Vapor hydration of SON68 glass from 90 °c to 200 °c: A kinetic study and corrosion products investigation

Journal of Non-Crystalline Solids

Volumn 358, Issue 21, 2012, Pages 2894-2905

  Neeway, James ^a   Abdelouas, Abdesselam ^a   Grambow, Bernd ^a   Schumacher, Stéphan ^b   Martin, Christelle ^b   Kogawa, Masashi ^c   Utsunomiya, Satoshi ^c   Gin, Stéphane ^d   Frugier, Pierre ^d  

^a UNIVERSITÉ DE NANTES   (France)

^b ANDRA   (France)

^c KYUSHU UNIVERSITY   (Japan)

^d CEA VALRHO Centre de Marcoule   (France)

Author keywords

Geological disposal; SON68; Vapor hydration

Indexed keywords

CHEMICAL COMPOSITIONS; CORROSION PRODUCTS; DISPOSAL SITES; DISSOLUTION RATES; ENERGY DISPERSIVE X RAY SPECTROSCOPY; EXPERIMENTAL CONDITIONS; EXTERNAL LAYERS; GEOLOGICAL DISPOSALS; GLASS CORROSION; GLASS HYDRATION PROCESS; GLASS SURFACES; HYDRATION RATE; KINETIC STUDY; MOBILE ELEMENTS; MOBILITY VARIATION; NUCLEAR WASTE GLASS; PRISTINE GLASS; SON68; SON68 GLASS; STAINLESS STEEL AUTOCLAVES; TOF SIMS; TOF-SIMS ANALYSIS; TRANSMISSION ELECTRON MICROSCOPY TEM; UNSATURATED CONDITION; VAPOR HYDRATION TESTS;

CORROSION RATE; EXPERIMENTS; GLASS; HYDRATION; LEACHING; SCANNING ELECTRON MICROSCOPY; SECONDARY ION MASS SPECTROMETRY; SOLUTIONS; TRANSMISSION ELECTRON MICROSCOPY; X RAY SPECTROSCOPY;

VAPORS;

EID: 84865998874     PISSN: 00223093     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.jnoncrysol.2012.07.020     Document Type: Article

References (45)

