Carbonaceous aerosol characteristics over a Pinus taeda plantation: Results from the CELTIC experiment

Atmospheric Environment

Volumn 45, Issue 3, 2011, Pages 794-801

  Geron, Chris ^a  

^a U S ENVIRONMENTAL PROTECTION AGENCY   (United States)

Author keywords

Biogenic volatile organic compounds; CELTIC elemental carbon; Organic carbon; Ozone; PM2.5; Radiocarbon

Indexed keywords

AERODYNAMIC DIAMETERS; AMBIENT AEROSOLS; BIOGENIC VOCS; BIOGENIC VOLATILE ORGANIC COMPOUNDS; BIOMASS-BURNING; BOX MODELS; CARBON SOURCE; CARBONACEOUS AEROSOL; CARBONACEOUS PARTICLES; CARYOPHYLLENE; CELTIC ELEMENTAL CARBON; CHEMICAL EMISSIONS; EMISSION FACTORS; FIELD STUDIES; FLORIDA; FOSSIL CARBON; HUMID PERIODS; LEVOGLUCOSAN; LOBLOLLY PINE PLANTATIONS; LOWER LIMITS; MAXIMUM TEMPERATURE; MODEL ESTIMATES; OC/EC RATIO; PINE CANOPIES; PINIC ACID; PINUS TAEDA; PM2.5; PRECIPITATION EVENTS; RADIOCARBON; RADIOCARBON ANALYSIS; REGRESSION RELATIONSHIP; RELATIVE CONTRIBUTION; RURAL SITE; SECONDARY ORGANIC AEROSOLS; SUBURBAN SITES; TEMPORAL PATTERN; TENNESSEE;

ATMOSPHERIC AEROSOLS; ATMOSPHERIC COMPOSITION; BIOMASS; ESTIMATION; FORESTRY; OXIDATION; OZONE; POTASSIUM; VOLATILE ORGANIC COMPOUNDS;

ORGANIC CARBON;

CARBON; CARBON DIOXIDE; CARYOPHYLLENE; ISOPRENE; LEVOGLUCOSAN; ORGANIC CARBON; PINENE; POTASSIUM; VOLATILE ORGANIC COMPOUND;

AERODYNAMICS; AEROSOL COMPOSITION; AEROSOL PROPERTY; ATMOSPHERIC MODELING; BIOGENIC EMISSION; BIOMASS BURNING; CARBON DIOXIDE; CONIFEROUS FOREST; DATA SET; EXPERIMENTAL STUDY; FOREST CANOPY; FOSSIL FUEL; NUMERICAL MODEL; ORGANIC CARBON; OXIDATION; PARTICLE SIZE; PLANTATION FORESTRY; REGRESSION ANALYSIS; RURAL AREA; SAMPLER; TEMPORAL ANALYSIS; VOLATILE ORGANIC COMPOUND;

AEROSOL; ARTICLE; BIOMASS; CANOPY; CARBON SOURCE; FOREST; HUMAN; LOBLOLLY PINE; NONHUMAN; PARTICULATE MATTER; PLANTATION; PRECIPITATION; PRIORITY JOURNAL;

AEROSOLS; BIOMASS; CARBON; FORESTRY; OXIDATION; OZONE; POTASSIUM; VOC;

DUKE FOREST; NORTH CAROLINA; UNITED STATES;

PINUS TAEDA;

EID: 78751585048     PISSN: 13522310     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.atmosenv.2010.07.015     Document Type: Article

References (47)

