Atmospheric test of the J(BrONO2)kBrO+NO2 ratio: Implications for total stratospheric Bry and bromine-mediated ozone loss

Atmospheric Chemistry and Physics

Volumn 13, Issue 13, 2013, Pages 6263-6274

  Kreycy, S ^a   Camy Peyret, C ^b   Chipperfield, M P ^c   Dorf, M ^a   Feng, W ^c   Hossaini, R ^c   Kritten, L ^d   Werner, B ^a   Pfeilsticker, K ^a  

^a UNIVERSITY OF HEIDELBERG   (Germany)

^b SORBONNE UNIVERSITÉ   (France)

^c UNIVERSITY OF LEEDS   (United Kingdom)

^d FREIE UNIVERSITÄT BERLIN   (Germany)

Author keywords

[No Author keywords available]

Indexed keywords

ATMOSPHERIC CHEMISTRY; AUTUMN; BROMINE; NITROGEN DIOXIDE; OZONE; OZONE DEPLETION; PHOTOCHEMISTRY; RADIATIVE TRANSFER; STRATOSPHERE;

SANDER;

EID: 84880624063     PISSN: 16807316     EISSN: 16807324     Source Type: Journal    
DOI: 10.5194/acp-13-6263-2013     Document Type: Article

References (30)

1. Aliwell, S., Van Roozendael, M., Johnston, P., Richter, A., Wagner, T., Arlander, D., Burrows, J., Fish, D., Jones, R., Tornkvist, K., Lambert, J.-C., Pfeisticker, K., and Pundt, I.: Analysis for BrO in zenith-sky spectra: an intercomparison exercise for analysis improvement, J. Geophys. Res., 107, 4199, doi:10.1029/2001JD000329, 2002. (Pubitemid 43197320)
2. Bösch, H., Camy-Peyret, C., Chipperfield, M. P., Fitzenberger, R., Harder, H., Schiller, C., Schneider, M., Trautmann, T., and Pfeilsticker, K.: Comparison of measured and modeled startospheric UV/visible actinic fluxes at large solar zenith angles, Geophys. Res. Lett., 28, 1179-1182, 2001. (Pubitemid 32579672)
3. Bösch, H., Camy-Peyret, C., Chipperfield, M. P., Fitzenberger, R., Harder, H., Platt, U., and Pfeilsticker, K.: Upper limits of stratospheric IO and OIO inferred from center-to-limb-darkening-corrected balloon-borne solar occultation visible spectra: implications for total gaseous iodine and stratospheric ozone, J. Geophys. Res., 108, 4455, doi:10.1029/2002JD003078, 2003.
4. Brinckmann, S., Engel, A., Bönisch, H., Quack, B., and Atlas, E.: Short-lived brominated hydrocarbons - observations in the source regions and the tropical tropopause layer, Atmos. Chem. Phys., 12, 1213-1228, doi:10.5194/acp-12-1213-2012, 2012.
5. 2 abundances retrieved from balloon borne direct sun observations and Envisat/SCIAMACHY limb measurements, Atmos. Chem. Phys., 6, 1293-1314, doi:10.5194/acp-6-1293-2006, 2006. (Pubitemid 44198605)
6. 2O profiles at high and mid-latitudes using the LPMA balloon borne Fourier Transform instrument, in: Air Pollution Research Report, Polar Stratospheric Ozone Symposium, Schliersee, 1995.
7. Chipperfield, M. P.: Multiannual simulations with a three-dimensional chemical transport model, J. Geophys. Res., 104, 1781-1805, 1999. (Pubitemid 29250695)
8. Chipperfield, M. P.: New version of the TOMCAT/SLIMCAT offline chemical transport model: intercomparison of stratospheric tracer experiments, Q. J. Roy. Meteorol. Soc., 132, 1179-1203, 2006. (Pubitemid 44097070)
9. Deutschmann, T., Beirle, S., Frieß, U., Grzegorski, M., Kern, C., Kritten, L., Platt, U., Puķīte, J., Wagner, T., Werner, B., and Pfeilsticker, K.: The Monte Carlo atmospheric radiative transfer model McArtim: introduction and validation of Jacobians and 3D features, J. Quant. Spectrosc. Ra., 112, 1119-1137, 2011.
10. Dorf, M., Bösch, H., Butz, A., Camy-Peyret, C., Chipperfield, M. P., Engel, A., Goutail, F., Grunow, K., Hendrick, F., Hrechanyy, S., Naujokat, B., Pommereau, J. P., Van Roozendael, M., Sioris, C., Stroh, F., Weidner, F., and Pfeilsticker, K.: Balloon-borne stratospheric BrO measurements: comparison with Envisat/SCIAMACHY BrO limb profiles, Atmos. Chem. Phys., 6, 2483-2501, doi:10.5194/acp-6-2483-2006, 2006a. (Pubitemid 43980752)
11. Dorf, M., Butler, J., Butz, A., Camy-Peyret, C., Chipperfield, M., Kritten, L., Montzka, S., Simmes, B., Weidner, F., and Pfeilsticker, K.: Long-term observations of stratospheric bromine reveal slow down in growth, Geophys. Res. Lett, 33, L24803, doi:10.1029/2006GL027714, 2006b. (Pubitemid 47277818)
12. Dorf, M., Butz, A., Camy-Peyret, C., Chipperfield, M. P., Kritten, L., and Pfeilsticker, K.: Bromine in the tropical troposphere and stratosphere as derived from balloon-borne BrO observations, Atmos. Chem. Phys., 8, 7265-7271, doi:10.5194/acp-8-7265-2008, 2008.
