Carboxylate-containing chelating agent interactions with amorphous chromium hydroxide: Adsorption and dissolution

Geochimica et Cosmochimica Acta

Volumn 72, Issue 13, 2008, Pages 3241-3257

  Carbonaro, Richard F ^a   Gray, Benjamin N ^a   Whitehead, Charles F ^a   Stone, Alan T ^a  

^a The Johns Hopkins University   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

ADSORPTION; CHELATING AGENT; CHROMIUM; DISSOLUTION; EDTA; HYDROXIDE; POROUS MEDIUM;

EID: 44949254806     PISSN: 00167037     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.gca.2008.04.010     Document Type: Article

References (82)

1. Anderson L.D., Kent D.B., and Davis A.D. Batch experiments characterizing the reduction of Cr(VI) using subtoxic material from a mildly reducing sand and gravel aquifer. Environ. Sci. Technol. 28 (1994) 178-185
2. Avena M.J., Giacomelli C.E., Garcia C.D., and DePauli C.P. Dissolution of chromium hydroxides monitored by turbidimetry. Langmuir 12 (1996) 6659-6664
3. Axe K., and Persson P. Time-dependent surface speciation of oxalate at the water-boehmite (γ-AlOOH) interface: implications for dissolution. Geochim. Cosmochim. Acta 65 (2001) 4481-4492
4. Ball J.W., and Izbicki J.A. Occurrence of hexavalent chromium in ground water in the western Mojave Desert, California. Appl. Geochem. 19 (2004) 1123-1135
5. Ball J.W., and Nordstrom D.K. Critical evaluation and selection of standard state thermodynamic properties for chromium metal and its aqueous ions, hydrolysis species, oxides, and hydroxides. J. Chem. Eng. Data 43 (1998) 895-918
6. Bartlett R.J., and Kimble J.M. Behavior of chromium in soils. 2. Hexavalent forms. J. Environ. Qual. 5 (1976) 383-386
7. Benjamin M.M., and Leckie J.O. Conceptual model for metal-ligand-surface interactions during adsorption. Environ. Sci. Technol. 15 (1981) 1050-1057
8. Berry W.J., Boothman W.S., Serbst J.R., and Edwards P.A. Predicting the toxicity of chromium in sediments. Environ. Toxicol. Chem. 23 (2004) 2981-2992
9. Biber M.V., Afonso M.D., and Stumm W. The coordination chemistry of weathering. 4. Inhibition of the dissolution of oxide minerals. Geochim. Cosmochim. Acta 58 (1994) 1999-2010
10. Blesa M.A., Magaz G., Salfity J.A., and Weisz A.D. Structure and reactivity of colloidal metal oxide particles immersed in water. Solid State Ion. 101 (1997) 1235-1241
11. Boily J.F., Nilsson N., Persson P., and Sjoberg S. Benzenecarboxylate surface complexation at the goethite (α-FeOOH)/water interface: I. A mechanistic description of pyromellitate surface complexes from the combined evidence of infrared spectroscopy, potentiometry, adsorption data, and surface complexation modeling. Langmuir 16 (2000) 5719-5729
12. Bondietti G., Sinniger J., and Stumm W. The reactivity of Fe(III) (hydr)oxides: effects of ligands in inhibiting the dissolution. Colloids Surf. A Physicochem. Eng. Aspects 79 (1993) 157-167
13. Borggaard O.K. Effects of phosphate on iron-oxide dissolution in ethylenediamine-N,N,N′,N′-tetraacetic acid and oxalate. Clay Clay Min. 39 (1991) 324-328
14. Burgisser C.S., and Stone A.T. Determination of EDTA, NTA, and other amino carboxylic acids and their Co(II) and Co(III) complexes by capillary electrophoresis. Environ. Sci. Technol. 31 (1997) 2656-2664
15. Burke T., Fagliano J., Goldoft M., Hazen R.E., Iglewicz R., and McKee T. Chromite ore processing residue in Hudson County, New Jersey. Environ. Health Prespect. 92 (1991) 131-137
