Laboratory study on the hygroscopic behavior of external and internal C2-C4 dicarboxylic acid-NaCl mixtures

Environmental Science and Technology

Volumn 47, Issue 18, 2013, Pages 10381-10388

  Ma, Qingxin ^a   Ma, Jinzhu ^a   Liu, Chang ^b   Lai, Chengyue ^a   He, Hong ^a  

^a RESEARCH CENTER FOR ECO ENVIRONMENTAL SCIENCES   (China)

^b STATE KEY LABORATORY OF SEVERE WEATHER   (China)

Author keywords

[No Author keywords available]

Indexed keywords

CHEMICAL COMPOSITIONS; CONVERSION PROCESS; DICARBOXYLATE SALTS; HYGROSCOPIC BEHAVIOR; LABORATORY STUDIES; NONLINEAR RELATIONS; ORGANIC COMPONENTS; TOTAL WATER CONTENT;

ATMOSPHERIC AEROSOLS; CARBOXYLATION; HUMIDITY CONTROL; ORGANIC ACIDS; OXALIC ACID;

MIXTURES;

MALONIC ACID; OXALIC ACID; SODIUM CHLORIDE; SUCCINIC ACID; WATER;

AEROSOL; CHEMICAL COMPOSITION; HYGROSCOPICITY; LABORATORY METHOD; OXALIC ACID; RELATIVE HUMIDITY; SODIUM CHLORIDE; WATER CONTENT;

ADSORPTION; AEROSOL; ANALYTIC METHOD; ARTICLE; ATMOSPHERE; CHEMICAL COMPOSITION; DISSOLUTION; HUMIDITY; HYDRATION; ISOTHERM; LABORATORY; WATER CONTENT; WETTABILITY;

ADSORPTION; DICARBOXYLIC ACIDS; HUMIDITY; SODIUM CHLORIDE; WATER; WETTABILITY;

EID: 84884217537     PISSN: 0013936X     EISSN: 15205851     Source Type: Journal    
DOI: 10.1021/es4023267     Document Type: Article

References (65)

