Uranyl adsorption onto hydrous ferric oxides - A re-evaluation for the diffuse layer model database

Environmental Science and Technology

Volumn 43, Issue 24, 2009, Pages 9260-9266

  Mahoney, John J ^a   Cadle, Sonya A ^b   Jakubowski, Andryan T ^c  

^a Mahoney Geochemical Consulting LLC   (United States)

^b GeoTrans Inc   (United States)

^c MWH AMERICAS INC   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

BEARING SURFACES; BEST FIT; COMPUTER CODES; DATA SETS; DICARBONATE; DIFFUSE-LAYER MODELS; EXPERIMENTAL DATA; HYDROUS FERRIC OXIDES; LINEAR FREE ENERGY RELATIONSHIPS; RE-EVALUATION; SURFACE COMPLEX; SURFACE COMPLEXATION;

ADSORPTION; COMPLEXATION; DATABASE SYSTEMS; DISSOLUTION; HAFNIUM COMPOUNDS; IRON OXIDES; LAGRANGE MULTIPLIERS; URANIUM; URANIUM ALLOYS; URANIUM COMPOUNDS;

SURFACE REACTIONS;

BICARBONATE; FERRIC OXIDE; UNCLASSIFIED DRUG; URANIUM DERIVATIVE; URANYL BICARBONATE; URANYL DERIVATIVE;

ADSORPTION; COMPLEXATION; DATABASE; DIFFUSION; DISSOLVED MATTER; IRON OXIDE; REACTION KINETICS; URANIUM;

ADSORPTION; ARTICLE; COMPUTER PROGRAM; CONTROLLED STUDY; DATA BASE; DIFFUSION; DISSOLUTION; ENERGY; GEOCHEMICAL ANALYSIS; MODEL; RADIATION ABSORPTION; RADIATION MEASUREMENT; SURFACE PROPERTY;

ADSORPTION; DATABASES, FACTUAL; FERRIC COMPOUNDS; MINING; MODELS, CHEMICAL; THERMODYNAMICS; URANIUM; WATER POLLUTANTS, RADIOACTIVE;

EID: 72849119056     PISSN: 0013936X     EISSN: 15205851     Source Type: Journal    
DOI: 10.1021/es901586w     Document Type: Article

References (21)

1. Langmuir, D. Aqueous Environmental Geochemistry; Prentice Hall: Upper Saddle River, NJ, 1997.
2. Hsi, C. K. D. Sorption of uranium (VI) by iron oxides. Ph.D. Dissertation, Colorado School of Mines, Golden, CO, 1981.
3. Hsi, C. K. D.; Langmuir, D. Adsorption of uranyl onto ferric oxyhydroxides: applications of a surface complexation site binding model. Geochim. Cosmochim. Acta 1985, 49, 2423-2432.
4. Payne, T. E.; Lumkin, G. R.; Waite, T. D. UraniumVI adsorption on model minerals. In Adsorption of Metals by Geomedia; Jenne, E. A., Ed.; Academic Press: New York, 1998; pp 75-97.
5. Payne, T. E. Uranium (VI) interactions with mineral surfaces: controlling factors and surface complexation modeling. Ph.D. Dissertation, University of New South Wales, Sydney, NSW, 1999.
6. Waite, T. D.; Davis, J. A.; Payne, T. E.; Waychunas, G. A.; Xu, N. Uranium(VI) adsorption to ferrihydrite: Application of a surface complexation model. Geochim. Cosmochim. Acta 1994, 57, 2251-2269.
7. Wazne, M.; Korfiatis, G. P.; Meng, X. Carbonate effects on hexavalent uranium adsorption by iron oxyhydroxide. Environ. Sci. Technol. 2003, 37, 3619-3624. (Pubitemid 36999306)
8. Morrison, S. J.; Spangler, R. R.; Tripathi, V. S. Adsorption of uranium(VI) on amorphous ferric oxyhydroxide at high concentrations of dissolved carbonate(IV) and sulfur(VI). J. Contam. Hydrol. 1995, 17, 333-346.
9. Fox, P. M.; Davis, J. A.; Zachara, J. M. The effect of calcium on aqueous uranium(VI) speciation and adsorption to ferrihydrite and quartz. Geochim. Cosmochim. Acta 2006, 70, 1379-1387. (Pubitemid 43316664)
10. Dzombak, D. A.; Morel, F. M. M. Surface Complexation ModelingsHydrous Ferric Oxide; John Wiley and Sons: New York, 1990.
11. Parkhurst, D. L.; Appelo, C. A. J. User's Guide to PHREEQC (Version 2)sAComputer Program for Speciation, Batch-Reaction, One-Dimensional Transport, and Inverse Geochemical Calculations; Water Resources Investigation Report 99-4259; USGS: Denver, CO, 1999.
12. Allison, J. D.; Brown, D. S.; Novo-Gradac, K. J. MINTEQA2/ PRODEFA2, A Geochemical Assessment Model for Environmental Systems, Version 3.0 User's Manual; EPA/600/3-91/021; U.S. EPA: Athens, GA, 1991.
13. Bethke, C.M.Geochemical Reaction Modeling; Oxford University Press: New York, 1996.
14. Baes, C. F., Jr.; Mesmer, R. E. The Hydrolysis of Cations; Wiley Interscience: New York, 1976.
15. Guillaumont, R.; Fanghähel, T.; Neck, V.; Fuger, J.; Palmer, D.; Grenthe, I.; Rand, M. H. Update on the Chemical Thermodynamics of Uranium, Neptunium, Plutonium, Americium and Technetium; Elsevier B.V.: Amsterdam, 2003.
16. Westall, J.; Hohl, H. Comparison of models for the oxide-solution interface. Adv. Colloid Interface Sci. 1980, 12, 265-294.
17. Appelo, C. A. J.; Van der Weiden, M. J. J.; Tournassat, C.; Charlet, L. Surface complexation of ferrous iron and carbonate on ferrihydrite and the mobilization of arsenic. Environ. Sci. Technol. 2002, 36, 3096-3103. (Pubitemid 34777682)
18. Poeter, E. P.; Hill, M. C.; Banta, E. R.; Mehl, S.; Christensen, S. UCODE-2005 and Six Other Computer Codes for Universal Sensitivity Analysis, Calibration and Uncertainty Evaluation; Techniques and Methods 6-A11; USGS: Reston, VA, 2005.
19. Skold, M. E.; Thyne, G. D.; McCray, J. E. Using UCODE-2005 and PHREEQC to determine thermodynamic constants from experimental data. Ground Water 2007, 45 (3), 368-373.
20. Herbelin, A. L.; Westall, J. C. FITEQLsA Computer Program for Determination of Chemical Equilibrium Constants from Experimental Data (Version 4.0); Report 99-01; Oregon State University: Corvallis, OR, 1999.
21. Mahoney, J. J.; Jakubowski, R. T. Assessment of uranyl sorption constants on ferrihydritesComparison of model derived constants and updates to the diffuse layer model database. In Uranium Mining and Hydrogeology; Merkel, B. J., Hasche-Berger, A., Eds.; Springer: Berlin, 2008; pp 919-928.