16. Carbonaro R. F. (2004) Sources, sinks, and speciation of chromium(III) (amino)carboxylate complexes in heterogeneous aqueous media. Ph.D. Dissertation, The Johns Hopkins University.
17. Carbonaro R.F., and Stone A.T. Speciation of chromium(III) and cobalt(III) (amino)carboxylate complexes using capillary electrophoresis. Anal. Chem. 77 (2005) 155-164
18. Casey W.H., and Ludwig C. The mechanism of dissolution of oxide minerals. Nature 381 (1996) 506-509
19. Chang H., and Matijevic E. Interactions of metal hydrous oxides with chelating agents. IV. Dissolution of hematite. J. Colloid Interface Sci. 92 (1983) 479-488
20. Costa M. Potential hazards of hexavalent chromate in our drinking water. Toxicol. Appl. Pharmacol. 188 (2003) 1-5
21. Davies C.W. Ion Association (1962), Butterworths, Washington, DC
22. Davis A., Kempton J.H., and Nicholson A. Groundwater transport of arsenic and chromium at a historical tannery, Woburn, Massachusetts, USA. Appl. Geochem. 9 (1994) 569-582
23. Davis J.A., Kent D.B., Rea B.A., Maest A.S., and Garabedian S.P. Influence of redox environment and aqueous speciation on metal transport in groundwater: preliminary results of trace injection studies. In: Allen H.E., Perdue E.M., and Brown D.S. (Eds). Metals in Groundwater (1993), Lewis Publishers, Boca Raton, FL 223-273
24. Degenhardt J., and McQuillan A.J. In situ ATR-FTIR spectroscopic study of adsorption of perchlorate, sulfate, and thiosulfate ions onto chromium(III) oxide hydroxide thin films. Langmuir 15 (1999) 4595-4602
25. Eary L.E., and Rai D. Chromate removal from aqueous wastes by reduction with ferrous ion. Environ. Sci. Technol. 22 (1988) 972-977
26. Eick M.J., Peak J.D., and Brady W.D. The effect of oxyanions on the oxalate-promoted dissolution of goethite. Soil Sci. Soc. Am. J. 63 (1999) 1133-1141
27. Filius J.D., Hiemstra T., and Van Riemsdijk W.H. Adsorption of small weak organic acids on goethite. J. Colloid Interface Sci. 195 (1997) 368-380
28. Filius J.D., Meeussen J.C.L., Hiemstra T., and Van Riemsdijk W.H. Modeling the binding of benzenecarboxylates by goethite: the ligand and charge distribution model. J. Colloid Interface Sci. 244 (2001) 31-42
29. 3 in dilute acids. Chimia 37 (1983) 338-341
30. 3 and BeO. Geochim. Cosmochim. Acta 50 (1986) 1847-1860
31. Giacomelli C.E., Avena M.J., Camara O.R., and Depauli C.P. Some physicochemical properties of the chromium(III) hydrous oxide aqueous-solution interface. J. Colloid Interface Sci. 169 (1995) 149-160
32. Helm L., and Merbach A.E. Water exchange on metal ions: experiments and simulations. Coord. Chem. Rev. 187 (1999) 151-181
33. Hiller S., Roe M.J., Geelhoed J.S., Fraser A.R., Farmer J.G., and Paterson E. Role of quantitative mineralogical analysis in the investigation of sites contaminated by chromite ore processing residue. Sci. Total Environ. 308 (2003) 195-210
34. Hug S.J., and Bahnemann D. Infrared spectra of oxalate, malonate and succinate adsorbed on the aqueous surface of rutile, anatase and lepidocrocite measured with in situ ATR FTIR. J. Electron Spectrosc. Relat. Phenom. 150 (2006) 208-219
35. 2 in the aqueous phase. Langmuir 10 (1994) 3587-3597
36. Irving H.M.N.H., and Al-Jarrah R.H. Complexes of chromium(III) with nitrilotriacetic acid and their extraction by solutions of aliquat-336 in dichloroethane. Anal. Chim. Acta 60 (1972) 345-355
37. James B.R., and Bartlett R.J. Behavior of chromium in soils: V. Fate of organically complexed Cr(III) added to soil. J. Environ. Qual. 12 (1983) 169-172