1. Andreae M.O., Merlet P. Emission of trace gases and aerosols from biomass burning. Global Biogeochemical Cycles 2001, 15(4):955-966.
2. 2.5 aerosols at nine Interagency Monitoring for Protection of Visual Environments (IMPROVE) network sites. Journal of Geophysical Research 2007, 112. 10.1029/2006JD007708.
3. Bhat S., Fraser M.P. Primary source attribution and analysis of a-pinene photooxidation products in Duke Forest, North Carolina. Atmospheric Environment 2007, 41:2958-2966.
4. Birch M.E., Cary R.A. Elemental carbon-based method for monitoring occupational exposures to particulate diesel exhaust. Aerosol Science and Technology 1996, 25:221-241.
5. Claeys M., et al. Formation of secondary organic aerosols through photooxidation of isoprene. Science 2004, 303:1173-1176.
6. Czoschke N.M., Jang M. Acidity effects on the formation of α-pinene ozone SOA in the presence of inorganic seed. Atmospheric Environment 2006, 40:4370-4380.
7. Duhl T.R., Helmig D., Guenther A. Sesquiterpene emissions from vegetation: a review. Biogeosciences 2008, 5:761-777.
8. Gallagher M.W., et al. Measurements of aerosol fluxes to speulder forest using a micrometeorological technique. Atmospheric Environment 1997, 31:359-373.
9. Gelencser A., May B., Simpson D., Sanchez-Ochoa A., Kasper-Giebl A., Puxbaum H., Caseiro A., Pio C., Legrand M. Source apportionment of PM2.5 organic aerosol over Europe: primary/secondary, natural/anthropogenic, and fossil/biogenic origin. Journal of Geophysical Research-Atmospheres 2007, 112:D23S04. 10.1029/2006JD008094.
10. Geron C. Carbonaceous aerosol over a Pinus taeda forest in Central North Carolina, USA. Atmospheric Environment 2009, 43:959-969.
11. Geron C., Guenther A., Greenberg J., Karl T., Rasmussen R. Biogenic volatile organic compound emissions from desert vegetation of the southwestern US. Atmospheric Environment 2006, 40:1645-1660.
12. Geron C., Guenther A., Pierce T. An improved model for estimating emissions of volatile organic compounds from forests in the eastern United States. Journal of Geophysical Research 1994, 99:12,773-712,791.
13. Griffin R.J., Cocker D.R., Flagan R.C., Seinfeld J.H. Organic aerosol formation from the oxidation of biogenic hydrocarbons. Journal of Geophysical Research 1999, 104:3555-3567.
14. Guenther A., et al. Estimates of global terrestrial isoprene emissions using MEGAN (Model of Emissions ofGases and Aerosols from Nature). Atmospheric Chemistry and Physics 2006, 6:3181-3210.
15. Guenther A., Zimmerman P., et al. Estimates of regional natural volatile organic compound fluxes from enclosure and ambient measurements. Journal of Geophysical Research 1996, 101(D1):1345-1359.
16. Guenther A., Zimmerman P.R., Harley P. Isoprene and monoterpene emission rate variability: model evaluations and sensitivity analyses. Journal of Geophysical Research 1993, 98:12,609-612,617.
17. Guenther A., Zimmerman P.R., Wildermuth M. Natural volatile organic compound emission rate estimates for U.S. woodland landscapes. Atmospheric Environment 1994, 28:1197-1210.
18. Helmig D., Ortega J., Guenther A., Herrick J.D., Geron C. Sesquiterpene emissions from loblolly pine and their potential contribution to biogenic aerosol formation in the Southeastern US. Atmospheric Environment 2006, 40:4150-4157.
19. 2. Global Change Biology 1999, 5:293-309.
20. Jaffe D., Tamura S., Harris J. Seasonal cycle and composition of background fine particles along the west coast of the US. Atmospheric Environment 2005, 39:297-306.
21. Jonsson A.M., Hallquist M., Ljungstrom E. Impact of humidity on the ozone initiated oxidation of limonene, Δ3-Carene, and α-Pinene. Environmental Science and Technology 2006, 40:188-194.
22. Juang J.-Y., et al. Eco-hydrological controls on triggers of summertime convective rainfall. Global Change Biology 2007, 13:1-10.
23. 2. Environmental Science and Technology 2006, 40:3807-3812.
24. Kleindienst T.E., et al. Estimates of the contributions of biogenic and anthropogenic hydrocarbons to secondary organic aerosol at a southeastern US location. Atmospheric Environment 2007, 41:8288-8300.
