Influence of pH and chloride concentration on the corrosion behavior of unalloyed copper in NaCl solution: A comparative study between the micro and macro scales

Materials

Volumn 5, Issue 12, 2012, Pages 2439-2464

  Arjmand, Farzin ^a   Adriaens, Annemie ^a  

^a GHENT UNIVERSITY   (Belgium)

Author keywords

Copper; EIS; Experimental design; Pitting corrosion; Polarization

Indexed keywords

ALKALINE PH; CHLORIDE CONCENTRATIONS; COMPARATIVE STUDIES; CORROSION BEHAVIOR; CORROSION POTENTIALS; CORROSIVE MEDIA; DROPLET CELLS; EIS; ELECTROCHEMICAL BEHAVIORS; ELECTROCHEMICAL RESPONSE; GRAIN SIZE; INFLUENCE OF PH; MACRO SCALE; MICRO AND MACRO; MICRO-CAPILLARIES; MICRO-SCALES; NACL CONCENTRATION; NACL SOLUTION; NEGATIVE POTENTIAL; PH VALUE; PIT INITIATION; POTENTIOSTATIC MEASUREMENTS;

ALKALINITY; DESIGN OF EXPERIMENTS; ELECTROCHEMICAL CORROSION; ELECTROCHEMICAL IMPEDANCE SPECTROSCOPY; EXPERIMENTS; PH; PITTING; POLARIZATION; SODIUM CHLORIDE; STATISTICS;

COPPER;

EID: 84869993761     PISSN: None     EISSN: 19961944     Source Type: Journal    
DOI: 10.3390/ma5122439     Document Type: Article

References (42)

