Reactions of beryllium halides in liquid ammonia: The tetraammineberyllium cation [Be(NH 3) 4] 2+, its hydrolysis products, and the action of Be 2+ as a fluoride-ion acceptor

Chemistry - A European Journal

Volumn 18, Issue 7, 2012, Pages 2131-2142

  Kraus, Florian ^a   Baer, Sebastian A ^a   Buchner, Magnus R ^a   Karttunen, Antti J ^b  

^a TECHNICAL UNIVERSITY OF MUNICH   (Germany)

^b UNIVERSITY OF EASTERN FINLAND   (Finland)

Author keywords

ab initio calculations; beryllium; halides; NMR spectroscopy; X ray diffraction

Indexed keywords

AB INITIO CALCULATIONS; DEUTERATIONS; DINUCLEAR; HALIDES; HYDROLYSIS PRODUCTS; LIQUID AMMONIA; NMR ANALYSIS; QUANTUM CHEMICAL CALCULATIONS; QUANTUM CHEMICAL STUDIES; SINGLE CRYSTAL X-RAY STRUCTURES; STRUCTURAL CHARACTERIZATION;

AMMONIA; BERYLLIUM; BERYLLIUM COMPOUNDS; CHEMICAL COMPOUNDS; CHLORINE; CHLORINE COMPOUNDS; DEUTERIUM; FLUORINE; HYDROLYSIS; NUCLEAR MAGNETIC RESONANCE SPECTROSCOPY; POSITIVE IONS; QUANTUM CHEMISTRY; RAMAN SPECTROSCOPY; X RAY DIFFRACTION;

LIQUIDS;

EID: 84856704767     PISSN: 09476539     EISSN: 15213765     Source Type: Journal    
DOI: 10.1002/chem.201103012     Document Type: Article

References (101)