25. 13C ratios. Journal of Geophysical Research 2002, 107:1-7.
26. 2 level in mid-latitudes of the northern hemisphere (1959-2003). Radiocarbon 2004, 46:1261-1272.
27. 2.5 ambient aerosol in Nashville TN. Atmospheric Environment 2004, 38:6053-6061.
28. 2.5 ambient aerosol in Tampa, FL. Aerosol Science and Technology 2006, 40:189-196.
29. Lim H.J., Turpin B.J. Origins of primary and secondary organic aerosol in Atlanta: results of time-resolved measurements during the Atlanta supersite experiment. Environmental Science and Technology 2002, 36(21):4489-4496.
30. Loescher H.W., et al. Characterization and dry deposition of carbonaceous aerosols in a wet tropical forest canopy. Journal of Geophysical Research 2004, 109.
31. Malm W.C., Schichtel B.A., et al. Spatial and monthly trends in speciated fine particle concentration in the United States. Journal of Geophysical Research 2004, 109(D3).
32. Mebust M.R., Eder B.K., Binkowski F.S., Roselle S.J. Models-3 Community Multiscale Air Quality (CMAQ) model aerosol component 2. Model evaluation. Journal of Geophysical Research 2003, 108:1-18. AAC 4.
33. Samet J.M., Dominici F., et al. Fine particulate air pollution and mortality in 20 U.S. cities, 1987-1994. The New England Journal of Medicine 2000, 343(24):1742-1749.
34. Schade G.W., Goldstein A.W., Lamanna M.S. Are monoterpene emissions influenced by humidity?. Geophysical Research Letters 1999, 26:2187-2190.
35. Schichtel B.A., et al. Fossil and contemporary fine particulate carbon fractions at 12 rural and urban sites in the United States. Journal of Geophysical Research 2008, 113. 10.1029/2007JD008605.
36. 2 enrichment. Global Change Biology 2008, 14:1-14.
37. Stroud C., et al. Cloud activating properties of aerosol observed during CELTIC. Journal of Aerosol Science 2007, 64:441-459.
38. Stuiver M. International agreements and the use of the new oxalic acid standard. Radiocarbon 1983, 25:793-795.
39. Subramanian R., Khlystov A., Cabada J., Robinson A. Positive and negative artifacts in particulate organic carbon measurements with denuded and undenuded sampler configurations. Aerosol Science & Technology 2004, 38:27-48.
40. Surratt J.D., et al. Evidence for organosulfates in secondary organic aerosol. Environmental Science and Technology 2007, 41:517-527.
41. Szidat S., Ruff M., Perron N., Wacker L., Synal H.A., Hallquist M., Shannigrahi A.S., Yttri K.E., Dye C., Simpson D. Fossil and non-fossil sources of organic carbon (OC) and elemental carbon (EC) in Goteborg, Sweden. Atmospheric Chemistry and Physics 2009, 9:1521-1535.
42. Szidat S., Jenk T.M., Gaggeler H.W., Synal H.A., Fisseha R., Baltensperger U., Kalberer M., Samburova V., Reimann S., Kasper-Giebl A., Hajdas I. Radiocarbon (C-14)-deduced biogenic and anthropogenic contributions to organic carbon (OC) of urban aerosols from Zurich, Switzerland. Atmospheric Environment 2004, 38:4035-4044.
43. Takahashi K., Hirabayashi M., Tanabe K., Shibata Y., Nishikawa M., Sakamoto K. Radiocarbon content in urban atmospheric aerosols. Water Air and Soil Pollution 2007, 185:305-310.
44. Turnipseed A.A., Huey L.G., Nemitz E., Stickel R., Higgs J., Tanner D.J., Slusher D.L., Sparks J.P., Flocke F., Guenther A. Eddy covariance fluxes of peroxyacetyl nitrates (PANs) and NOy to a coniferous forest. Journal of Geophysics Research 2006, 111:D09304. 10.1029/2005JD006631.
45. Turpin B.J., Saxena P., et al. Measuring and simulating particulate organics in the atmosphere: problems and prospects. Atmospheric Environment 2000, 34(18):2983-3013.
46. 2.5 mass concentrations:revisiting common assumptions for estimating organic mass. Aerosol Science and Technology 2001, 35:602-610.
47. Yu S., Bhave P.V., Dennis R.L., Mathur R. Seasonal and regional variations of primary and secondary organic aerosols over the continental United States: semi-empirical estimates and model evaluation. Environmental Science and Technology 2007, 41:4690-4697.