Effects of 2 nm size added heterogeneity on non-exponential dielectric response, and the dynamic heterogeneity view of molecular liquids

Journal of Chemical Physics

Volumn 137, Issue 10, 2012, Pages

  Johari, G P ^a   Khouri, J ^a  

^a MCMASTER UNIVERSITY   (Canada)

Author keywords

[No Author keywords available]

Indexed keywords

DIELECTRIC RELAXATION SPECTRA; DIELECTRIC RESPONSE; DIFFERENT SIZES; DIGLYCIDYL ETHER OF BISPHENOL-A; DIPOLAR GROUPS; DYNAMIC HETEROGENEITY; EFFECTS OF TEMPERATURE; LINEAR RESPONSE; MOLECULAR LIQUIDS; MOLECULAR SIZE; NON-LINEAR RESPONSE; PLASTIC CRYSTALS; POLYHEDRAL OLIGOMERIC SILSESQUIOXANES; PROBE MOLECULES; RESPONSE PARAMETERS; RIGID MOLECULES; SIDE-CHAINS; SILSESQUIOXANES; TRANSLATIONAL DIFFUSION;

ETHERS; MOLECULES; OLIGOMERS; PHENOLS; DIELECTRIC RELAXATION; MIXTURES;

DIELECTRIC LIQUIDS;

2,2 BIS(4 GLYCIDYLOXYPHENYL)PROPANE; 2,2-BIS(4-GLYCIDYLOXYPHENYL)PROPANE; BENZHYDRYL DERIVATIVE; EPOXIDE; ORGANOSILICON DERIVATIVE;

ARTICLE; CHEMICAL STRUCTURE; CHEMISTRY; ELECTROCHEMICAL IMPEDANCE SPECTROSCOPY; PARTICLE SIZE; SURFACE PROPERTY;

BENZHYDRYL COMPOUNDS; DIELECTRIC SPECTROSCOPY; EPOXY COMPOUNDS; MODELS, MOLECULAR; MOLECULAR STRUCTURE; ORGANOSILICON COMPOUNDS; PARTICLE SIZE; SURFACE PROPERTIES;

EID: 84866409919     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.4748355     Document Type: Article

References (51)