1. K. Dehnicke, B. Neumüller, Z. Anorg. Allg. Chem. 2008, 634, 2703-2728.
2. S. Metz, M. C. Holthausen, G. Frenking, Z. Anorg. Allg. Chem. 2006, 632, 814-818.
3. J. R. Bill, D. G. Mack, M. T. Falta, L. A. Maier, A. K. Sullivan, F. G. Joslin, A. K. Martin, B. M. Freed, B. L. Kotzin, A. P. Fontenot, J. Immunol. 2005, 175, 7029-7037.
4. K. J. Cummings, A. B. Stefaniak, M. A. Virji, K. Kreiss, Environ. Health Perspect. 2009, 117, 1250-1256.
5. L. S. Newman, Sarcoidosis 1995, 12, 7-19.
6. L. Richeldi, R. Sorrentino, C. Saltini, Science 1993, 262, 242-244.
7. B. L. Scott, T. M. McCleskey, A. Chaudhary, E. Hong-Geller, S. Gnanakaran, Chem. Commun. 2008, 2837-2847.
8. C. Strupp, Ann. Occup. Hyg. 2011, 55, 30-42.
9. C. Strupp, Ann. Occup. Hyg. 2011, 55, 43-56.
10. Z. Wang, G. M. Farris, L. S. Newman, Y. Shou, L. A. Maier, H. N. Smith, B. L. Marrone, Toxicology 2001, 165, 27-38.
11. Z. Wang, P. S. White, M. Petrovic, O. L. Tatum, L. S. Newman, L. A. Maier, B. L. Marrone, J. Immunol. 1999, 163, 1647-1653.
12. A. F. Holleman, E. Wiberg, Lehrbuch der Anorganischen Chemie, Vol. 102, Walter de Gruyter, Berlin, New York, 2007, pp. 1-2149.
13. H. Schmidbaur, M. Schmidt, A. Schier, J. Riede, T. Tamm, P. Pyykkö, J. Am. Chem. Soc. 1998, 120, 2967-2968.
14. H. Schmidbaur, Coord. Chem. Rev. 2001, 215, 223-242.
15. M. Schmidt, H. Schmidbaur, Z. Naturforsch. 1998, 53b, 1294-1300.
16. M. Schmidt, A. Bauer, H. Schmidbaur, Inorg. Chem. 1997, 36, 2040-2043.
17. M. Schmidt, A. Schier, J. Riede, H. Schmidbaur, Inorg. Chem. 1998, 37, 3452-3453.
18. H. Kakihana, L. G. Sillén, Acta Chem. Scand. 1956, 10, 985-1005.
19. M. P. Dressel, S. Nogai, R. J. F. Berger, H. Schmidbaur, Z. Naturforsch. 2003, 58b, 173-182.
20. H. Schmidbaur, O. Kumberger, J. Riede, Inorg. Chem. 1991, 30, 3101-3103.
21. R. Han, G. Parkin, Inorg. Chem. 1993, 32, 4968-4970.
22. K. Ruhlandt-Senge, R. A. Bartlett, M. Olmstead, P. P. Power, Inorg. Chem. 1993, 32, 1724-1728.
23. Y. Sohrin, H. Kokusen, S. Kihara, M. Matsui, Y. Kushi, M. Shiro, J. Am. Chem. Soc. 1993, 115, 4128-4136.
24. B. Neumüller, K. Dehnicke, R. Puchta, Z. Anorg. Allg. Chem. 2008, 634, 1473-1476.
25. R. Puchta, R. van Eldik, Z. Anorg. Allg. Chem. 2008, 634, 735-739.
26. R. Puchta, R. van Eldik, Helv. Chim. Acta 2008, 91, 1063-1071.
27. R. Puchta, R. van Eldik, Z. Anorg. Allg. Chem. 2008, 634, 1915-1920.
28. R. Puchta, N. van Eikema Hommes, R. van Eldik, Helv. Chim. Acta 2005, 88, 911-922.
29. R. Puchta, E. Pasgreta, R. van Eldik, Advances in Inorganic Chemistry and Radiochemistry 2009, 61, 523-571.
30. R. Puchta, B. Neumüller, K. Dehnicke, Z. Anorg. Allg. Chem. 2009, 635, 1196-1199.
31. A. Mederos, S. Dominguez, E. Chinea, F. Brito, F. Cecconi, J. Coord. Chem. 2001, 53, 191-222.
32. C. Y. Wong, J. D. Woolins, Coord. Chem. Rev. 1994, 130, 243-273.
33. D. A. Everest, The Chemistry of Beryllium, Elsevier Publishing Company, Amsterdam, London, NewYork, 1964, pp. 1-151.
34. F. Cecconi, C. A. Ghilardi, S. Midollini, A. Orlandini, A. Mederos, Inorg. Chem. 1998, 37, 146-148.
35. W. Massa, K. Dehnicke, Z. Anorg. Allg. Chem. 2007, 633, 1366-1370.
36. C. A. Beevers, H. A. Lipson, Z. Kristallogr. 1932, 82, 297.
37. I. G. Dance, H. C. Freeman, Acta Crystallogr. B 1969, 25, 304-310.
38. V. Divjakovic, A. Edenharter, W. Nowicki, B. Ribar, Z. Kristallogr. 1976, 144, 314.
39. H. D. Lutz, H. Möller, M. Maneva, W. Paulus, A. Cousson, J. P. Lauriat, E. Elkaim, Z. Kristallogr. 1996, 211, 170.