1. E. Gaucher, C. Robelin, J.M. Matray, G. Négrel, Y. Gros, J.F. Heitz, A. Vinsot, H. Rebours, A. Cassagnabère, and A. Bouchet ANDRA underground research laboratory: interpretation of the mineralogical and geochemical data acquired in the Callovian-Oxfordian formation by investigative drilling Phys. Chem. Earth, Parts A/B/C 29 2004 55 77
2. ANDRA, Dossier 2005 Argile, Tome Phenomenological Evolution of a Geological Repository ANDRA Report C.RP.ADS.04.0025 2005 1 525
3. J.K. Bates, W.L. Ebert, and T.J. Gerding Vapor hydration and subsequent leaching of transuranic-containing SRL and WV glasses Proceedings of the International High-Level Radioactive Waste Management Topical Meeting, American Nuclear Society, Las Vgas, NV, April 8-12 1990 1095
4. J.K. Bates, L.J. Jardine, and M.J. Steindler Hydration aging of nuclear waste glass Science 218 1982 51 54
5. J.S. Luo, W.L. Ebert, J.J. Mazer, and J.K. Bates Simulation of natural corrosion by vapor hydration test: seven-year results Mater. Res. Soc. Symp. Proc. 465 1997 157 163
6. T.A. Abrajano Jr., J.K. Bates, and J.J. Mazer Aqueous corrosion of natural and nuclear waste glasses II. Mechanisms of vapor hydration of nuclear waste glasses J. Non-Cryst. Solids 108 1989 269 288
7. A. Jiricka, J.D. Vienna, P. Hrma, and D.M. Strachan The effect of experimental conditions and evaluation techniques on the alteration of low activity glasses by vapor hydration J. Non-Cryst. Solids 292 2001 25 43
8. W.L. Gong, L.M. Wang, R.C. Ewing, E. Vernaz, J.K. Bates, and W.L. Ebert Analytical electron microscopy study of surface layers formed on the French SON68 nuclear waste glass during vapor hydration at 200 °C J. Nucl. Mater. 254 1998 249 265
9. W.L. Ebert, J.K. Bates, and W.L. Bourcier The hydration of borosilicate waste glass in liquid water and steam at 200 °C Waste Manage. 11 1991 205 221
10. K.L. Hull Reasserting the utility of obsidian hydration dating: a temperature-dependent empirical approach to practical temporal resolution with archaeological obsidians J. Archaeol. Sci. 28 2001 1025 1040
11. L.M. Anovitz, J.M. Elam, L.R. Riciputi, and D.R. Cole The failure of obsidian hydration dating: sources, implications, and new directions J. Archaeol. Sci. 26 1999 735 752
12. J.K. Bates, and E.C. Buck Waste glass weathering Mater. Res. Soc. Symp. Proc. 44 1993 15 27
13. W.L. Ebert, R.F. Hoburg, and J.K. Bates The sorption of water on obsidian and a nuclear waste glass Phys. Chem. Glasses 32 1990 133 137
14. 2O)4, a new compound formed during vapor hydration of an actinide-bearing borosilicate waste glass J. Nucl. Mater. 278 2000 290 300
15. D.M. Strachan Glass dissolution: testing and modeling for long-term behavior J. Nucl. Mater. 298 2001 69 77
16. A. International Standard Test Method for Measuring Waste Glass or Glass Ceramic Durability by Vapor Hydration Test (C1663) 2009 West Conshohocken, PA
17. P. Frugier, S. Gin, Y. Minet, T. Chave, B. Bonin, N. Godon, J.E. Lartigue, P. Jollivet, A. Ayral, L. De Windt, and G. Santarini SON68 nuclear glass dissolution kinetics: current state of knowledge and basis of the new GRAAL model J. Nucl. Mater. 380 2008 8 21
18. K.S. Pitzer, and D.J. Bradley Thermodynamics of High Temperature Brines 1979 Lawrence Berkeley Lab., Univ. California Berkeley, CA, USA 40
19. K.M. Davis, and M. Tomozawa An infrared spectroscopic study of water-related species in silica glasses J. Non-Cryst. Solids 201 1996 177 198
20. K. Ferrand, A. Abdelouas, and B. Grambow Water diffusion in the simulated French nuclear waste glass SON 68 contacting silica rich solutions: Experimental and modeling J. Nucl. Mater. 355 2006 54 67
21. M. Tsuji, S. Komareneni, and P. Malla Substituted tobermorites: 27Al and 29Si MASNMR, cation exchange, and water sorption studies J. Am. Chem. Soc. 74 1991 274 279
22. P. Mandaliev, T. Stumpf, J. Tits, R. Dähn, C. Walther, and E. Wieland Uptake of Eu(III) by 11 Å tobermorite and xonotlite: a TRLFS and EXAFS study Geochim. Cosmochim. Acta 75 2011 2017 2029
23. D.M. Strachan, and T.L. Croak Compositional effects on long-term dissolution of borosilicate glass J. Non-Cryst. Solids 272 2000 22 33
24. P. Van Iseghem, and B. Grambow The long-term corrosion and modelling of two simulated Belgian reference high-level waste glasses MRS Online Proc. Libr. 112 1987 631 640