1. J. G. Kirkwood and R. M. Fuoss, J. Am. Chem. Soc. 63, 385 (1941). 10.1021/ja01847a013
2. M. Cardona, R. V. Chamberlin, and W. Marx, Ann. Phys. (Leipzig) 16, 842 (2007). 10.1002/andp.200710269
3. C. K. Majumdar, Solid State Comm. 9, 1087 (1971). 10.1016/0038-1098(71) 90468-6
4. A. Hunt, J. Non-Cryst. Solids 160, 183 (1993). 10.1016/0022-3093(93) 91265-5
5. K. L. Ngai, Relaxation and Diffusion in Complex Systems (Springer, New York, 2011).
6. G. Adam and J. H. Gibbs, J. Chem. Phys. 43, 139 (1965). 10.1063/1.1696442
7. K. Schmidt-Rohr and H. W. Spiess, Phys. Rev. Lett. 66, 3020 (1991). 10.1103/PhysRevLett.66.3020
8. S. C. Kuebler, A. Heuer, and H. W. Spiess, Phys. Rev. E 56, 741 (1997). 10.1103/PhysRevE.56.741
9. H. Sillescu, J. Chem. Phys. 104, 4877 (1996). 10.1063/1.471121
10. R. Böhmer, G. Diezemann, G. Hinze, and H. Sillescu, J. Chem. Phys. 108, 890 (1998). 10.1063/1.475452
11. R. Böhmer, R. V. Chamberlin, G. Diezemann, B. Geil, A. Heuer, H. Hinze, S. C. Kuebler, R. Richert, B. Schiener, H. Sillescu, H. W. Spiess, U. Tracht, and W. Wilhelm, J. Non-Cryst. Solids 235, 1 (1998). 10.1016/S0022- 3093(98)00581-X
12. U. Tracht, M. Wilhelm, A. Heuer, H. Feng, K. Schmidt-Rohr, and H. W. Spiess, Phys. Rev. Lett. 81, 2727 (1998). 10.1103/PhysRevLett.81.2727
13. S. A. Reinsberg, X. H. Qiu, M. Wilhelm, H. W. Spiess, and M. D. Ediger, J. Chem. Phys. 114, 7299 (2001). 10.1063/1.1369160
14. W. Schnauss, F. Fujara, and H. Sillescu, J. Chem. Phys. 97, 1378 (1992). 10.1063/1.463264
15. A. Dö G. Hinze, G. Diezemann, R. Böhmer, and H. Sillescu, Acta Polym. 49, 56 (1998). 10.1002/(SICI)1521-4044(199801)49:156::AID-APOL56>3.0. CO;2-7
16. W. W. Graessley, J. Chem. Phys. 130, 164502 (2009). 10.1063/1.3119641
17. S. A. Mackowiak, L. M. Leone, and L. J. Kaufman, Phys. Chem. Chem. Phys. 13, 1786 (2011). 10.1039/c0cp01860k
18. C. T. Moynihan and J. Shroeder, J. Non-Cryst. Solids 160, 52 (1993). 10.1016/0022-3093(93)90283-4
19. J. Schroeder, M. A. Whitmore, M. R. Silvestri, S. K. Saha, and C. T. Moynihan, J. Non. Cryst. Solids 161, 157 (1993). 10.1016/0022-3093(93)90689-U
20. M. Lee, S. K. Saha, C. T. Moynihan, and J. Schroeder, J. Non. Cryst. Solids 222, 369 (1997). 10.1016/S0022-3093(97)90138-1
21. N. A. Bokov, J. Non-Cyst. Solids 17 7, 74 (1994). 10.1016/0022-3093(94) 90516-9
22. G. P. Johari and M. Goldstein, J. Chem. Phys. 53, 2372 (1970). 10.1063/1.1674335
23. G. P. Johari, Ann. N. Y. Acad. Sci. 279, 117 (1976). 10.1111/j.1749-6632. 1976.tb39701.x
24. K. L. Ngai, R. Casalini, S. Capaccioli, M. Paluch, and C. M. Roland, Dispersion of the structural relaxation and the vitrification of liquids., in Fractals, Diffusion and Relaxation in Disordered Complex Systems, Advances in Chemical Physics Vol. 133 (Wiley, New York, 2006), Chap. 10.
25. J. Khouri and G. P. Johari, J. Phys. Chem. B. 115, 13489 (2011). 10.1021/jp2071343
26. J. Khouri and G. P. Johari, Thermochim. Acta 540, 74 (2012). 10.1016/j.tca.2012.04.012
27. K. Venkateshan and G. P. Johari, J. Phys. Chem. B 108, 15049 (2004). 10.1021/jp0476951
28. E. W. Montroll and J. T. Bendler, J. Stat. Phys. 34, 129 (1984). 10.1007/BF01770352
29. M. Dishon, G. H. Weiss, and J. T. Bendler, J. Res. Natl. Bur. Stand. 90, 27 (1985). 10.6028/jres.090.002
30. K. Ueno and C. A. Angell, J. Phys. Chem. B 115, 13994 (2011). The POSS used in their study had seven iso-octyl groups and one propylamine group bonded to the Si atoms at these vertices. 10.1021/jp111398r
31. N. A. Bokov, J. Non-Cyst. Solids 354, 1119 (2008). 10.1016/j.jnoncrysol. 2006.10.078
32. K. Adachi, S. Suga, and S. Seki, Bull. Chem. Soc. Jpn. 41, 1073 (1968). 10.1246/bcsj.41.1073
33. G. P. Johari, Phil. Mag. 41, 41 (1980). 10.1080/13642818008245368
34. O. Yamamuro, M. Ishikawa, I. Kishimoto, J.-J. Pinvidic, and T. Matsuo, J. Phys. Soc. Jpn. 68, 2969 (1999). 10.1143/JPSJ.68.2969
35. R. Brand, P. Lunkenheimer, and A. Loidl, J. Chem. Phys. 116, 10386 (2002). 10.1063/1.1477186
36. K. Pathmanathan and G. P. Johari, J. Phys. C 18, 6535 (1985). 10.1088/0022-3719/18/35/018
37. D. A. Turton and K. Wynne, J. Chem. Phys. 131, 201101 (2009). 10.1063/1.3265862
38. D. J. Bernal, Proc. R. Soc. London A 280, 299 (1964). 10.1098/rspa.1964.0147
39. W. W. Wood, in Physics of Simple Fluids, edited by, H. N. V. Temperley, J. S. Rowlinson, and, G. S. Rushbrooke, (North Holland, Amsterdam, 1968), pp. 115-230.
40. J. M. Ziman, Models of Disorder, the Theoretical Physics of Homogeneously Disordered Systems (Cambridge University Press, New York, 1982).
41. K. L. Ngai and S. Capaccioli, J. Phys.: Condens. Matter 20, 244101 (2008). 10.1088/0953-8984/20/24/244101
42. A. I. Nielsen, T. Christensen, B. Jakobsen, K. Niss, N. B. Olsen, R. Richert, and J. C. Dyre, J. Chem. Phys. 130, 154508 (2009). 10.1063/1.3098911
43. R. Zangi, S. A. Mackowiak, and L. J. Kaufman, J. Chem. Phys. 126, 104501 (2007). 10.1063/1.2434969
44. S. A. Mackowiak, J. M. Noble, and L. J. Kaufman, J. Chem. Phys. 135, 214503 (2011). 10.1063/1.3664125
45. G. P. Johari, J. Chem. Phys. 137, 027101 (2012). 10.1063/1.4732080
46. G. P. Johari and C. P. Smyth, J. Am. Chem. Soc. 91, 5168 (1969). 10.1021/ja01046a043
47. J. G. Berberian and R. H. Cole, J. Chem. Phys. 84, 6921 (1986). 10.1063/1.450698
48. J. G. Berberian, J. Non-Cryst. Solids 131-133, 48 (1991). 10.1016/0022-3093(91)90270-G
49. W. Huang, S. Shahriari and R. Richert, J. Chem. Phys 123, 164504 (2005). 10.1063/1.2084949
50. L-M. Wang, Y. Tian, R. Liu, and R. Richert, J. Phys. Chem. B 114, 3618 (2010). 10.1021/jp912223j
51. E. Tombari and G. P. Johari, J. Chem. Phys. 97, 6677 (1992). 10.1063/1.463673