40. S. K. Sikka, R. Chidambaram, Acta Crystallogr. B 1969, 25, 310-315.
41. M. Wildner, D. Stoilova, M. Georgiev, V. Karadjova, J. Mol. Struct. 2004, 707, 123.
42. B. T. R. Littlefield, C. Hinde, M. T. Weller, Dalton Trans. 2011, 40, 782-784.
43. J. Jander, V. Doetsch, U. Engelhardt, J. Fischer, C. Lafrenz, H. Nagel, W. Renz, G. Türk, T. von Volkmann, G. Weber, in Chemie in nichtwäßrigen ionisierenden Lösungsmitteln-Chemie in wasserfreiem flüssigem Ammoniak, 1 st ed., (Eds.: G. Jander, H. Spandau, C. C. Addison,) Friedr. Vieweg & Sohn, Braunschweig 1966, pp. 1-561.
44. D. Nicholls, Topics in Inorganic and General Chemistry, Monograph 17: Inorganic Chemistry in liquid Ammonia, Elsevier Scientific Publishing Company, Amsterdam, Oxford, NewYork, 1979, pp. 1-238.
45. M. P. Lebeau, Ann. Chim. Phys. 1899, 16, 457-503.
46. K. Mieleitner, H. Steinmetz, Z. Anorg. Allg. Chem. 1913, 80, 71-78.
47. F. W. Bergstrom, J. Am. Chem. Soc. 1928, 50, 657-662.
48. A. I. Grigor'ev, N. K. Evseeva, V. A. Sipachev, Zhurnal Strukturnoi Khimii 1969, 10, 469-473.
49. R. A. Kovar, G. L. Morgan, J. Am. Chem. Soc. 1970, 92, 5067-5072.
50. K. H. Schmidt, A. Müller, Coord. Chem. Rev. 1976, 19, 41-97.
51. W. Biltz, C. Messerknecht, Z. Anorg. Allg. Chem. 1925, 148, 157-169.
52. E. C. Franklin, C. A. Kraus, American Chemical Journal 1898, 20, 820-853.
53. W. Biltz, E. Rahlfs, Z. Anorg. Allg. Chem. 1927, 166, 351-376.
54. A. I. Grigor′ev, V. A. Sipachev, A. V. Novoselova, Russ. J. Inorg. Chem. 1967, 12, 319-321.
55. F. Kraus, M. B. Fichtl, S. A. Baer, Z. Naturforsch. 2009, 64b, 257-262.
56. B. Neumüller, K. Dehnicke, Z. Anorg. Allg. Chem. 2010, 636, 515-517.
57. B. Neumüller, K. Dehnicke, Z. Anorg. Allg. Chem. 2010, 636, 1767-1771.
58. B. Neumüller, K. Dehnicke, Z. Anorg. Allg. Chem. 2010, 636, 1516-1521.
59. S. Chadwick, U. Englich, K. Ruhlandt-Senge, Angew. Chem. 1998, 110, 3204-3206
60. Angew. Chem. Int. Ed. 1998, 37, 3007-3009.
61. S. Chadwick, U. Englich, K. Ruhlandt-Senge, Angew. Chem. 1998, 110, 3204-3206.
62. D. F. Gaines, K. M. Coleson, D. F. Hillenbrand, J. Magn. Reson. 1981, 44, 84-88.
63. P. G. Plieger, K. D. John, T. S. Keizer, T. M. McCleskey, A. K. Burell, R. L. Martin, J. Am. Chem. Soc. 2004, 126, 14651-14658.
64. R. Essmann, J. Mol. Struct. 1995, 351, 91-94.
65. K. Nakamoto, Infrared and Raman Spectra of Inorganic and Coordination Compounds, 4 th ed., John Wiley & Sons, NewYork, Chichester, Brisbane, Toronto, Singapore, 1986.
66. M. Prytz, Z. Anorg. Allg. Chem. 1929, 180, 355-369.
67. M. Prytz, Z. Anorg. Allg. Chem. 1931, 197, 103-112.
68. M. Prytz, Z. Anorg. Allg. Chem. 1937, 231, 238-248.
69. H. Diebler, M. Eigen, Z. Phys. Chem. (Muenchen Ger.) 1959, 20, 299-302.
70. H. Ohtaki, Inorg. Chem. 1967, 6, 808-813.
71. R. A. Gilbert, A. B. Garrett, J. Am. Chem. Soc. 1956, 78, 5501-5505.
72. M. Herlem, Bull. Soc. Chim. Fr. 1967, 1687-1692.
73. J. Badoz-Lambling, M. Herlem, A. Thiebault, Anal. Lett. 1969, 2, 35-39.
74. J. Bruno, J. Chem. Soc. Dalton Trans. 1987, 2431-2437.
75. R. Puchta, R. Kolbig, F. Weller, B. Neumüller, W. Massa, K. Dehnicke, Z. Anorg. Allg. Chem. 2010, 636, 2364-2371.
76. Y. Sohrin, H. Kokusen, S. Kihara, M. Matsui, Y. Kushi, M. Shiro, Chem. Lett. 1992, 1461-1464.
77. R. Faure, F. Bertin, H. Loiseleur, G. Thomas-David, Acta Crystallogr. B 1974, 30, 462-467.
78. Y. Sohrin, M. Matsui, Y. Hata, H. Hasegawa, H. Kokusen, Inorg. Chem. 1994, 33, 4376-4383.