1. Orr, C., Jr.; Kurd, F.; Corbett, W. Aerosol size and relative humidity J. Colloid Sci. 1965, 13, 472-482
2. Charlson, R. J.; Schwartz, S. E.; Hales, J. M.; Cess, R. D.; Coakley, J. A.; Hansen, J. E.; Hofmann, D. J. Climate forcing by anthropogenic aerosols Science 1992, 255 (5043) 423-430
3. Pilinis, C.; Pandis, S. N.; Seinfeld, J. H. Sensitivity of direct climate forcing by atmospheric aerosols to aerosol size and composition J. Geophys. Res. 1995, 100 (D9) 18,739-18,754
4. Lewis, R.; Schwartz, E. Sea Salt Aerosol Production: Mechanisms, Methods, Measurements and Models-A Critical Review. American Geophysical Union: 2004; Vol. 152.
5. Rossi, M. J. Heterogeneous reactions on salts Chem. Rev. 2003, 103 (12) 4823-4882
6. Finlayson-Pitts, B. The tropospheric chemistry of sea salt: A molecular-level view of the chemistry of NaCl and NaBr Chem. Rev. 2003, 103 (12) 4801-4822
7. Dai, Q.; Hu, J.; Salmeron, M. Adsorption of water on NaCl (100) surfaces: Role of atomic steps J. Phys. Chem. B 1997, 101 (11) 1994-1998 (Pubitemid 127609236)
8. Xu, L.; Bluhm, H.; Salmeron, M. An AFM study of the tribological properties of NaCl (100) surfaces under moist air Surf. Sci. 1998, 407 (1) 251-255 (Pubitemid 128399987)
9. 3 aerosols to changes in relative humidity from 298 to 238 K J. Phys. Chem. A 2000, 104 (10) 2038-2047
10. Foster, M.; Ewing, G. Adsorption of water on the NaCl (001) surface. II. An infrared study at ambient temperatures J. Chem. Phys. 2000, 112, 6817-6826 (Pubitemid 33638901)
11. Hameri, K.; Laaksonen, A.; Vakeva, M.; Suni, T. Hygroscopic growth of ultrafine sodium chloride particles J. Geophys. Res. 2001, 106 (D18) 20,749-20,757
12. Joutsensaari, J.; Vaattovaara, P.; Vesterinen, M.; H meri, K.; Laaksonen, A. A novel tandem differential mobility analyzer with organic vapor treatment of aerosol particles Atmos. Chem. Phys. 2001, 1 (1) 51-60
13. Ebert, M.; Inerle-Hof, M.; Weinbruch, S. Environmental scanning electron microscopy as a new technique to determine the hygroscopic behaviour of individual aerosol particles Atmos. Environ. 2002, 36 (39-40) 5909-5916 (Pubitemid 35428835)
14. Krueger, B. J.; Grassian, V. H.; Iedema, M. J.; Cowin, J. P.; Laskin, A. Probing heterogeneous chemistry of individual atmospheric particles using scanning electron microscopy and energy-dispersive X-ray analysis Anal. Chem. 2003, 75 (19) 5170-5179 (Pubitemid 37238570)
15. Schuttlefield, J.; Al-Hosney, H.; Zachariah, A.; Grassian, V. H. Attenuated total reflection fourier transform infrared spectroscopy to investigate water uptake and phase transitions in atmospherically relevant particles Appl. Spectrosc. 2007, 61 (3) 283-292 (Pubitemid 46493870)
16. Ma, Q.; He, H.; Liu, Y. In situ DRIFTS study of hygroscopic behavior of mineral aerosol J. Environ. Sci. 2010, 22 (4) 555-560
17. Ma, Q.; Liu, Y.; He, H. The utilization of physisorption analyzer for studying the hygroscopic properties of atmospheric relevant particles J. Phys. Chem. A 2010, 114, 4232-4237
18. Cohen, M.; Flagan, R.; Seinfeld, J. Studies of concentrated electrolyte solutions using the electrodynamic balance. 1. Water activities for single-electrolyte solutions J. Phys. Chem. 1987, 91 (17) 4563-4574
19. Kerminen, V.-M.; Teinilä, K.; Hillamo, R.; Pakkanen, T. Substitution of chloride in sea-salt particles by inorganic and organic anions J. Aerosol Sci. 1998, 29 (8) 929-942 (Pubitemid 28370507)
20. Yao, X.; Fang, M.; Chan, C. K. Size distributions and formation of dicarboxylic acids in atmospheric particles Atmos. Environ. 2002, 36 (13) 2099-2107 (Pubitemid 34626275)
21. Johansen, A. M.; Siefert, R. L.; Hoffmann, M. R. Chemical characterization of ambient aerosol collected during the southwest monsoon and intermonsoon seasons over the Arabian Sea: Anions and cations J. Geophys. Res. 1999, 104 (26) 325-326
22. Tervahattu, H.; Hartonen, K.; Kerminen, V.-M.; Kupiainen, K.; Aarnio, P.; Koskentalo, T.; Tuck, A. F.; Vaida, V. New evidence of an organic layer on marine aerosols J. Geophys. Res. 2002, 107 (D7) 4053
