Radiolysis of acetic acid aqueous solutions-Effect of pH and persulfate addition

Chemical Engineering Journal

Volumn 174, Issue 2-3, 2011, Pages 504-509

  Criquet, Justine ^a   Karpel Vel Leitner, Nathalie ^a  

^a UNIVERSITÉ DE POITIERS   (France)

Author keywords

Carboxylic acid; E Beam; Oxidation; Sulfate radical; Water treatment

Indexed keywords

ACID SOLUTIONS; E-BEAM; HIGH YIELD; HYDROXYL RADICALS; INITIAL PH; INORGANIC CARBON; OXALIC ACID; SOLVATED ELECTRON; SULFATE RADICAL; SULFATE RADICALS;

ACETIC ACID; CARBOXYLIC ACIDS; DEGRADATION; IONIZING RADIATION; MINERALOGY; PETROLEUM TAR; RADIATION CHEMISTRY; RADIOLYSIS; RATE CONSTANTS; SOLUTIONS; WATER TREATMENT;

PH EFFECTS;

EID: 80054769124     PISSN: 13858947     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.cej.2011.07.079     Document Type: Article

References (44)

1. Boukari S.O.B., Pellizzari F., Karpel Vel Leitner N. Influence of persulfate ions on the removal of phenol in aqueous solution using electron beam irradiation. J. Hazard. Mater. 2011, 185:844-851.
2. Zhang S.J., Yu H.Q., Li Q.R. Radiolytic degradation of Acid Orange 7: a mechanistic study. Chemosphere 2005, 61:1003-1011.
3. Liu S.Y., Chen Y.P., Yu H.Q., Zhang S.J. Kinetics and mechanisms of radiation-induced degradation of acetochlor. Chemosphere 2005, 59:13-19.
4. Bojanowska-Czajka A., Drzewicz P., Zimek Z., Nichipor H., Nałe{ogonek}cz-Jawecki G., Sawicki J., Kozyra C., Trojanowicz M. Radiolytic degradation of pesticide 4-chloro-2-methylphenoxyacetic acid (MCPA)-experimental data and kinetic modelling. Radiat. Phys. Chem. 2007, 76:1806-1814.
5. Karpel Vel Leitner N., Berger P., Gehringer P. γ-Irradiation for the removal of atrazine in aqueous solution containing humic substances. Radiat. Phys. Chem. 1999, 55:317-322.
6. Yu S., Lee B., Lee M., Cho I.H., Chang S.W. Decomposition and mineralization of cefaclor by ionizing radiation: kinetics and effects of the radical scavengers. Chemosphere 2008, 71:2106-2112.
7. Spinks J., Woods R. An Introduction to Radiation Chemistry 1990, John Wiley & Sons Pub., New York. third ed.
8. Getoff N., Solar S. Radiation induced decomposition of chlorinated phenols in water. Radiat. Phys. Chem. 1988, 31:121-130.
9. Lee B., Jeong S.W. Effects of additives on 2,4,6-trinitrotoluene (TNT) removal and its mineralization in aqueous solution by gamma irradiation. J. Hazard. Mater. 2009, 165:435-440.
10. Gehringer P., Eschweiler H. Ozone/electron beam process for water treatment: design, limitations and economic considerations. Ozone: Sci. Eng. 1999, 21:523-538.
11. Zele S.R., Nickelsen M.G., Cooper W.J., Kurucz C.N., Waite T.D. Modeling kinetics of benzene, phenol, and toluene removal in aqueous solution using the high-energy electron beam process. Environnemental Applications of Ionizing Radiation 1998, 395-415. John Wiley & Sons, Inc. W.J. Cooper, R.D. Curry, E. O'Shea (Eds.).
12. Criquet J., Karpel Vel Leitner N. Electron beam irradiation of aqueous solution of persulfate ions. Chem. Eng. J. 2011, 169:256-262.
13. Rickman K.A., Mezyk S.P. Kinetic and mechanisms of sulfate radical oxidation of β-lactam antibiotics in water. Chemosphere 2010, 81:359-365.
14. Stanbury D.M. Reduction potentials involving inorganic free radicals in aqueous solution. Adv. Inorg. Chem. 1989, 33:69-138.
15. Anipsitakis G.P., Dionysiou D.D. Degradation of organic contaminants with sulfate radicals generated by peroxymonosulfate with cobalt. Environ. Sci. Technol. 2003, 37:4790-4797.
16. Liang C., Bruell C.J., Marley M.C., Sperry K.L. Persulfate oxidation for in situ remediation of TCE. II. Activated by chelated ferrous ion. Chemosphere 2004, 55:1225-1233.
17. Waldemer R.H., Tratnyek P.G., Johnson R.L., Nurmi J.T. Oxidation of chlorinated ethenes by heat-activated persulfate: kinetics and products. Environ. Sci. Technol. 2007, 41:1010-1015.
18. Hincapié Perez M., Maldonado P.G.M.I., Malato O., Oller F.I.P.I., Gernjak W., Malato S. Degradation of pesticides in water using solar advanced oxidation processes. Appl. Catal. B: Environ. 2006, 64:272-281.