25. S. Gin, and J.P. Mestre SON 68 nuclear glass alteration kinetics between pH 7 and pH 11.5 J. Nucl. Mater. 295 2001 83 96
26. S. Ribet, and S. Gin Role of neoformed phases on the mechanisms controlling the resumption of SON68 glass alteration in alkaline media J. Nucl. Mater. 324 2004 152 164
27. Y. Inagaki, A. Shinkai, K. Idemistu, T. Arima, H. Yoshikawa, and M. Yui Aqueous alteration of Japanese simulated waste glass P0798: effects of alteration-phase formation on alteration rate and cesium retention J. Nucl. Mater. 354 2006 171 184
28. J. Gauthier, H. Thomassin, and P. Le Coustumer Rôle de matériaux zéolitiques lors de l'altération expérimentale du verre nucléaire R7T7 C. R. Acad. Sci. II 5 1999 331 336
29. P. Frugier, T. Chave, S. Gin, and J.E. Lartigue Application of the GRAAL model to leaching experiments with SON68 nuclear glass in initially pure water J. Nucl. Mater. 392 2009 552 567
30. R.J. Short, R.J. Hand, N.C. Hyatt, and G. Möbus Environment and oxidation state of molybdenum in simulated high level nuclear waste glass compositions J. Nucl. Mater. 340 2005 179 186
31. 4): secondary solid solution formation during HLW borosilicate-glass dissolution Radiochim. Acta 92 2004 639 643
32. A. Abdelouas, J.-L. Crovisier, W. Lutze, B. Grambow, J.-C. Dran, and R. Müller Surface layers on a borosilicate nuclear waste glass corroded in MgCl2 solution J. Nucl. Mater. 240 1997 100 111
33. A. Abdelouas, J.-L. Crovisier, W. Lutze, R. Müller, and W. Bernotat Structure and chemical properties of surface layers developed on R7T7 simulated nuclear waste glass altered in brine at 190 °C Eur. J. Mineral. 7 1995 1101 1113
34. A. Sneyers, B. Grambow, P. Hernan, H.-J. Alheid, J.-F. Aranyossy, and L. Johnson NF-PRO introduction: recent advances in integrating European research on the near-field system Euradwaste 2008; 7th European Commission Conference on the Management and Disposal of Radioactive Waste 2008
35. P.K. Abraitis, B.P. McGrail, D.P. Trivedi, F.R. Livens, and D.J. Vaughan Single-pass flow-through experiments on a simulated waste glass in alkaline media at 40 °C: II. Experiments conducted with buffer solutions containing controlled quantities of Si and Al J. Nucl. Mater. 280 2000 206 215
36. P.K. Abraitis, B.P. McGrail, D.P. Trivedi, F.R. Livens, and D.J. Vaughan Single-pass flow-through experiments on a simulated waste glass in alkaline media at 40 °C: I. Experiments conducted at variable solution flow rate to glass surface area ratio J. Nucl. Mater. 280 2000 196 205
37. J.R. Houston, J.L. Herberg, R.S. Maxwell, and S.A. Carroll Association of dissolved aluminum with silica: connecting molecular structure to surface reactivity using NMR Geochim. Cosmochim. Acta 72 2008 3326 3337
38. F. Angeli, T. Charpentier, M. Gaillard, and P. Jollivet Influence of zirconium on the structure of pristine and leached soda-lime borosilicate glasses: towards a quantitative approach by 17O MQMAS NMR J. Non-Cryst. Solids 354 2008 3713 3722
39. P. Van Iseghem, M. Aertsens, S. Gin, D. Deneele, B. Grambow, P. McGrail, D. Strachan, and G. Wicks A Critical Evaluation of the Dissolution Mechanisms of High-level Waste Glasses in Conditions of Relevance for Geological Disposal (GLAMOR) Contract FIKW-CT-2001-20140 2006 European Commission
40. J.K. Bates, M.G. Seitz, and M.J. Steindler The relevance of vapor phase hydration aging to nuclear waste isolation Nucl. Chem. Waste Manag. 5 1984 63 73
41. A. Abdelouas, J.-L. Crovisier, J. Caurel, and E. Vernaz Analyse par microscopie électronique à transmission des produits de l'altération hydrothermale à 250 °C du verre nucléaire R7T7 C. R. Acad. Sci. Paris 317 series II 1993 1333 1340
42. C. Cailleteau, C. Weigel, A. Ledieu, P. Barboux, and F. Devreux On the effect of glass composition in the dissolution of glasses by water J. Non-Cryst. Solids 354 2008 117 123
43. N. Valle, A. Verney-Carron, J. Sterpenich, G. Libourel, E. Deloule, and P. Jollivet Elemental and isotopic (29Si and 18O) tracing of glass alteration mechanisms Geochim. Cosmochim. Acta 74 2010 3412 3431
44. S. Gin, C. Guittonneau, N. Godon, D. Neff, D. Rebiscoul, M. Cabie, and S. Mostefaoui Nuclear glass durability: new insight into alteration layer properties J. Phys. Chem. C 115 2011 18696 18706
45. S. Gin Protective Effect of the alteration gel: a key mechanism in the long-term behavior of nuclear waste glass Mater. Res. Soc. Symp. Proc. 663 2001 207 215