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The nature of the built-in polarization in the case of PL from neutral excitons could be clarified by the temperature dependence of the amplitude of the polarization. In contrast to the mechanism related to thermalization, the valence-band mixing is not expected to strongly depend on temperature. Unfortunately the cryostat which we use for rotation of the sample in the present work is not temperature-variable. Here we must therefore limit ourselves to identifying the two alternative explanations for the origins of the built-in polarization. It is hoped that future studies will be able to eventually resolve this issue.
-
The nature of the built-in polarization in the case of PL from neutral excitons could be clarified by the temperature dependence of the amplitude of the polarization. In contrast to the mechanism related to thermalization, the valence-band mixing is not expected to strongly depend on temperature. Unfortunately the cryostat which we use for rotation of the sample in the present work is not temperature-variable. Here we must therefore limit ourselves to identifying the two alternative explanations for the origins of the built-in polarization. It is hoped that future studies will be able to eventually resolve this issue.
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This probably also agrees with the experimental results of Ref., which is, however, obscured by the fact that the authors of Ref. had not subtracted the built-in polarization from the measured signal. The variable phase of the second angular harmonic obtained in the CL configuration in Ref. apparently comes from the summation of two 2φ -contributions: the CL conversion itself and the built-in polarization. These two 2φ -harmonics are phase-shifted by 45°, and their amplitudes are controlled by unrelated physical mechanisms.
-
This probably also agrees with the experimental results of Ref., which is, however, obscured by the fact that the authors of Ref. had not subtracted the built-in polarization from the measured signal. The variable phase of the second angular harmonic obtained in the CL configuration in Ref. apparently comes from the summation of two 2φ -contributions: the CL conversion itself and the built-in polarization. These two 2φ -harmonics are phase-shifted by 45°, and their amplitudes are controlled by unrelated physical mechanisms.
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34
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Specifically, if one succeeds in obtaining specimens comprised of similar QDs but with a more regular alignment, the conversion amplitude may be increased by almost one order of magnitude, making the results more convincing. One should also note that due to limitations of the experimental apparatus used in this study, we were not able to rotate the sample in the same arrangement as for application of the magnetic field, and that was why the procedure of separation of different signals and artifacts became less reliable.
-
Specifically, if one succeeds in obtaining specimens comprised of similar QDs but with a more regular alignment, the conversion amplitude may be increased by almost one order of magnitude, making the results more convincing. One should also note that due to limitations of the experimental apparatus used in this study, we were not able to rotate the sample in the same arrangement as for application of the magnetic field, and that was why the procedure of separation of different signals and artifacts became less reliable.
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