38. James B.R., and Bartlett R.J. Behavior of chromium in soils: VII. Adsorption and reduction of hexavalent forms. J. Environ. Qual. 12 (1983) 177-181
39. Jones D.L., Dennis P.G., Owen A.G., and van Hees P.A.W. Organic acid behavior in soils-misconceptions and knowledge gaps. Plant Soil 248 (2003) 31-41
40. Kouvo O., and Vuorelainen Y. Eskoalite, a new chromium mineral. Am. Min. 43 (1958) 1098-1106
41. Kraemer S.M., Chiu V.Q., and Hering J.G. Influence of pH and competitive adsorption on the kinetics of ligand-promoted dissolution of aluminum oxide. Environ. Sci. Technol. 32 (1998) 2876-2882
42. Kumanomido H., Patel R.C., and Matijevic E. Interactions of amino acids with hydrous metal oxides. J. Colloid Interface Sci. 66 (1978) 183-191
43. 3. J. Colloid Interface Sci. (1980) 75
44. Lee G., and Hering J.G. Oxidative dissolution of chromium(III) hydroxide at pH 9, 3, and 2 with product inhibition at pH 2. Environ. Sci. Technol. 39 (2005) 4921-4928
45. Magaz G.E., Rodenas L.G., Morando P.J., and Blesa M.A. Electrokinetic behaviour and interaction with oxalic acid of different hydrous chromium(III) oxides. Croat. Chem. Acta 71 (1998) 917-927
46. Margerum D.W., Cayley G.R., Weatherburn D.C., and Pagenkopf G.K. In: Martell A.E. (Ed). Coordination Chemistry vol. 2 (1978), American Chemical Society, Washington, DC
47. Marschner H. Mineral Nutrition of Higher Plants. second ed. (1995), Academic Press
48. Martell A.E., and Hancock R.D. Metal Complexes in Aqueous Solution (1996), Plenum Press, New York
49. Martell A. E., Smith R. M. and Motekaitis R. J. (2004) NIST Critically Selected Stability Constants of Metal Complexes. NIST.
50. Milton C., Appleman D. E., Appleman M. H., Chao E. C. T., Cuttitta F., Dinnin J. I., Dwornik E. J., Ingram B. L. and Rose H. J. (1976) Merumite: A Complex Assemblage of Chromium Minerals from Guyana. USGS.
51. Noren K., and Persson P. Adsorption of monocarboxylates at the water/goethite interface: the importance of hydrogen bonding. Geochim. Cosmochim. Acta 71 (2007) 5717-5730
52. Nowack B., and Sigg L. Dissolution of Fe(III) hydroxides by metal-EDTA complexes. Geochim. Cosmochim. Acta 61 (1997) 951-963
53. Nowack B., Xue H., and Sigg L. Influence of natural and anthropogenic ligands on metal transport during infiltration of river water to groundwater. Environ. Sci. Technol. 31 (1997) 866-872
54. Ogino H., Watanabe T., and Tanaka N. Equilibrium and kinetic studies of the reactions of N-substituted ethylenediamine-N,N′,N′-triacetatoaquachromium(III) with acetate ions. Inorg. Chem. 14 (1975) 2093-2097
55. Oze C., Fendorf S.E., Bird D.K., and Coleman R. Chromium geochemistry of serpentine soils. Int. Geol. Rev. 46 (2004) 97-126
56. Palmer C.D., and Wittbrodt P.R. Processes affecting the remediation of chromium-contaminated sites. Environ. Health Perspect. 92 (1991) 25-40
57. Papelis C., Hayes K.F., and Leckie J.O. HYDRAQL (1988), Environmental Engineering and Science, Department of Civil Engineering, Stanford University, Stanford, CA
58. 2 in acidic solutions. Environ. Sci. Technol. 36 (2002) 901-907
59. 3. J. Colloid Interface Sci. 80 (1981) 74-83
60. Rai D., Sass B.M., and Moore D.A. Chromium(III) hydrolysis constants and solubility of chromium(III) hydroxide. Inorg. Chem. 26 (1987) 345-349
61. Reartes G.B., Morando P.J., Blesa M.A., Hewlett P.B., and Matijevic E. Reactivity of chromium-oxide in aqueous-solutions. 1. Oxidative dissolution. Chem. Mat. 3 (1991) 1101-1106
62. Reartes G.B., Morando P.J., Blesa M.A., Hewlett P.B., and Matijevic E. Reactivity of chromium-oxide in aqueous-solutions. 2. Acid dissolution. Langmuir 11 (1995) 2277-2284