13. Erle, F., Grendel A., Perner D., Platt, U., and Pfeilsticker, K.: Evidence of heterogeneous bromine chemistry on cold stratospheric sulphate aerosols, Geophys. Res. Lett., 25, 23, 4329-4332, 1998. (Pubitemid 29178303)
14. Feng, W., Chipperfield, M., Davies, S., von der Gathen, S., Kyro, E., Volk, C., Ulanovsky, A., and Belyaev, G.: Large chemical ozone loss in 2004/05 Arctic Winter/Spring, Geophys. Res. Lett., 34, L09803, doi:10.1029/2006GL029098, 2007. (Pubitemid 47008170)
15. Ferlemann, F., Bauer, N., Fitzenberger, R., Harder, H., Osterkamp, H., Perner, D., Platt, U., Scheider, M., Vradelis, P., and Pfeilsticker, K.: Differential optical absorption spectroscopy instrument for stratospheric balloon-borne trace gas studies, Appl. Opt., 39, 2377-2386, 2000.
16. Gurlit, W., Bösch, H., Bovensmann, H., and Burrows., J. P., Butz, A., Camy-Peyret, C., Dorf, M., Gerilowski, K., Lindner, A., Noël, S., Platt, U., Weidner, F., and Pfeilsticker, K.: The UV-A and visible solar irradiance spectrum: inter-comparison of absolutely calibrated, spectrally medium resolution solar irradiance spectra from balloon- and satellite-borne measurements, Atmos. Chem. Phys., 5, 1879-1890, doi:10.5194/acp-5-1879-2005, 2005. (Pubitemid 41264073)
17. Harder, H., Camy-Peyret, C., Ferlemann, F., Fitzenberger, R., Hawat, T., Osterkamp, H., Schneider, M., Perner, D., Platt, U., Vradelis, P., and Pfeilsticker, K.: Stratospheric BrO profiles measured at different latitudes and seasons: atmospheric observations, Geophys. Res. Lett., 25, 3843-3846, 1998.
18. Harder, H., Bösch, H., Camy-Peyret, C., Chipperfield, M., Fitzenberger, R., Payan, S., Perner, D., Platt, U., Sinnhuber, B.-M., and Pfeilsticker, K.: Comparison of measured and modeled Stratospheric BrO: implications for the total amount of stratospheric bromine, Geophys. Res. Lett., 27, 3695-3698, 2000.
19. 3, Atmos. Meas. Tech., 3, 933-946, doi:10.5194/amt-3-933-2010, 2010.
20. Laube, J. C., Engel, A., Bönisch, H., Möbius, T., and Worton., D. R., Sturges, W. T., Grunow, K., and Schmidt, U.: Contribution of very short-lived organic substances to stratospheric chlorine and bromine in the tropics - a case study, Atmos. Chem. Phys., 8, 7325-7334, doi:10.5194/acp-8- 7325-2008, 2008.
21. 2 profile measurements in the artic vortex, Geophys. Res. Lett., 25, 2663-2666, 1998. (Pubitemid 29126157)
22. Platt, U. and Stutz, J.: Differential Optical Absorption Spec-troscopy (DOAS), Principle and Applications, ISBN 3-340-21193-4, Springer Verlag, Heidelberg, 2008.
23. Salawitch, R.: Atmospheric chemistry: biogenic bromine, Nature, 439, 275-277, 2006. (Pubitemid 43128842)
24. Sander, S., and Friedl., R. R., Barkern, J., Golden, D., Kurylo, M., Wine, P., Abbat, J., Burkholder, J., Moortgart, C., Huie, R., and Orkin, R. E.: Chemical kinetics and photochemical data for use in atmospheric studies, Technical Report, NASA/JPL Publication, 17, 2011.
25. Sinnhuber, B.-M., Rozanov, A., Sheode, N., Afe, O. T., Richter, A., Sinnhuber, M., Wittrock, F., Burrows, J. P., and Stiller., G. P., von Clarmann, T., and Linden, A.: Global observations of stratospheric bromine monoxide from SCIAMACHY, Geophys. Res. Lett., 32, 1-5, 2005. (Pubitemid 41782744)
26. Sinnhuber, B.-M., Sheode, N., Sinnhuber, M., Chipperfield, M. P., and Feng, W.: The contribution of anthropogenic bromine emissions to past stratospheric ozone trends: a modelling study, Atmos. Chem. Phys., 9, 2863-2871, doi:10.5194/acp-9-2863-2009, 2009.
27. Soller, R., Nicovich, J., and Wine, P.: Bromine nitrate photochemistry: quantum yields for O, Br, and BrO over the wavelength range 248-355 nm, J. Phys. Chem. A, 106, 8378-8385, 2002. (Pubitemid 35382462)
28. Spencer, J. E. and Rowland, F. S.: Bromine nitrate and its stratospheric significance, J. Phys. Chem., 82, 7-10, 1977.
29. von Glasow, R., von Kuhlmann, R., Lawrence, M. G., Platt, U., and Crutzen, P. J.: Impact of reactive bromine chemistry in the troposphere, Atmos. Chem. Phys., 4, 2481-2497, doi:10.5194/acp-4-2481-2004, 2004. (Pubitemid 40191225)
30. 2, and BrO: technical set-up and validation of the method, Atmos. Chem. Phys., 5, 1409-1422, doi:10.5194/acp-5-1409-2005, 2005. (Pubitemid 40899890)