Fraction of organic carbon predicts labile desorption rates of chlorinated organic pollutants in laboratory-spiked geosorbents

Environmental Toxicology and Chemistry

Volumn 29, Issue 5, 2010, Pages 1049-1055

  Ginsbach, Jake W ^a   Killops, Kato L ^a   Olsen, Robert M ^a   Peterson, Brittney ^a   Dunnivant, Frank M ^a  

^a WHITMAN COLLEGE   (United States)

Author keywords

Chlorinated organic pollutants; Desorption kinetics; Dredging; Organic carbon; Resuspension events

Indexed keywords

DESORPTION; ENVIRONMENTAL IMPACT; ORGANIC CARBON; RATE CONSTANTS;

DESORPTION KINETICS; DESORPTION MEASUREMENTS; DESORPTION RATE; DESORPTION RATE CONSTANTS; DIFFUSION MODEL; EMPIRICAL MODEL; ENVIRONMENTAL QUALITY; EXPERIMENTAL EVIDENCE; GEOSORBENTS; HUMAN HEALTH; KINETIC MODELS; KINETICS EXPERIMENTS; MESOPORE; ORGANIC MATERIALS; ORGANIC MATTER; PREDICTIVE MODELS; RE-SUSPENSION; RELEASE RATE; RESUSPENSION EVENTS; SITE-SPECIFIC; THEORETICAL MODELS;

ORGANIC POLLUTANTS;

ORGANIC CARBON; ORGANIC MATTER; CARBON; DIELDRIN; SOIL; WATER POLLUTANT;

CHLORINATED HYDROCARBON; DESORPTION; DREDGING; EMPIRICAL ANALYSIS; ENVIRONMENTAL IMPACT; ENVIRONMENTAL MODELING; ORGANIC CARBON; ORGANIC POLLUTANT; REACTION KINETICS; RESUSPENSION; SEDIMENT POLLUTION; SUSPENDED SEDIMENT;

ARTICLE; CORRELATION ANALYSIS; DIFFUSION; EXPERIMENTAL MODEL; KINETICS; PRIORITY JOURNAL; THEORETICAL MODEL; ADSORPTION; BIOLOGICAL MODEL; CHEMISTRY; SEDIMENT; SOIL; TIME; WATER POLLUTANT;

ADSORPTION; CARBON; DIELDRIN; GEOLOGIC SEDIMENTS; MODELS, BIOLOGICAL; SOIL; TIME FACTORS; WATER POLLUTANTS, CHEMICAL;

EID: 77953567580     PISSN: 07307268     EISSN: 15528618     Source Type: Journal    
DOI: 10.1002/etc.138     Document Type: Article

References (34)