1. Kear, G.; Walsh, F.C.; Barker, D.B.; Stokes, K.S. Electrochemical corrosion characteristics of copper in filtered and artificial seawater as a function of mass transfer conditions. In EuroCorr. 2000; Institute of Corrosion: Leighton Buzzard, UK, 2000.
2. Mathiyarasu, J.; Palaniswamy, N.; Muralidharan, V.S. Electrochemical behaviour of copper-nickel alloy in chloride solution. J. Chem. Sci. 1999, 111, 377-386.
3. Georgiadou, M.; Alkire, R. Modelling of copper etching in aerated chloride solutions. J. Appl. Electrochem. 1998, 28, 127-134.
4. Wagner, D.; Peimemann, H.; Siedlarek, H.; Campbell, S.A.; Campbell, N.; Walsh, F.C. Development in Marine Corrosion; The Royal Society of Chemistry: Cambridge, UK, 1998; pp. 103-118.
5. King, F.; Quin, M.J.; Litke, C.D. Oxygen reduction on copper in neutral NaCl solution. J. Electroanal. Chem. 1995, 385, 45-55.
6. Mansfeld, F.B.; Liu, G.; Xiao, H.; Tsai, C.H.; Little, B.J. The corrosion behavior of copper alloys, stainless steels and titanium in seawater. Corros. Sci. 1994, 36, 2063-2095.
7. Wood, R.J.K.; Fry, S.A. Corrosion of pure copper in flowing seawater under cavitating and noncavitating flow conditions. J. Fluids. Eng. 1990, 112, 218-224.
8. Deslouis, C.; Tribollet, B.; Mengoli, G.; Musiani, M. Electrochemical behaviour of copper in neutral aerated chloride solution. I. Steady-state investigation. J. Appl. Electrochem. 1988, 18, 374-383.
9. Lee, H.P.; Nobe, K. Kinetics and Mechanisms of Cu Electrodissolution in Chloride Media. J. Electrochem. Soc. 1986, 133, 2035-2043.
10. Smyrl, W.H. Digital Impedance for Faradaic Analysis: II. Electrodissolution of Cu in HCl. J. Electrochem. Soc. 1985, 132, 1555-1562.
11. Sanchez, M.; Gamby, J.; Perrot, H.; Rose, D.; Vivier, V. Microelectrochemistry of copper in NaCl solution: Comparison between conventional microelectrode and microelectrochemical cell. Electrochem. Commun. 2010, 12, 1230-1232.
12. Pilaski, M.; Hamelmann, T.; Moehring, A.; Lohrengel, M.M. Impedance spectroscopy in micro systems. Electrochim. Acta 2002, 47, 2127-2134.
13. Lohrengel, M.M.; Heiroth, S.; Kluger, K.; Pilaski, M.; Walther, B. Microimpedance-Localized material analysis. Electrochim. Acta 2006, 51, 1431-1436.
14. Dubuisson, E.; Lavie, P.; Dalard, F.; Caire, J.P.; Szunerits, S. Study of the atmospheric corrosion of galvanised steel in a micrometric electrolytic droplet. Electrochem. Commun. 2006, 8, 911-915.
15. Jorcin, J.B.; Krawiec, H.; Pebere, N.; Vignal, V. Comparison of local electrochemical impedance measurements derived from bi-electrode and microcapillary techniques. Electrochim. Acta 2009, 54, 5775-5781.
16. Birbilis, N.; Padgett, B.N.; Buchheit, R.G. Limitations in microelectrochemical capillary cell testing and transformation of electrochemical transients for acquisition of microcell impedance data. Electrochim. Acta 2005, 50, 3536-3544.
17. Dong, C.F.; Fu, A.Q.; Li, X.G.; Cheng, Y.F. Localized EIS characterization of corrosion of steel at coating defect under cathodic protection. Electrochim. Acta 2008, 54, 628-633.
18. Zhang, G.A.; Cheng, Y.F. Micro-electrochemical characterization and Mott-Schottky analysis of corrosion of welded X70 pipeline steel in carbonate/bicarbonate solution. Electrochim. Acta 2009, 55, 316-324.
19. Tang, X.; Cheng, Y.F. Micro-electrochemical characterization of the effect of applied stress on local anodic dissolution behavior of pipeline steel under near-neutral pH condition. Electrochim. Acta 2009, 54, 1499-1505.
20. Tang, X.; Cheng, Y.F. Localized dissolution electrochemistry at surface irregularities of pipeline steel. Appl. Surf. Sci. 2008, 254, 5199-5205.
21. Krawiec, H.; Vignal, V.; Banas, J. Local electrochemical impedance measurements on inclusion-containing stainless steels using microcapillary-based techniques. Electrochim. Acta 2009, 54, 6070-6074.
22. Li, M.C.; Cheng, Y.F. Corrosion of the stressed pipe steel in carbonate-bicarbonate solution studied by scanning localized electrochemical impedance spectroscopy. Electrochim. Acta 2008, 53, 2831-2836.
23. Zhong, C.; Tang, X.; Cheng, Y.F. Corrosion of steel under the defected coating studied by localized electrochemical impedance spectroscopy. Electrochim. Acta 2008, 53, 4740-4747.
24. Krawiec, H.; Vignal, V.; Amar, H.; Peyre, P. Local electrochemical impedance spectroscopy study of the influence of ageing in air and laser shock processing on the micro-electrochemical behaviour of AA2050-T8 aluminium alloy. Electrochim. Acta 2011, 56, 9581-9587.
25. Fleischmann, M.; Lasserre, F.J. Robinson, D. Swan, The application of microelectrodes to the study of homogeneous processes coupled to electrode reactions: Part I. EC' and CE reactions. J. Electroanal. Chem. 1984, 117, 97-114.
26. Galceran, J.; Puy, J.; Salvador, J.; Cecilia, J.; Van Leeuwen, H.P. Voltammetric liability of metal complexes at spherical microelectrodes with various radii. J. Electroanal. Chem. 2001, 505, 85-94.
27. Brookes, B.A.; Macfie, G.; Compton, R.G. Simulation of square wave voltammetry at hemispherical electrodes: electrochemically reversible, irreversible and quasi-reversible processes. J. Phys. Chem. B 2000, 104, 5784-5789.
28. Van Leeuwen, H.P.; Pinheiro, J.P. Lability criteria for metal complexes in micro-electrode voltammetry. J. Electroanal. Chem. 1999, 471, 55-61.
29. Molina, A.; Serna, C.; Martinez-Ortiz, F. Square wave voltammetry for a pseudo-first-order catalytic process at spherical electrodes. J. Electroanal. Chem. 2000, 486, 9-15.
30. Komrosky-Lovrić, S.; Lovrić, M.; Bond, A. Square-wave voltammetry at spherical and disk microelectrodes as a function of electrode radius and frequency. Electroanalysis 1993, 5, 29-40.
31. Schultz, J.; W.; Bressel, A. Principles of electrochemical micro- and nano-system technologies. Electrochim. Acta 2001, 47, 3-21.
32. Bohni, H.; Suter, T.; Schreyer, A. Micro- and nanotechniques to study localized corrosion. Electrochim. Acta 1995, 40, 1361-1368.
33. Arjmand, F.; Adriaens, A. Investigation of 304L stainless steel in a NaCl solution using a microcapillary electrochemical droplet cell: Comparison with conventional electrochemical techniques. Electrochim. Acta 2012, 59, 222-227.
34. Alfantazi, A.M.; Ahmed, T.M.; Tromans, D. Corrosion behavior of copper alloys in chloride media. Mater. Design 2009, 30, 2425-2430.
35. Arjmand, F.; Adriaens, A. Electrochemical quantification of copper-based alloys using voltammetry of microparticles: optimization of the experimental conditions. J. Solid State Electrochem. 2012, 16, 535-543.
36. Bonora, P.L.; Deflorian, F.; Fedrizzi, L. Electrochemical impedance spectroscopy as a tool for investigating underpaint corrosion. Electrochim. Acta 1996, 41, 1073-1082
37. Ruan, C.; Yang, L.; Li, Y. Immunobiosensor chips for detection of escherichia coli O157:H7 using electrochemical impedance spectroscopy. Anal. Chem. 2002, 74, 4814-4820.
38. Liu, C.; Bi, Q.; Leyland, A.; Matthews, A. An electrochemical impedance spectroscopy study of the corrosion behaviour of PVD coated steels in 0.5 N NaCl aqueous solution: Part I. Establishment of equivalent circuits for EIS data modelling. Corros. Sci. 2003, 45, 1243-1256.
39. Andreatta, F.; Lohrengel, M.M.; Terryn, H.; de Wit, J.H.W. Electrochemical characterisation of aluminium AA7075-T6 and solution heat treated AA7075 using a micro-capillary cell. Electrochim. Acta 2003, 48, 3239-3247.
40. Box, G.E.P.; Hunter, W.G.; Hunter, J.S. Statistics for Experimenters: An Introduction to Design, Data Analysis and Model Building; John Wiley and Sons: New York, NY, USA, 1978.
41. Stephan, D.D.; Werner, J.; Yeater, R.P. Essential regression and experimental design for chemist and engineers, MS Excel add in software package, 1998-2001. Available online: http://www.jowerner.homepage.t-online.de/ERPref.html (accessed on 20 November 2012).
42. Bulacov, I.; Jirkovsky, J.; Muller, M.; Heimann, R.B. Induction plasma-sprayed photocatalytically active titania coatings and their characterisation by micro-Raman spectroscopy. Surf. Coat. Technol. 2006, 201, 255-264.