Coherent transfer via environment-induced vibronic resonance

Journal of Chemical Physics

Volumn 130, Issue 21, 2009, Pages

  Tamura, Hiroyuki ^a  

^a TOHOKU UNIVERSITY   (Japan)

Author keywords

[No Author keywords available]

Indexed keywords

COHERENT POPULATION TRANSFER; COHERENT TRANSFER; COUPLED ELECTRONIC STATE; ENVIRONMENT DYNAMICS; HIGH FREQUENCY SYSTEMS; LOW FREQUENCY; LOW-FREQUENCY MODES; QUANTUM DYNAMICS CALCULATIONS; REALISTIC SYSTEMS; RESONANCE CONDITION; TRANSFER PHENOMENON;

QUANTUM THEORY; RESONANCE;

DYNAMICS;

EID: 67249102770     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.3146903     Document Type: Article

References (23)

1. P. W. Milonni and J. H. Eberly, Lasers (Wiley, New York, 1998), p. 191.
2. I. Lizuain and J. G. Muga, Phys. Rev. A 1050-2947 75, 033613 (2007). 10.1103/PhysRevA.75.033613
3. J. Cao, C. J. Bardeen, and K. R. Wilson, J. Chem. Phys. 0021-9606 113, 1898 (2000) 10.1063/1.481993; A. A. Budini, R. L. de Matos Filho, and N. Zagury, Phys. Rev. A 1050-2947 65, 041402 (R) (2002). 10.1103/PhysRevA.65.041402
4. G. S. Engel, T. R. Calhoun, E. L. Read, T. -K. Ahn, T. Mancal, Y. -C. Cheng, R. E. Blankenship, and G. R. Fleming, Nature (London) 0028-0836 446, 782 (2007). 10.1038/nature05678
5. H. Lee, Y. C. Cheng, and G. R. Fleming, Science 0036-8075 316, 462 (2007).
6. H. Köppel, W. Domcke, and L. S. Cederbaum, Adv. Chem. Phys. 0065-2385 57, 59 (1984). 10.1002/9780470142813.ch2
7. V. May and O. Kühn, Charge and Energy Transfer Dynamics in Molecular Systems (Wiley-VCH, Weinheim and Chichester, 2004).
8. G. D. Scholes and G. Rumbles, Nature Mater. 1476-1122 5, 683 (2006). 10.1038/nmat1710
9. B. C. Stipe, M. A. Rezaei, and W. Ho, Science 0036-8075 280, 1732 (1998) 10.1126/science.280.5370.1732; L. J. Lauhon and W. Ho, Phys. Rev. B 0163-1829 60, R8525 (1999). 10.1103/PhysRevB.60.R8525
10. Y. Ohta, A. V. Soudackov, and S. Hammes-Schiffer, J. Chem. Phys. 0021-9606 125, 144522 (2006). 10.1063/1.2354500
11. D. Egorova, A. Kühl, and W. Domcke, Chem. Phys. 0301-0104 268, 105 (2001). 10.1016/S0301-0104(01)00293-2
12. D. Egorova, M. Thoss, and W. Domcke, J. Chem. Phys. 0021-9606 119, 2761 (2003). 10.1063/1.1587121
13. H. Wang, M. Thoss, and W. H. Miller, J. Chem. Phys. 0021-9606 115, 2979 (2001). 10.1063/1.1385561
14. M. Thoss, H. Wang, and W. H. Miller, J. Chem. Phys. 0021-9606 115, 2991 (2001). 10.1063/1.1385562
15. O. Kühn, V. May, and M. Schreiber, J. Chem. Phys. 0021-9606 101, 10404 (1994). 10.1063/1.467921
16. D. Egorova, Chem. Phys. 0301-0104 347, 166 (2008) 10.1016/j.chemphys. 2007.12.019; D. Egorova, M. Gelin, and W. Domcke, J. Chem. Phys. 0021-9606 126, 074314 (2007). 10.1063/1.2435353
17. H. Tamura, J. G. S. Ramon, E. R. Bittner, and I. Burghardt, Phys. Rev. Lett. 0031-9007 100, 107402 (2008) 10.1103/PhysRevLett.100.107402; H. Tamura, J. G. S. Ramon, E. R. Bittner, and I. Burghardt, J. Phys. Chem. B 1089-5647 112, 495 (2008) 10.1021/jp077270p; H. Tamura, E. R. Bittner, and I. Burghardt, J. Chem. Phys. 0021-9606 127, 034706 (2007) 10.1063/1.2748050; H. Tamura, E. R. Bittner, and I. Burghardt, J. Chem. Phys. 0021-9606 126, 021103 (2007). 10.1063/1.2431358
18. H. -D. Meyer, U. Manthe, and L. S. Cederbaum, Chem. Phys. Lett. 0009-2614 165, 73 (1990) 10.1016/0009-2614(90)87014-I; M. H. Beck, A. Jäckle, G. A. Worth, and H. -D. Meyer, Phys. Rep. 0370-1573 324, 1 (2000). 10.1016/S0370-1573(99)00047-2
19. L. S. Cederbaum, E. Gindensperger, and I. Burghardt, Phys. Rev. Lett. 0031-9007 94, 113003 (2005) 10.1103/PhysRevLett.94.113003; E. Gindensperger, I. Burghardt, and L. S. Cederbaum, J. Chem. Phys. 0021-9606 124, 144103 (2006) 10.1063/1.2183304; I. Burghardt, E. Gindensperger, and L. S. Cederbaum, Mol. Phys. 0026-8976 104, 1081 (2006) 10.1080/00268970500417887; E. Gindensperger, H. Köppel, and L. S. Cederbaum, J. Chem. Phys. 0021-9606 126, 034106 (2007) 10.1063/1.2426342; E. Gindensperger and L. S. Cederbaum, J. Chem. Phys. 0021-9606 127, 124107 (2007). 10.1063/1.2778682
20. U. Weiss, Quantum Dissipative Systems (World Scientific, Singapore, 1999); A. Garg, J. N. Onuchic, and V. Ambegaokar, J. Chem. Phys. 0021-9606 83, 4491 (1985). 10.1063/1.449017
21. A. Damjanovic, I. Kosztin, U. Kleinekathöfer, and K. Schulten, Phys. Rev. E 1063-651X 65, 031919 (2002). 10.1103/PhysRevE.65.031919
22. See EPAPS Document No. E-JCPSA6-130-002923 for the parameters of the environmental modes and the basis functions expanding the wave functions. For more information on EPAPS, see http://www.aip.org/pubservs/epaps.html.
23. We have carried out some preliminary calculations based on the reduced density matrix explicitly accounting for the system plus the effective environmental mode (X1) and approximating other environmental modes as a stochastic bath (unpublished). Here, the narrow- and wide-band environments are replaced by effective environments that induce slow and fast dissipations, respectively. The reduced model can reproduce the qualitative feature of the environment-induced transfer to some extent.