Mutable lewis and brønsted acidity of aluminated SBA-15 as revealed by NMR of adsorbed pyridine- 15N

Langmuir

Volumn 27, Issue 19, 2011, Pages 12115-12123

  Gurinov, Andrey A ^a,b   Rozhkova, Yulia A ^b   Zukal, Arnošt ^c   Čejka, Jiří ^c   Shenderovich, Ilya G ^a,b  

^a FREIE UNIVERSITÄT BERLIN   (Germany)

^b ST PETERSBURG STATE UNIVERSITY   (Russian Federation)

^c J HEYROVSKÝ INSTITUTE OF PHYSICAL CHEMISTRY   (Czech Republic)

Author keywords

[No Author keywords available]

Indexed keywords

ACID SITE; ACTIVE SITE; ADSORPTION PROPERTIES; ALUMINUM FILM; ATOMIC RATIO; ELECTRON DONORS; ELECTRON-ACCEPTING; EXPERIMENTAL SPECTRA; GASEOUS NITROGEN; INNER SURFACES; LEWIS ACID SITE; LEWIS ACIDITY; LEWIS SITES; MESO-PORES; MESOPORE WALLS; NMR TECHNIQUES; NUMERICAL VALUES; PENTACOORDINATED; ROOM TEMPERATURE; SI/AL RATIO; SILANOL GROUPS; SILICA SURFACE; SURFACE DENSITY; VARIABLE TEMPERATURE;

ADSORPTION; MESOPOROUS MATERIALS; NITROGEN; PYRIDINE; SILICA; SURFACES;

ALUMINUM;

ACID; NITROGEN; PYRIDINE; PYRIDINE DERIVATIVE; SBA 15; SBA-15; SILICON DIOXIDE;

ADSORPTION; ARTICLE; CHEMICAL STRUCTURE; CHEMISTRY; NUCLEAR MAGNETIC RESONANCE SPECTROSCOPY; PH; SURFACE PROPERTY; TEMPERATURE;

ACIDS; ADSORPTION; HYDROGEN-ION CONCENTRATION; MAGNETIC RESONANCE SPECTROSCOPY; MOLECULAR STRUCTURE; NITROGEN ISOTOPES; PYRIDINES; SILICON DIOXIDE; SURFACE PROPERTIES; TEMPERATURE;

EID: 80053305631     PISSN: 07437463     EISSN: 15205827     Source Type: Journal    
DOI: 10.1021/la2017566     Document Type: Article

References (47)

