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Volumn 121, Issue 5, 2004, Pages 2117-2124

Preparation and resolution of molecular states by coherent sequences of phase-locked ultrashort laser pulses

Author keywords

[No Author keywords available]

Indexed keywords

ELECTRIC FIELD EFFECTS; ELECTRIC POTENTIAL; ELECTRONIC STRUCTURE; FLUORESCENCE; FUNCTIONS; HAMILTONIANS; HOLOGRAPHIC INTERFEROMETRY; MOLECULAR DYNAMICS; MOLECULAR VIBRATIONS; QUANTUM THEORY;

EID: 4043143419     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.1767513     Document Type: Article
Times cited : (6)

References (37)
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    • T. C. Weinacht, J. Ahn, and P. H. Bucksbaum, Phys. Rev. Lett. 80, 5508 (1998); ibid. Nature (London) 397, 233 (1999).
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    • to be published
    • T. S. Humble and J. A. Cina, Phys. Rev. Lett. (to be published). In this paper three electronic surfaces are considered with no knowledge of the surface where the target state evolves.
    • Phys. Rev. Lett.
    • Humble, T.S.1    Cina, J.A.2
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    • R. Duarte-Zamorano and V. Romero-Rochín (unpublished)
    • R. Duarte-Zamorano and V. Romero-Rochín (unpublished).
  • 27
    • 4043049759 scopus 로고    scopus 로고
    • note
    • -15 s when the laser pulse is interacting with the molecule while the later is used when the Hamiltonian describing the system is time-independent, that is, when the molecule evolves without interaction.
  • 28
    • 0001097952 scopus 로고    scopus 로고
    • If the pulses are very short (less than a few optical cycles) and the system dynamics very rapid (competitive with the electronic transition frequency) that the rotating-wave approximation breaks down, one could turn to an alternative approach to electronic interference spectroscopy that has recently been developed; see A. W. Albrecht, J. D. Hybl, S. M. Gallagher Faeder, and D. M. Jonas, J. Chem. Phys. 111, 10934 (1999). In this work a method for clocking intrapulse delays by spectral interferometry rather than controlling them, as in the original phase-locking scheme of Schere and co-workers Ref. 15, is demonstrated. This new technique can operate even when the undersampling rate, (1/2π)Ω, of conventional phase locking is inadequate.
    • (1999) J. Chem. Phys. , vol.111 , pp. 10934
    • Albrecht, A.W.1    Hybl, J.D.2    Gallagher Faeder, S.M.3    Jonas, D.M.4
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