63. Rodenas L.A.G., Iglesias A.M., Weisz A.D., Morando P.J., and Blesa M.A. Surface complexation description of the dissolution of chromium(III) hydrous oxides by oxalic acid. Inorg. Chem. 36 (1997) 6423-6430
64. Sass B.M., and Rai D. Solubility of amorphous chromium(III)-iron(III) hydroxide solid solutions. Inorg. Chem. 26 (1987) 2228-2232
65. Segal M.G., and Williams W.J. Kinetics of metal-oxide dissolution-oxidative dissolution of chromium(III) oxide by potassium-permanganate. J. Chem. Soc. Faraday Trans. I 82 (1986) 3245-3254
66. Selmer-Olsen A.R. Spectrophotometric determination of chromium with 1,2-diaminocyclohexanetetraacetic acid. Anal. Chim. Acta 26 (1962) 482-486
67. Sigg L., and Stumm W. The interaction of anions and weak acids with the hydrous goethite (α-FeOOH) surface. Colloids Surf. 2 (1981) 101-117
68. 2O, in aqueous suspension. A study of the chemical changes involved in its aging. Inorg. Chem. 25 (1986) 266-271
69. Sprycha R., and Matijevic E. Monodispersed colloidal chromium hydroxide sulfate ion system as a calibration standard for microelectrophoresis. Colloids Surf. 47 (1990) 195-210
70. Stone A.T., Torrents A., Smolen J., Vasudevan D., and Hadley J. Adsorption of organic compounds possessing ligand donor groups at the oxide water interface. Environ. Sci. Technol. 27 (1993) 895-909
71. Stumm W. Chemistry of the Solid-Water Interface: Processes at the Mineral-Water Interface and Particle-Water Interface in Natural Systems (1992), Wiley-Interscience, New York
72. Stumm W. Reactivity at the mineral-water interface: dissolution and inhibition. Colloids Surf. A Physicochem. Eng. Aspects 120 (1997) 143-166
73. Stumm W. Chemistry of the Solid-Water Interface: Processes at the Mineral-Water and Particle-Water Interface in Natural Systems (2001), John Wiley & Sons
74. Stumm W., and Wollast R. Coordination chemistry of weathering-kinetics of the surface-controlled dissolution of oxide minerals. Rev. Geophys. 28 (1990) 53-69
75. Thomas R.P., Hillier S.J., Roe M.J., Geelhoed J.S., Graham M.C., Paterson E., and Farmer J.G. Analytical characterisation of solid- and solution-phase chromium species at copr-contaminated sites. Environ. Geochem. Health 23 (2001) 195-199
76. 2 - in aqueous solution. Bull. Chem. Soc. Jpn. 36 (1963) 554-559
77. von Meyenburg U., Siroky O., and Schwarzenbach G. Deprotonation of metal aquo ions. 2. Aquochromium(III) ion-structure of active chromium hydroxides. Helv. Chim. Acta 56 (1973) 1099-1114
78. Whitehead C. F. (2003) (Amino)carboxylate coordination reactions with ferric (hydr)oxides: adsorption and ligand-assisted dissolution. Ph.D. Dissertation, The Johns Hopkins University.
79. Yates D.E., and Healy T.W. Mechanism of anion adsorption at the ferric and chromic oxide/water interfaces. J. Colloid Interface Sci. 52 (1975) 222-228
80. Yu Q., Kandegedara A., Xu Y., and Rorabacher D.B. Avoiding interferences from Good's buffers: a contiguous series of noncomplexing tertiary amine buffers covering the entire range of pH 3-11. Anal. Biochem. 253 (1997) 50-56
81. Zachara J.M., Ainsworth C.C., Brown G.E., Catalano J.G., McKinley J.P., Qafoku O., Smith S.C., Szecsody J.E., Traina S.J., and Warner J.A. Chromium speciation and mobility in a high level nuclear waste vadose zone plume. Geochim. Cosmochim. Acta 68 (2004) 13-30
82. Zinder B., Furrer G., and Stumm W. The coordination chemistry of weathering. 2. Dissolution of Fe(III) oxides. Geochim. Cosmochim. Acta 50 (1986) 1861-1869