Controlled Synthesis and Characterization of Highly Dispersed Molybdenum Oxide Supported on Silica SBA-15

ChemCatChem

Volumn 3, Issue 11, 2011, Pages 1814-1821

  Thielemann, Jörg P ^a,b   Weinberg, Gisela ^b   Hess, Christian ^a  

^a DARMSTADT UNIVERSITY OF TECHNOLOGY   (Germany)

^b FRITZ HABER INSTITUT DER MAX PLANCK GESELLSCHAFT   (Germany)

Author keywords

Molybdenum; Raman spectroscopy; Silicates; Structure activity relationships; Synthesis design

Indexed keywords

AMBIENT CONDITIONS; BINDING ENERGY SHIFTS; CONTROLLED SYNTHESIS; ENERGY DISPERSIVE X-RAY; FUNCTIONALIZED; HIGH DENSITY; MESOPOROUS SBA-15; MO DENSITY; MOLYBDENUM OXIDE CATALYSTS; OXIDE SURFACE; STRUCTURE ACTIVITY RELATIONSHIPS; SUPPORTED ON SILICA; SYNTHESIS DESIGN; SYNTHESIS MECHANISM; X RAY FLUORESCENCE; XPS ANALYSIS;

BINDING ENERGY; CALCINATION; CRYSTALLINE MATERIALS; DEHYDRATION; DEWATERING; DISPERSIONS; MOLYBDENUM; PHOTOELECTRONS; RAMAN SCATTERING; RAMAN SPECTROSCOPY; SILICA; SILICATES; THERMOANALYSIS; X RAY PHOTOELECTRON SPECTROSCOPY;

MOLYBDENUM OXIDE;

EID: 84858081503     PISSN: 18673880     EISSN: 18673899     Source Type: Journal    
DOI: 10.1002/cctc.201100154     Document Type: Article

References (58)

