electron transport in enzyme "wiring" hydrogels, J. Am. Chem. Soc., 125, 4951-4957, 2003. (Pubitemid 36505388)
26. Noziere, B., Dziedzic, P., and Cordova, A.: Products and kinetics of the liquid-phase reaction of glyoxal catalyzed by ammonium ions (NH4+), J. Phys. Chem. A, 113, 231-237, 2009.
27. Odum, J. R., Hoffmann, T., Bowman, F., Collins, D., Flagan, R. C., and Seinfeld, J. H.: Gas/particle partitioning and secondary organic aerosol yields, Environ. Sci. Technol., 30, 2580-2585, 1996.
28. Pankow, J. F.: An absorption model of the gas/aerosol partitioning involved in the formation of secondary organic aerosol, Atmos. Environ., 28, 189-193, 1994.
29. Parashar, D. C., Kulshrestha, U. C., and Jain, M.: Precipitation and aerosol studies in India, Environ. Monit. Assess., 66, 47-61, 2001. (Pubitemid 32093934)
30. Sareen, N., Schwier, A. N., Shapiro, E. L., Mitroo, D., and Mc-Neill, V. F.: Secondary organic material formed by methylglyoxal in aqueous aerosol mimics, Atmos. Chem. Phys., 10, 997-1016, doi:10.5194/acp-10-997-2010, 2010.
31. Schwier, A. N., Sareen, N., Mitroo, D., Shapiro, E. L., and McNeill, V. F.: Glyoxal-Methylglyoxal Cross-Reactions in Secondary Organic Aerosol Formation, Environ. Sci. Technol., 44, 6174-6182, 2010.
32. See, S. W., Wang, Y. H., and Balasubramanian, R.: Contrasting reactive oxygen species and transition metal concentrations in combustion aerosols, Environ. Res., 103, 317-324, 2007. (Pubitemid 46217203)
33. Seinfeld, J. H. and Pandis, S. N.: Atmospheric chemistry and physics: From air pollution to climate change, 2nd Edn., Wiley, Hoboken, 2006.
34. Shapiro, E. L., Szprengiel, J., Sareen, N., Jen, C. N., Giordano, M. R., and McNeill, V. F.: Light-absorbing secondary organic material formed by glyoxal in aqueous aerosol mimics, Atmos. Chem. Phys., 9, 2289-2300, doi:10.5194/acp-9-2289-2009, 2009.
35. Surratt, J. D., Kroll, J. H., Kleindienst, T., E., Edney, E. O., Claeys, M., Sorooshian, A., Ng, N. L., Offenberg, J. H., Lewandowski, M., Jaoui, M., Flagan, R., and Seinfeld, J. H.: Evidence for organosulfates in secondary organic aerosol, Environ. Sci. Technol., 41, 517-527, doi:10.1021/es062081q, 2007. (Pubitemid 46106285)
36. Surratt, J. D., Gomez-Gonzalez, Y., Chan, A.W. H., Vermeylen, R., Shahgholi, M., Kleindienst, T. E., Edney, E. O., Offenberg, J. H., Lewandowski, M., Jaoui, M., Maenhaut, W., Claeys, M., Flagan, R. C., and Seinfeld, J. H.: Organosulfate formation in biogenic secondary organic aerosol, J. Phys. Chem. A, 112, 8345-8378, doi:10.1021/jp802310p, 2008.
37. Tan, Y., Perri, M. J., Seitzinger S. P., and Turpin, B. J.: Effects of precursor concentration and acidic sulfate in aqueous glyoxal-OH radical oxidation and implications for secondary organic aerosol, Environ. Sci. Technol., 43, 8105-8112, doi:10.1021/es901742f, 2009.
38. Tan, Y., Carlton, A. G., Seitzinger, S. P., and Turpin, B. J.: SOA from methylglyoxal in clouds and wet aerosols: Measurement and prediction of key products, Atmos. Environ., 44, 5218-5226, 2010.
39. Trainic, M., Riziq, A. A., Lavi, A., Flores, J. M., and Rudich, Y.: The optical, physical and chemical properties of the products of glyoxal uptake on ammonium sulfate seed aerosols, Atmos. Chem. Phys., 11, 9697-9707, doi:10.5194/acp-11-9697-2011, 2011.
40. Trainic, M., Riziq, A. A., Lavi, A., and Rudich, Y.: The role of interfacial water in the heterogeneous uptake of glyoxal by mixed glycine and ammonium sulfate aerosols, J. Phys. Chem. A., 116, 5948-5957, doi:10.1021/jp2104837, 2012.
41. Yasmeen, F., Sauret, N., Gal, J. -F, Maria, P.-C, Massi, L., Maenhaut, W., and Claeys, M.: Characterization of oligomers from methylglyoxal under dark conditions: a pathway to produce secondary organic aerosol through cloud processing during nighttime, Atmos. Chem. Phys., 10, 3803-3812, doi:10.5194/acp-10-3803-2010, 2010.
42. Yu, G., Bayer A. R., Galloway, M. M., Korshavn, K. J., Fry, C. G., and Keutsch, F. N.: Glyoxal in Aqueous Ammonium Sulfate Solutions: Products, Kinetics and Hydration Effects, Environ. Sci. Technol., 45, 6336-6342, 2011.
43. Zhao, J., Levitt, N. P., Zhang, R. Y., and Chen, J. M.: Heterogeneous reactions of methylglyoxal in acidic media: Implications for secondary organic aerosol formation, Environ. Sci. Technol., 40, 7682-7687, 2006. (Pubitemid 46012562)
44. Zhang, Q., Jimenez, J. L., Canagaratna, M. R., Allan, J. D., Coe, H., Ulbrich, I., Alfarra, M. R., Takami, A., Middlebrook, A. M., Sun, Y. L., Dzepina, K., Dunlea, E., Docherty, K., DeCarlo, P. F., Salcedo, D., Onasch, T., Jayne, J. T., Miyoshi, T., Shimono, A., Hatakeyama, S., Takegawa, N., Kondo, Y., Schneider, J., Drewnick, F., Borrmann, S., Weimer, S., Demerjian, K., Williams, P., Bower, K., Bahreini, R., Cottrell, L., Griffin, R. J., Rautiainen, J., Sun, J. Y., Zhang, Y. M., and Worsnop, D. R.: Ubiquity and dominance of oxygenated speciesin organic aerosols in anthropogenically-influenced Northern Hemisphere midlatitudes, Geophys. Res. Lett., 34, L13801, doi:10.1029/2007GL029979, 2007. (Pubitemid 47399659)