1. Choi AL, Levy JI, Dockery DW, Ryan LM, Tolbert PE, Altshul LM, Korrick SA. 2006. Does living near a superfund site contribute to higher polychlorinated biphenyl (PCB) exposure? Environ Health Perspect 114:1092-1098.
2. Hornbuckle KC,AchmanDR,EisenreichSJ.1993.Over-waterand overland polychlorinated-biphenyls in Green Bay, Lake-Michigan. Environ Sci Technol 27:87-98.
3. Vorhees DJ, Cullen AC, Altshul LM. 1999. Polychlorinated biphenyls in house dust and yard soil near a Superfund site. Environ Sci Technol 33:2151-2156.
4. Otto DME, Buttner JK, Arquette DM, Moon TW. 1996. Impaired inducibility of xenobiotic and antioxidant responses in rainbow trout exposed to polychlorinated biphenyl contaminated sediments in the St Lawrence River. Chemosphere 33:2021-2032.
5. Cheng C, Atkinson J, Depinto J. 1995. Desorption during resuspension events-kinetic v equilibrium-model. Mar Freshw Res 46: 251-256.
6. Birdwell JE, Thibodeaux LJ. 2007. A kinetic model of short-term dissolved contaminant release during dredge-generated bed sediment resuspension. Environ Eng Sci 24:1431-1442.
7. Huang WL, Young TM, Schlautman MA, Yu H, Weber WJ. 1997. A distributed reactivity model for sorption by soils and sediments. General isotherm nonlinearity and applicability of the dual reactive domain model. Environ Sci Technol 31:1703-1710.
8. CornelissenG,HaftkaJ,ParsonsJ,GustafssonO.2005.Sorptiontoblack carbon of organic compounds with varying polarity and planarity. Environ Sci Technol 39:3688-3694.
9. Abu A, Smith S. 2006. Mechanistic characterization of adsorption and slow desorption of phenanthrene aged in soils. Environ Sci Technol 40:5409-5414.
10. Braida WJ, Pignatello JJ,LuYF, Ravikovitch PI,Neimark AV, Xing BS. 2003. Sorption hysteresis of benzene in charcoal particles. Environ Sci Technol 37:409-417.
11. Ran Y, Xing BS, Rao PSC, Fu JM. 2004. Importance of adsorption (hole-filling) mechanism for hydrophobic organic contaminants on an aquifer kerogen isolate. Environ Sci Technol 38:4340-4348.
12. Johnson MD, Keinath TM, Weber WJ. 2001. A distributed reactivity model for sorption by sails and sediments. Characterization and modeling of phenanthrene desorption rates. Environ Sci Technol 35: 1688-1695.
13. Birdwell JE, Cook RL, Thibodeaux LJ. 2007. Desorption kinetics of hydrophobicorganic chemicals fromsedimenttowater:Areviewofdata and models. Environ Toxicol Chem 26:424-434.
14. Chai YZ, Kochetkov A, Reible DD. 2006. Desorption resistance of polycyclic aromatic hydrocarbons and duration of exposure. Environ Toxicol Chem 25:2827-2833.
15. Kukkonen JVK, Landrum PF, Mitra S, Gossiaux DC, Gunnarsson J, Weston D. 2003. Sediment characteristics affecting desorption kinetics of select PAHand PCBcongenersfor seven laboratoryspiked sediments. Environ Sci Technol 37:4656-4663.
16. Shor LM, Rockne KJ, Taghon GL, Young LY, Kosson DS. 2003. Desorption kinetics for field-aged polycyclic aromatic hydrocarbons from sediments. Environ Sci Technol 37:1535-1544.
17. Chai YZ, Kochetkov A, Reible DD. 2006. Modeling biphasic sorption and desorption of hydrophobic organic contaminants in sediments. Environ Toxicol Chem 25:3133-3140.
18. WalkleyA,BlackAI.1934.AnexaminationoftheDegtjareff methodfor determining soil organic matter, and a proposed modification of the chromic acid titration method. Soil Sci 37:29-38.
19. RockneKJ, TaghonGL,Kosson DS.2000.Porestructureofsootdeposits from several combustion sources. Chemosphere 41:1125-1135.
20. Cornelissen G, vanNoort PCM, Govers HAJ. 1997. Desorption kinetics of chlorobenzenes, polycyclic aromatic hydrocarbons, and polychlori-nated biphenyls: Sediment extraction with Tenax® and effects of contact time and solute hydrophobicity. Environ Toxicol Chem 16: 1351-1357.
21. Saalfield SL, Wnuk JD, Murray MM, Dunnivant FM. 2007. A comparison of two techniques for studying sediment desorption kinetics of hydrophobic pollutants. Chemosphere 66:384-389.
22. Cornelissen G, VanNoort PCM, Parsons JR, Govers HAJ. 1997. Temperature dependence of slow adsorption and desorption kinetics of organic compounds in sediments. Environ Sci Technol 31:454-460.
23. Kan AT, Fu G, Hunter M, Chen W, Ward CH, Tomson MB. 1998. Irreversible sorptionofneutralhydrocarbonstosediments: Experimental observations and model predictions. Environ Sci Technol 32:892-902.
24. Johnson MD, Huang WH, Weber WJ. 2001. A distributed reactivity model for sorption by soils and sediments. Simulated diagenesis of natural sediment organic matter and its impact on sorptionfdesorption equilibria. Environ Sci Technol 35:1680-1687.
25. Karickhoff SW, Brown D, Scott TA. 1979. Sorption of hydrophobic pollutants on natural sediments. Water Res 13:241-248.
26. Zhao DY, Pignatello JJ. 2004. Model-aided characterizationofTenax®-TA for aromatic compound uptake from water. Environ Toxicol Chem 23: 1592-1599.
27. U.S. Environmental Protection Agency. 1996. Soil screening guidance: Technical background document Appendix K. Soil organic carbon (KOC)fwater (KOW) partition coefficients. EPAf540fR95f128. Technical Background. Washington, DC.
28. Steinberg SM, Pignatello JJ, Sawhney BL. 1987. Persistence of 1,2-dibromoethane in soils-entrapment in intraparticle micropores. Environ Sci Technol 21:1201-1208.
29. Holmen BA, Gschwend PM. 1997. Estimating sorption rates of hydrophobic organic compounds in iron oxide and aluminosilicate clay-coated aquifer sands. Environ Sci Technol 31:105-113.
30. Ghosh U, Gillette JS, Luthy RG, Zare RN. 2000. Microscale location, characterization, and association of polycyclic aromatic hydrocarbons on harbor sediment particles. Environ Sci Technol 34:1729-1736.
31. Weber WJ, Kim SH, Johnson MD. 2002. Distributed reactivity modelfor sorption by soils and sediments. High-concentration co-contaminant effects on phenanthrene sorption and desorption. Environ Sci Technol 36:3625-3634.
32. Neogi P. 1996. Diffusion in Polymers. CRC, New York, NY, USA.
33. Tchobanoglous G, Burton F, Eddy M. 1991. Wastewater Engineering: Treatment, Disposal, Reuse, 3rd ed. McGraw-Hill, New York,NY, USA.
34. Ehlers GAC, Loibner AP. 2006. Linking organic pollutant (bio)avail-ability with geosorbent properties and biomimetic methodology: A review of geosorbent characterisation and (bio)availability prediction. Environ Pollut 141:494-512.