1. M. A. Banares, H. Hu, I. E. Wachs, J. Catal. 1994, 150, 407.
2. W. Zhang, S. T. Oyama, J. Phys. Chem. 1996, 100, 10759.
3. H. Liu, E. Iglesia, J. Catal. 2002, 208, 1.
4. M. A. Banares, N. D. Spencer, M. D. Jones, I. E. Wachs, J. Catal. 1994, 146, 204.
5. K. Chen, A. T. Bell, E. Iglesia, J. Catal. 2002, 209, 35.
6. Z. Song, N. Mimura, J. T. Bravo-Suarez, T. Akita, S. Tsubota, S. T. Oyama, Appl. Catal. A: Gen. 2007, 316, 142.
7. K. A. Vikulov, I. V. Elev, B. N. Shelimov, V. B. Kazansky, J. Mol. Catal. 1989, 55, 126.
8. J. Handzlik, J. Ogonowski, R. Dula, J. Stoch, E. M. Serwicka, React. Kinet. Catal. Lett. 2003, 79, 135.
9. J. Handzlik, J. Phys. Chem. B 2005, 109, 20794.
10. J. J. P. Biermann, F. J. J. Janssen, J. R. H. Ross, Appl. Catal. A: Gen. 1992, 86, 165.
11. I. Nova, L. Lietti, L. Casagrande, L. Dall′Acqua, E. Giamello, P. Forzatti, Appl. Catal. B 1998, 17, 245.
12. H. Hu, I. E. Wachs, S. R. Bare, J. Phys. Chem. 1995, 99, 10897.
13. A. N. Desikan, W. Zhang, S. T. Oyama, J. Catal. 1995, 157, 740.
14. G. Tsilomelekis, A. Christodoulakis, S. Boghosian, Catal. Today 2007, 127, 139.
15. T. Ono, H. Kamisuki, H. Hisashi, H. Miyata, J. Catal. 1989, 116, 303.
16. G. Mestl, T. K. K. Srinivasan, Catal. Rev. Sci. Eng. 1998, 40, 451.
17. L. J. Gregoriades, J. Döbler, J. Sauer, J. Phys. Chem. C 2010, 114, 2967.
18. J. P. Thielemann, J. Kröhnert, C. Hess, J. Phys. Chem. C 2010, 114, 17092.
19. Z. Huang, W. Bensch, W. Sigle, P. A. vanAken, L. Kienle, T. Vitoya, H. Modrow, T. Ressler, J. Mater. Sci. 2008, 43, 244.
20. Y. Lou, H. Wang, Q. Zhang, Y. Wang, J. Catal. 2007, 247, 245.
21. P. C. Bakala, E. Briot, L. Salles, J. M. Brégeault, Appl. Catal. A: Gen. 2006, 300, 91.
22. J. A. Melero, J. Iglesias, J. M. Arsuaga, J. Sainz-Pardo, P. deFrutos, S. Blazquez, Appl. Catal. A: Gen. 2007, 331, 84.
23. H. Balcar, D. Mishra, E. Marceau, X. Carrier, N. Zilkova, Z. Bastl, Appl. Catal. A: Gen. 2009, 359, 129.
24. S. Chempath, Y. Zhang, A. T. Bell, J. Phys. Chem. C 2007, 111, 1291.
25. E. L. Lee, I. E. Wachs, J. Phys. Chem. C 2008, 112, 6487.
26. Y. Iwasawa, K. Asakura, H. Ishii, H. Kuroda, Z. Phys. Chem. 1985, 144, 105.
27. Y. Iwasawa, Adv. Catal. 1987, 35, 187.
28. Y. V. Plyuto, I. V. Babich, I. V. Plyuto, A. D. VanLangeveld, J. A. Moulijn, Appl. Surf. Sci. 1997, 119, 11.
29. Y. Barbaux, A. R. Elamrani, E. Payen, L. Gengembre, J. P. Bonelle, B. Grzybowska, Appl. Catal. 1988, 44, 117.
30. N. K. Nag, J. Phys. Chem. 1987, 91, 2324.
31. C. Hess, G. Tzolova-Müller, R. Herbert, J. Phys. Chem. C 2007, 111, 9471.
32. C. Hess, J. Catal. 2007, 248, 120.
33. D. TrongOn, D. Desplantier-Giscard, C. Danumah, S. Kaliaguine, Appl. Catal. A: Gen. 2001, 222, 299.
34. A. Taguchi, F. Schüth, Microporous Mesoporous Mater. 2005, 77, 1.
35. R. Ryoo, S. Jun, J. Phys. Chem. B 1997, 101, 317.
36. J. M. Kisler, M. L. Gee, G. W. Stevens, A. J. O'Connor, Chem. Mater. 2003, 15, 619.
37. A. S. O'Neil, R. Mokaya, M. Poliakoff, J. Am. Chem. Soc. 2002, 124, 10636.
38. R. Herbert, D. Wang, R. Schomäcker, R. Schlögl, C. Hess, ChemPhysChem 2009, 10, 2230.
39. J. Jarupatrakorn, M. P. Coles, T. D. Tilley, Chem. Mater. 2005, 17, 1818.
40. D. Y. Zhao, Q. S. Huo, J. L. Feng, B. F. Chmelka, G. D. Stucky, J. Am. Chem. Soc. 1998, 120, 6024.
41. S. Brunauer, P. H. Emmett, E. Teller, J. Am. Chem. Soc. 1938, 60, 309.
42. L. Jelinek, E. Kováts, Langmuir 1994, 10, 4225.
43. D. Briggs, M. P. Seah, Practical Surface Analysis, Wiley, Chichester, 1990.
44. C. J. Brinker, R. Kirkpatrick, D. R. Tallant, B. C. Bunker, B. Montez, J. Non-Cryst. Solids 1988, 99, 418.
45. D. R. Tallant, B. C. Bunker, C. J. Brinker, C. A. Balfe, Mater. Res. Soc. Symp. Proc. 1986, 73, 261.
46. B. C. Brinker, D. R. Tallant, E. P. Roth, C. S. Ashley, Mater. Res. Soc. Symp. Proc. 1986, 61, 387.
47. R. H. Stolen, G. E. Walrafen, J. Chem. Phys. 1976, 64, 2623.
48. D. Lin-Vien, N. B. Colthup, W. G. Fateley, J. G. Grasselli, The Handbook of Infrared and Raman Characteristic Frequencies of Organic Molecules, Academic Press, Boston, 1991.
49. H. Okabayashi, K. Taga, K. Miyagai, T. Uehara, T. Yoshida, E. Nishio, J. Phys. Chem. 1991, 95, 7932.
50. I. Shimizu, H. Okabayashi, K. Taga, A. Yoshino, E. Nishio, C. J. O'Connor, Vib. Spectrosc. 1997, 14, 125.
51. T. M. McEvoy, K. J. Stevenson, Langmuir 2005, 21, 3521.
52. J. P. Thielemann, T. Ressler, A. Walter, G. Tzolova-Müller, C. Hess, Appl. Catal. A: Gen. 2011, 399, 28.
53. C. Hess, R. Schlögl, Chem. Phys. Lett. 2006, 432, 139.
54. J. Moulder, W. Stickle, P. Sobol, K. Bomben, Handbook of X-ray Photoelectron Spectroscopy, Perkin-Elmer Corporation, 1992, and references therein.
55. Similarly, for the samples with higher molybdenum loadings (11.0 and 13.9wt%) FWHM values of 2.8±0.2eV were obtained.
56. S. O. Grim, L. J. Matienzo, Inorg. Chem. 1975, 14, 1014.
57. R. J. Colton, A. M. Guzman, J. W. Rabalais, J. Appl. Phys. 1978, 49, 409.
58. G. K. Wertheim, Z. Phys. B 1987, 66, 53.