23. Laskin, A.; Iedema, M. J.; Cowin, J. P. Quantitative time-resolved monitoring of nitrate formation in sea salt particles using a CCSEM/EDX single particle analysis Environ. Sci. Technol. 2002, 36 (23) 4948-4955 (Pubitemid 35424828)
24. Yao, X.; Fang, M.; Chan, C. K. Experimental study of the sampling artifact of chloride depletion from collected sea salt aerosols Environ. Sci. Technol. 2001, 35 (3) 600-605 (Pubitemid 32125971)
25. Laskin, A.; Moffet, R. C.; Gilles, M. K.; Fast, J. D.; Zaveri, R. A.; Wang, B.; Nigge, P.; Shutthanandan, J. Tropospheric chemistry of internally mixed sea salt and organic particles: Surprising reactivity of NaCl with weak organic acids J. Geophys. Res. 2012, 117, D15302
26. Chan, C. K.; Ha, Z.; Choi, M. Y. Study of water activities of aerosols of mixtures of sodium and magnesium salts Atmos. Environ. 2000, 34 (28) 4795-4803
27. Kanakidou, M.; Seinfeld, J.; Pandis, S.; Barnes, I.; Dentener, F.; Facchini, M.; Van Dingenen, R.; Ervens, B.; Nenes, A.; Nielsen, C. Organic aerosol and global climate modelling: A review Atmos. Chem. Phys. 2005, 5 (4) 1053-1123 (Pubitemid 40560480)
28. Kawamura, K.; Ikushima, K. Seasonal changes in the distribution of dicarboxylic acids in the urban atmosphere Environ. Sci. Technol. 1993, 27 (10) 2227-2235 (Pubitemid 24396537)
29. Chebbi, A.; Carlier, P. Carboxylic acids in the troposphere, occurrence, sources, and sinks: A review Atmos. Environ. 1996, 30 (24) 4233-4249
30. Mochida, M.; Kawabata, A.; Kawamura, K.; Hatsushika, H.; Yamazaki, K. Seasonal variation and origins of dicarboxylic acids in the marine atmosphere over the western North Pacific J. Geophys. Res. 2003, 108 (D6) 4193
31. Sullivan, R. C.; Prather, K. A. Investigations of the diurnal cycle and mixing state of oxalic acid in individual particles in Asian aerosol outflow Environ. Sci. Technol. 2007, 41 (23) 8062-8069 (Pubitemid 350224413)
32. Wang, G.; Xie, M.; Hu, S.; Gao, S.; Tachibana, E.; Kawamura, K. Dicarboxylic acids, metals and isotopic compositions of C and N in atmospheric aerosols from inland China: Implications for dust and coal burning emission and secondary aerosol formation Atmos. Chem. Phys. 2010, 10, 6087-6096
33. Rohrl, A.; Lammel, G. Low-molecular weight dicarboxylic acids and glyoxylic acid: Seasonal and air mass characteristics Environ. Sci. Technol. 2001, 35 (1) 95-101 (Pubitemid 32048410)
34. Yang, L.; Yu, L. E. Measurements of oxalic acid, oxalates, malonic acid, and malonates in atmospheric particulates Environ. sci. Technol. 2008, 42 (24) 9268-9275
35. Wang, G.; Kawamura, K.; Cheng, C.; Li, J.; Cao, J.; Zhang, R.; Zhang, T.; Liu, S.; Zhao, Z. Molecular distribution and stable carbon isotopic composition of dicarboxylic acids, ketocarboxylic acids, and α-dicarbonyls in size-resolved atmospheric particles from Xi'an City, China Environ. Sci. Technol. 2012, 46 (9) 4783
36. Yu, J.; Huang, X.; Xu, J.; Hu, M. When aerosol sulfate goes up, so does oxalate: Implication for the formation mechanisms of oxalate Environ. Sci. Technol. 2005, 39 (1) 128-133 (Pubitemid 40066284)
37. Sorooshian, A.; Lu, M. L.; Brechtel, F. J.; Jonsson, H.; Feingold, G.; Flagan, R. C.; Seinfeld, J. H. On the source of organic acid aerosol layers above clouds Environ. Sci. Technol. 2007, 41 (13) 4647-4654 (Pubitemid 47047402)
38. Facchini, M.; Mircea, M.; Fuzzi, S.; Charlson, R. Cloud albedo enhancement by surface-active organic solutes in growing droplets Nature 1999, 401 (6750) 257-259
39. Yu, S. Role of organic acids (formic, acetic, pyruvic and oxalic) in the formation of cloud condensation nuclei (CCN): A review Atmos. Res. 2000, 53 (4) 185-217 (Pubitemid 30306274)
40. Yang, F.; Chen, H.; Wang, X.; Yang, X.; Du, J.; Chen, J. Single particle mass spectrometry of oxalic acid in ambient aerosols in Shanghai: Mixing state and formation mechanism Atmos. Environ. 2009, 43 (25) 3876-3882
41. Peng, C.; Chan, M.; Chan, C. The hygroscopic properties of dicarboxylic and multifunctional acids: Measurements and UNIFAC predictions Environ. Sci. Technol. 2001, 35 (22) 4495-4501 (Pubitemid 33070060)
