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All measured fluorescence-decay curves were first individually fitted by sums of up to three exponentials. However, because the individual fit results showed nearly identical decay constants for d(T)20 and d(TTCTT) 4 and for dT(TCT)6T, d(TC)10, d(TC) 9T, and d(C)20 within the standard deviations, we decided to perform a joint fit to the respective transients with the rationale being to determine more-precise values for those decay times and to elucidate possible similarities of the dynamics. Common time constants were also identified, when the time profiles for the purine single strands and the double strands were individually fitted, and joint fits to the respective data were therefore performed for those strands as well. The fitted time profiles and time constants and amplitudes are given in fig. S3 and table S1
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20 within the standard deviations, we decided to perform a joint fit to the respective transients with the rationale being to determine more-precise values for those decay times and to elucidate possible similarities of the dynamics. Common time constants were also identified, when the time profiles for the purine single strands and the double strands were individually fitted, and joint fits to the respective data were therefore performed for those strands as well. The fitted time profiles and time constants and amplitudes are given in fig. S3 and table S1.
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This work has been supported by the Deutsche Forschungsgemeinschaft. Furthermore, the authors thank J. Grötzinger for letting us take the CD spectra
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This work has been supported by the Deutsche Forschungsgemeinschaft. Furthermore, the authors thank J. Grötzinger for letting us take the CD spectra.
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