79. J. A. Tossel, J. Magn. Reson. 1998, 135, 203-207.
80. E. Wolska, W. Szajda, J. Appl. Spectrosc. 1983, 38, 137-140.
81. P. Pyykkö, Mol. Phys. 2008, 106, 1965-1974.
82. P. E. Hansen, Progress in NMR Spectroscopy 1988, 20, 207-255.
83. W. H. Casey, B. L. Phillips, M. Karlsson, S. Nordin, J. P. Nordin, D. J. Sullivan, S. Neugebauer-Crawford, Geochim. Cosmochim. Acta 2000, 64, 2951-2964.
84. A. P. Lee, B. L. Phillips, M. Karlsson, S. Nordin, J. P. Nordin, D. J. Sullivan, S. Neugebauer-Crawford, Geochim. Cosmochim. Acta 2002, 66, 577-587.
85. F. Kraus, S. A. Baer, M. B. Fichtl, Eur. J. Inorg. Chem. 2009, 441-447.
86. Pfisterer, K., Doktorarbeit, Universität Regensburg, 2002.
87. H. J. Berthold, W. Preibsch, E. Vonholdt, Angew. Chem. 1988, 100, 1581-1583.
88. H. J. Berthold, E. Vonholdt, R. Wartchow, T. Vogt, Z. Kristallogr. 1992, 200, 225-235.
89. H. J. Berthold, E. Vonholdt, R. Wartchow, T. Vogt, Z. Kristallogr. 1993, 203, 199-214.
90. S. A. Baer, F. Kraus, Z. Naturforsch. 2010, 65b, 1177-1184.
91. C. Adamo, V. Barone, J. Chem. Phys. 1999, 110, 6158-6170.
92. J. P. Perdew, K. Burke, M. Ernzerhof, Phys. Rev. Lett. 1996, 77, 3865-3868.
93. T. H. Dunning Jr., J. Chem. Phys. 1989, 90, 1007.
94. F. Weigend, R. Ahlrichs, Phys. Chem. Chem. Phys. 2005, 7, 3297-3305.
95. A. E. Reed, R. B. Weinstock, F. Weinhold, J. Chem. Phys. 1985, 83, 735-746.
96. M. E. Harding, T. Metzroth, J. Gauss, A. A. Auer, J. Chem. Theory Comput. 2008, 4, 64-74.
97. J. F. Stanton J. Gauss, M. E. Harding, P. G. Szalay, with contributions from: A. A. Auer, R. J. Bartlett, U. Benedikt, C. Berger, D. E. Bernholdt, Y. J. Bomble, L. Cheng, O. Christiansen, M. Heckert, O. Heun, C. Huber, T.-C. Jagau, D. Jonsson, J. Jusélius, K. Klein, W. J. Lauderdale, D. A. Matthews, T. Metzroth, L. A. Mück, D. P. O'Neill, D. R. Price, E. Prochnow, C. Puzzarini, K. Ruud, F. Schiffmann, W. Schwalbach, S. Stopkowicz, A. Tajti, J. Vázquez, F. Wang, J. D. Watts and the integral packages MOLECULE (J. Almlöf and P. R. Taylor), PROPS (P. R. Taylor), ABACUS (T. Helgaker, H. J. Aa. Jensen, P. Jørgensen, and J. Olsen), and ECP routines by A. V. Mitin and C. van Wüllen. CFOUR, Coupled-Cluster techniques for Computational Chemistry; 2011.
98. R. Ahlrichs, M. Bär, M. Häser, H. Horn, C. Kölmel, Chem. Phys. Lett. 1989, 162, 165-169.
99. Gaussian 09, Revision A.1, M. J. Frisch, G. W. Trucks, H. B. Schlegel, G. E. Scuseria, M. A. Robb, J. R. Cheeseman, G. Scalmani, V. Barone, B. Mennucci, G. A. Petersson, H. Nakatsuji, M. Caricato, X. Li, H. P. Hratchian, A. F. Izmaylov, J. Bloino, G. Zheng, J. L. Sonnenberg, M. Hada, M. Ehara, K. Toyota, R. Fukuda, J. Hasegawa, M. Ishida, T. Nakajima, Y. Honda, O. Kitao, H. Nakai, T. Vreven, J. A. Montgomery, Jr., J. E. Peralta, F. Ogliaro, M. Bearpark, J. J. Heyd, E. Brothers, K. N. Kudin, V. N. Staroverov, R. Kobayashi, J. Normand, K. Raghavachari, A. Rendell, J. C. Burant, S. S. Iyengar, J. Tomasi, M. Cossi, N. Rega, J. M. Millam, M. Klene, J. E. Knox, J. B. Cross, V. Bakken, C. Adamo, J. Jaramillo, R. Gomperts, R. E. Stratmann, O. Yazyev, A. J. Austin, R. Cammi, C. Pomelli, J. W. Ochterski, R. L. Martin, K. Morokuma, V. G. Zakrzewski, G. A. Voth, P. Salvador, J. J. Dannenberg, S. Dapprich, A. D. Daniels, Ö. Farkas, J. B. Foresman, J. V. Ortiz, J. Cioslowski, D. J. Fox, Gaussian, Inc., Wallingford CT, 2009.
100. Kohout, M. DGrid. [4.6] 2011, Radebeul.
101. Oxford Diffraction. CrysalisRED. [1.171.32.15]. 2008. UK, Oxford Diffraction.