42. Prenni, A.; DeMott, P.; Kreidenweis, S.; Sherman, D.; Russell, L.; Ming, Y. The effects of low molecular weight dicarboxylic acids on cloud formation J. Phys. Chem. A 2001, 105 (50) 11240-11248 (Pubitemid 35378566)
43. Braban, C.; Carroll, M.; Styler, S.; Abbatt, J. Phase transitions of malonic and oxalic acid aerosols J. Phys. Chem. A 2003, 107 (34) 6594-6602
44. Wise, M. E.; Surratt, J. D.; Curtis, D. B.; Shilling, J. E.; Tolbert, M. A. Hygroscopic growth of ammonium sulfate/dicarboxylic acids J. Geophys. Res 2003, 108 (20) 4638
45. Cruz, C. N.; Pandis, S. N. Deliquescence and hygroscopic growth of mixed inorganic-organic atmospheric aerosol Environ. Sci. Technol. 2000, 34 (20) 4313-4319
46. Francis, D.; Pope, B. J. D.-S.; Paul, T.; Griffiths; Simon, L.; Clegg; Cox, R. Anthony Studies of single aerosol particles containing malonic acid, glutaric acid, and their mixtures with sodium chloride. I. Hygroscopic growth J. Phys. Chem. A 2010, 114, 5335-5341
47. 3 Phys. Chem. Chem. Phys. 2010, 12 (36) 10896-10903
48. Gysel, M.; Weingartner, E.; Baltensperger, U. Hygroscopicity of aerosol particles at low temperatures. 2. Theoretical and experimental hygroscopic properties of laboratory generated aerosols Environ. Sci. Technol. 2002, 36 (1) 63-68 (Pubitemid 34052874)
49. Wise, M.; Biskos, G.; Martin, S.; Russell, L.; Buseck, P. Phase transitions of single salt particles studied using a transmission electron microscope with an environmental cell Aerosol Sci. Technol. 2005, 39 (9) 849-856 (Pubitemid 41611562)
50. Ma, Q.; He, H.; Liu, C. Hygroscopic properties of oxalic acid and atmospherically relevant oxalates Atmos. Environ. 2013, 69, 281-288
51. Ma, Q.; He, H. Synergistic effect in the humidifying process of atmospheric relevant calcium nitrate, calcite and oxalic acid mixtures Atmos. Environ. 2012, 50, 97-102
52. Saxena, P.; Hildemann, L. Water absorption by organics: Survey of laboratory evidence and evaluation of UNIFAC for estimating water activity Environ. Sci. Technol. 1997, 31 (11) 3318-3324 (Pubitemid 27500299)
53. Brooks, S.; Wise, M.; Cushing, M.; Tolbert, M. Deliquescence behavior of organic/ammonium sulfate aerosol Geophys. Res. Lett. 2002, 29 (19) 1917
54. Stokes, R.; Robinson, R. Interactions in aqueous nonelectrolyte solutions. I. Solute-solvent equilibria J. Phys. Chem. 1966, 70 (7) 2126-2131
55. Seinfeld, J.; Pandis, S., Atmospheric Chemistry and Physics: From Air Pollution to Climate Change; John Wiley: New York, 1998.
56. Zdanovskii, A. New methods for calculating solubilities of electrolytes in multicomponent systems Zhur. Fiz. Kim 1948, 22, 1475-1485
57. Peng, C.; Chan, C. K. The water cycles of water-soluble organic salts of atmospheric importance Atmos. Environ. 2001, 35 (7) 1183-1192 (Pubitemid 32101381)
58. Wu, Z. J.; Nowak, A.; Poulain, L.; Herrmann, H.; Wiedensohler, A. Hygroscopic behavior of atmospherically relevant water-soluble carboxylic salts and their influence on the water uptake of ammonium sulfate Atmos. Chem. Phys. 2011, 11, 12617-12626
59. Ebisuzaki, Y.; Angel, S. M. Raman study of hydrogen bonding in α and β-oxalic acid dihydrate J. Raman Spectrosc. 1981, 11 (4) 306-311
60. Nieminen, J.; Rasanen, M.; Murto, J. Matrix isolation and ab initio studies of oxalic acid J. Phys. Chem. 1992, 96, 5303-5308
61. Mohaček-Grošev, V.; Grdadolnik, J.; Stare, J.; Hadži, D. Identification of hydrogen bond modes in polarized Raman spectra of single crystals of α-oxalic acid dihydrate J. Raman Spectrosc. 2009, 40 (11) 1605-1614
62. Frost, R. L. Raman spectroscopy of natural oxalates Anal. Chim. Acta 2004, 517, 207-214 (Pubitemid 38798326)
63. Haynes, W. M.; Lide, D. R. CRC Handbook of Chemistry and Physics; CRC Press: Boca Raton, FL, 2011
64. 3 and the effect on the hygroscopic behaviour of these particles Phys. Chem. Chem. Phys. 2012, 14, 8403-8409
65. Sullivan, R.; Moore, M.; Petters, M.; Kreidenweis, S.; Roberts, G.; Prather, K. Effect of chemical mixing state on the hygroscopicity and cloud nucleation properties of calcium mineral dust particles Atmos. Chem. Phys. 2009, 9, 3303-3316