Improved working model for interpreting the excitation wavelength- and fluence-dependent response in pulsed laser-induced size reduction of aqueous gold nanoparticles

Journal of Physical Chemistry C

Volumn 115, Issue 12, 2011, Pages 5063-5072

  Werner, Daniel ^a   Hashimoto, Shuichi ^a  

^a UNIVERSITY OF TOKUSHIMA   (Japan)

Author keywords

[No Author keywords available]

Indexed keywords

ABSORPTION CROSS SECTIONS; AQUEOUS SOLUTIONS; BOILING TEMPERATURE; COULOMB EXPLOSION; ELECTRON PHONON; ENERGY DEPOSITIONS; EVAPORATION MODEL; EXCITATION WAVELENGTH; FEMTO-SECOND LASER; FLUENCES; FRAGMENTATION EFFICIENCY; GOLD NANOPARTICLES; GOLD PARTICLES; LASER ENERGIES; LASER FLUENCES; LASER INDUCED; LASER INTENSITIES; LATTICE TEMPERATURES; MECHANISTIC ASPECTS; NANOSECOND LASER EXCITATION; NANOSECOND LASER PULSE; NON EQUILIBRIUM; NUMERICAL SIMULATION; OPTICAL EFFECTS; PHOTO-THERMAL; PHOTOTHERMAL MELTING; PICOSECOND LASER; QUASI-EQUILIBRIUM; SIZE REDUCTIONS; SPECTRAL REGION; STRIKING EFFECTS; SURFACE PLASMONS; TEMPERATURE RISE; TIME EVOLUTIONS; TWO-TEMPERATURE MODELS; WORKING MODELS;

BOILING POINT; COMPUTER SIMULATION; DIELECTRIC DEVICES; ELECTRON TEMPERATURE; EXPLOSIONS; EXPLOSIVES; GOLD; GOLD DEPOSITS; LASER EXCITATION; MELTING; METAL DRAWING; NANOPARTICLES; PHONONS; SIZE DETERMINATION; SURFACE PLASMON RESONANCE; ULTRAFAST LASERS;

PULSED LASERS;

EID: 79953033220     PISSN: 19327447     EISSN: 19327455     Source Type: Journal    
DOI: 10.1021/jp109255g     Document Type: Article

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51. -2) occur.
52. We assumed various heat capacities of gold NPs dependent on the excitation wavelength (ref 15). The heat capacity can be reduced by 40% on excitation of the interband transition from 5d to 6sp compared to that observed for excitation of the intraband excitation within 6sp.