1. Morell, J.; Chatterjee, S.; Klar, P. J.; Mauder, D.; Shenderovich, I.; Hoffmann, F.; Froba, M. Chem.-Eur. J. 2008, 14, 5935-5940
2. Taguchi, A.; Schüth, F. Microporous Mesoporous Mater. 2004, 77, 1-45
3. Øye, G.; Sjöblom, J.; Stöcker, M. Adv. Synth. Catal. 2001, 89-90, 439-466
4. Parida, S. K.; Dash, S.; Patel, S.; Mishra, B. K. Adv. Colloid Interface Sci. 2006, 121, 77-110
5. Corma, A.; Garcia, H. Adv. Synth. Catal. 2006, 348, 1391-1412
6. Martín-Aranda, R. M.; Čejka, J. Top. Catal. 2010, 53, 141-153
7. Akcakayiran, D.; Mauder, D.; Hess, C.; Sievers, T. K.; Kurth, D. G.; Shenderovich, I. G.; Limbach, H.-H.; Findenegg, G. H. J. Phys. Chem. B 2008, 112, 14637-14647
8. Mauder, D.; Akcakayiran, D.; Lesnichin, S. B.; Findenegg, G. H.; Shenderovich, I. G. J. Phys. Chem. C 2009, 113, 19185-19192
9. Brunel, D.; Blanc, A. C.; Galarneau, A.; Fajula, F. Catal. Today 2002, 73, 139-152
10. Trombetta, M.; Busca, G.; Lenarda, M.; Storaro, L.; Pavan, M. Appl. Catal., A 1999, 182, 225-235
11. Hunger, M.; Schenk, U.; Breuninger, M.; Gläser, R.; Weitkamp, J. Microporous Mesoporous Mater. 1999, 27, 261-271
12. Dědeček, J.; Žilková, N.; Čejka, J. Microporous Mesoporous Mater. 2001, 44-45, 259-266
13. Xu, M.; Wang, W.; Seiler, M.; Buchholz, A.; Hunger, M. J. Phys. Chem. B 2002, 106, 3202-3208
14. Luo, Q.; Deng, F.; Yuan, Z.; Yang, J.; Zhang, M.; Yue, Y.; Ye, C. J. Phys. Chem. B 2003, 107, 2435-2442
15. Hu, W.; Luo, Q.; Su, Y.; Chen, L.; Yue, Y.; Ye, C.; Deng, F. Microporous Mesoporous Mater. 2006, 92, 22-30
16. Wang, Y.; Lang, N.; Tuel, A. Microporous Mesoporous Mater. 2006, 93, 46-54
17. Góra-Marek, K.; Derewiński, M.; Sarv, P.; Datka, J. Catal. Today 2005, 101, 131-138
18. Ip, B. C. K.; Andreeva, D. V.; Buntkowsky, G.; Akcakayiran, D.; Findenegg, G. H.; Shenderovich, I. G. Microporous Mesoporous Mater. 2010, 134, 22-28
19. Mokaya, R. Chem. Commun. 2000, 1891-1892
20. Zukal, A.; Mayerová, J.; Čejka, J. Phys. Chem. Chem. Phys. 2010, 12, 5240-5247
21. Zukal, A.; Šiklová, H.; Čejka, J. Langmuir 2008, 24, 9837-9842
22. Shenderovich, I. G.; Mauder, D.; Akcakayiran, D.; Buntkowsky, G.; Limbach, H.-H.; Findenegg, G. H. J. Phys. Chem. B 2007, 111, 12088-12096
23. Lorente, P.; Shenderovich, I. G.; Golubev, N. S.; Denisov, G. S.; Buntkowsky, G.; Limbach, H.-H. Magn. Reson. Chem. 2001, 39, S18-S29
24. Shenderovich, I. G.; Buntkowsky, G.; Schreiber, A.; Gedat, E.; Sharif, S.; Albrecht, J.; Golubev, N. S.; Findenegg, G. H.; Limbach, H.-H. J. Phys. Chem. B 2003, 107, 11924-11939
25. Lesnichin, S. B.; Kamdem, N.; Mauder, D.; Denisov, G. S.; Shenderovich, I. G. Russ. J. Gen. Chem. 2010, 80, 2027-2031
26. Ripmeester, J. A. J. Am. Chem. Soc. 1983, 105, 2925-2927
27. Maciel, G. E.; Haw, J. F.; Chuang, I.-S.; Hawkins, B. L.; Early, T. A.; McKay, D. R.; Petrakis, L. J. Am. Chem. Soc. 1983, 105, 5529-5535
28. Haw, J. F.; Chuang, I.-S.; Hawkins, B. L.; Maciel, G. E. J. Am. Chem. Soc. 1983, 105, 7206-7207
29. Anwander, R.; Nagl, I.; Widenmeyer, M.; Engelhardt, G.; Groeger, O.; Palm, C.; Röser, Th. J. Phys. Chem. B 2000, 104, 3532-3544
30. Emeis, C. A. J. Catal. 1993, 141, 347-354
31. Andreeva, D. V.; Ip, B.; Gurinov, A.; Tolstoy, P. M.; Shenderovich, I. G.; Limbach, H.-H. J. Phys. Chem. A 2006, 110, 10872-10879
32. Sharif, S.; Shenderovich, I. G.; Gonzalez, L.; Denisov, G. S.; Silverman, D. N.; Limbach, H.-H. J. Phys. Chem. A 2007, 111, 6084-6093
33. Gruenberg, B.; Emmler, Th.; Gedat, E.; Shenderovich, I. G.; Findenegg, G. H.; Limbach, H.-H.; Buntkowsky, G. Chem.-Eur. J. 2004, 10, 5689-5696
34. Limbach, H. H.; Tolstoy, P. M.; Perez-Hernandez, N.; Guo, J.; Shenderovich, I. G.; Denisov, G. S. Isr. J. Chem. 2009, 49, 199-216
35. Pizzanelli, S.; Kababya, S.; Frydman, V.; Landau, M.; Vega, S. J. Phys. Chem. B 2005, 109, 8029-8039
36. Hunger, M.; Freude, D.; Pfeifer, H. J. Chem. Soc., Faraday Trans. 1991, 87, 657-662
37. Hunger, M. Solid State Nucl. Magn. Reson. 1996, 6, 1-29
38. Wakabayashi, F.; Kondo, J.; Wada, A.; Domen, K.; Hirose, C. J. Phys. Chem. 1993, 97, 10761-10768
39. Gallo, J. M. R.; Bisio, C.; Gatti, G.; Marchese, L.; Pastore, H. O. Langmuir 2010, 26, 5791-5800
40. Handjani, S.; Dzwigaj, S.; Blanchard, J.; Marceau, E.; Kraft, J.-M.; Che, M. Top. Catal. 2009, 52, 334-343
41. Dragoi, B.; Dumitriu, E.; Guimon, C.; Auroux, A. Microporous Mesoporous Mater. 2009, 121, 7-17
42. Gomez-Cazalilla, M.; Merida-Robles, J. M.; Gurbani, A.; Rodriguez-Castellon, E.; Jimenez-Lopez, A. J. Solid State Chem. 2007, 180, 1130-1140
43. Oumi, Y.; Takagi, H.; Sumiya, S.; Mizuno, R.; Uozumi, T.; Sano, T. Microporous Mesoporous Mater. 2001, 44-45, 267-274
44. Sumiya, S.; Oumi, Y.; Uozumi, T.; Sano, T. J. Mater. Chem. 2001, 11, 1111-1115
45. Gedeon, A.; Lassoued, A.; Bonardet, J. L.; Fraissard, J. Microporous Mesoporous Mater. 2001, 44-45, 801-806
46. Marthala, V. R. R.; Rabl, S.; Huang, J.; Rezai, S. A. S.; Thomas, B.; Hunger, M. J. Catal. 2008, 257, 134-141
47. Marthala, V. R. R.; Frey, J.; Hunger, M. Catal. Lett. 2010, 135, 91-97