19. Romero A., Santos A., Vicente C., Gonzales C. Diuron abatment using activated persulphate: effect of pH, Fe(II) and oxidant dosage. Chem. Eng. J. 2010, 162:257-265.
20. Diaz Kirmser E.M., Martire D.O., Gonzalez M.C., Rosso J.A. Degradation of the herbicides clomazone, paraquat and glyphosate by thermally activated persulfate. J. Agric. Food Chem. 2010, 58:12858-12862.
21. Vicente F., Santos A., Romero A., Rodriguez S. Kinetic study of diuron oxidation and mineralization by persulphate: effect of temperature, oxidant concentration and iron dosage method. Chem. Eng. J. 2011, 170:127-135.
22. Antoniou M.G., de la Cruz A.A., Dionysiou D.D. Intermediates and reaction pathways from the degradation of microcystin-LR with sulfate radicals. Environ. Sci. Technol. 2010, 44:7238-7244.
23. Antoniou M.G., de la Cruz A.A., Dionysiou D.D. Degradation of microcystin-LR using sulfate radicals generated through photolysis, thermolysis and e-transfer mechanisms. Appl. Catal. B.: Environ. 2010, 96:290-298.
24. Mendez-Diaz J., Sanchez-Polo M., Rivera-Utrilla J., Canonica S., von Gunten U. Advanced oxidation of the surfactant SDBS by means hydroxyl and sulphate radicals. Chem. Eng. J. 2010, 163:272-281.
25. Chan T.W., Graham N.J.D., Chu W. Degradation of iopromide by combined UV irradiation and peroxydisulfate. J. Hazard. Mater. 2010, 181:508-513.
26. Wang D., Li Y., Yang M., Han M. Decomposition of polycyclic aromatic hydrocarbons in atmospheric aqueous droplets through sulfate anion radicals: an experimental and theoretical study. Sci. Total Environ. 2008, 393:64-71.
27. Xu X.R., Li X.Z. Degradation of azo dye orange G in aqueous solution by persulfate and ferrous ion. Sep. Purif. Technol. 2010, 72:105-111.
28. Kusic H., Peternel I., Ukic S., Koprivanac N., Bolanca T., Papic S., Loncaric Bozic A. Modeling of iron activated persulfate oxidation treating reactive azo dye in water matrix. Chem. Eng. J. 2011, 172:109-121.
29. - radicals. Radiat. Res. 1978, 76:15-22.
30. Pellizzari F., Follut F., Karpel Vel Leitner N. A simplified reaction model predicting the effect of some parameters on the degradation of phenol in the electron beam process. Radiochim. Acta 2006, 94:481-486.
31. Follut F., Legube B., Karpel Vel Leitner N. Modelling of phenol removal in aqueous solution depending on the electron beam energy. Radiat. Phys. Chem. 2007, 76:827-833.
32. Villegas E., Pomeranz Y., Shellenberger J.A. Colorimetric determination of persulfate with alcian blue. Anal. Chim. Acta 1963, 29:145-148.
33. Mincher B.J., Curry R.D. Considerations for choice of a kinetic fig. of merit in process radiation chemistry for waste treatment. Appl. Radiat. Isot. 2000, 52:189-193.
34. 2 systems. Water Res. 1997, 31:1383-1397.
35. Criquet J., Nebout P., Karpel Vel Leitner N. Enhancement of carboxylic acid degradation with sulfate radical generated by persulfate activation. Water Sci. Technol. 2010, 61:1221-1226.
36. Criquet J., Karpel Vel Leitner N. Degradation of acetic acid with sulfate radical generated by persulfate ions photolysis. Chemosphere 2009, 77:194-200.
37. Gordeev A.V., Kosareva I.M., Bykov G.L., Ershov B.G. Simulation of the radiation-chemical transformations of acetic acid in aqueous solutions 2007, 41:233-238.
38. Buxton G.V., Greenstock C.L., Helman W.P., Ross A.B. Rate constants for reactions of radicals in aqueous solution. J. Phys. Chem. Ref. Data 1988, 17:513-886.
39. -: a study on the γ-radiolysis and pulse radiolysis of acetate in oxygenated aqueous solutions. Z. Naturforsch. 1985, 39b:217-221.
40. Herrmann H., Ervens B., Jacobi H.W., Wolke R., Nowacki P., Zellner R. CAPRAM 2.3: a chemical aqueous phase radical mechanism for tropospheric chemistry. J. Atmos. Chem. 2000, 36:231-284.
41. -. J. Phys. Chem. 1975, 79:2693-2700.
42. Furman O.S., Teel A.L., Ahmad M., Merker M.C., Watts R.J. Effect of basicity on persulfate reactivity. J. Environ. Eng. 2011, 137:241-247.
43. Liang C., Liang C.P., Chen C.C. pH dependence of persulfate activation by EDTA/Fe(III) for degradation of trichloroethylene. J. Contam. Hydrol. 2009, 106:173-182.
44. Liang C., Su H.W. Identification of sulfate and hydroxyl radicals in thermally activated persulfate. Ind. Eng. Chem. Res. 2009, 48:5558-5562.