XPS and TEM studies on the role of the support and alkali promoter in Ru/MgO and Ru-Cs+ZMgO catalysts for ammonia-synthesis

Journal of Physical Chemistry C

Volumn 111, Issue 26, 2007, Pages 9427-9436

  Larichev, Yurii V ^a   Moroz, Boris L ^a   Zaikovskii, Vladimir I ^a   Yunusov, Safar M ^b   Kalyuzhnaya, Elena S ^b   Shur, Vladimir B ^b   Bukhtiyarov, Valerii I ^a  

^a BORESKOV INSTITUTE OF CATALYSIS   (Russian Federation)

^b A N NESMEYANOV INSTITUTE OF ORGANOELEMENT COMPOUNDS   (Russian Federation)

Author keywords

[No Author keywords available]

Indexed keywords

CESIUM COMPOUNDS; CHARACTERIZATION; FERMI LEVEL; MAGNESIA; RUTHENIUM; WETTING; X RAY PHOTOELECTRON SPECTROSCOPY;

ENERGY DISPERSIVE X-RAY (EDX) MICROANALYSIS; FINAL STATE EFFECTS; WETNESS TECHNIQUE;

CATALYSTS;

EID: 34547458637     PISSN: 19327447     EISSN: 19327455     Source Type: Journal    
DOI: 10.1021/jp066970b     Document Type: Article

References (45)

1. Schloegl, R. In Handbook of Heterogeneous Catalysis; Ertl, G.; Knozinger, H.; Weitkamp, J., Eds.; Wiley-VCH: Weinheim, Germany, 1997; Vol. 4, Chapter 2.1, p 1697.
2. Czuppon, T. A.; Knez, S. A.; Schneider, R. V.; Worobets, G. Chem. Eng. 1993, 100, 19.
3. Kowalczyk, Z.; Jodzis, S.; Rarog, W.; Zielinski, J.; Pielaszek, J. Appl. Catal., A 1998, 173, 153.
4. Aika, K.; Niwa, Y. In Studies in Surface Science and Catalysis; Hattori, H., Otsuka, K., Eds.; Elsevier Science: Tokyo, 1999; Vol. 121, p 327.
5. Bielawa, H.; Hinrichsen, O.; Birkner, A.; Muhler, M. Angew. Chem., Int. Ed. 2001, 40, 1061.
6. Aika, K.; Ohya, A.; Ozaki, A.; Inoue, Y.; Yasumori, Y. J. Catal. 1985, 92, 305.
7. Aika, K.; Takano, T.; Murata, S. J. Catal. 1992, 136, 126.
8. Khaja, M. S.; Rama, R. K. S.; Rama, R. P. Indian J. Chem., Ser. A 1993, 32, 383.
9. Yunusov, S. M.; Moroz, B. L.; Ivanova, A. S.; Likholobov, V. A.; Shur, V. B. J. Mol. Catal. A: Chem. 1998, 132, 263.
10. Moggi, P.; Predieri, G.; Maione, A. Catal. Lett. 2002, 79, 7.
11. Muhler, M.; Rosowski, F.; Hinrichsen, O.; Hornung, A.; Ertl, G. In Studies in Surface Science and Catalysis; Hightower, J. W., Delglass, W. N., Iglesia, E., Bell, A. T., Eds.; Elsevier Science: New York, 1996; Vol. 101, p 317.
12. Yunusov, S. M.; Likholobov, V. A.; Shur, V. B. Appl. Catal., A 1997, 158, L35.
13. Aika, K.; Tamaru, K. In Ammonia: Catalysis and Manufacture; Nielsen, A., Ed.; Springer: Berlin, 1995; p 104.
14. Aika, K.; Kubota, J.; Kadowaki, Y.; Niwa, Y.; Izumi, Y. Appl. Surf. Sci. 1997, 121/122, 488.
15. Hinrichsen, O.; Rosowski, F.; Hornung, A.; Muhler, M.; Ertl, G. J. Catal. 1997, 165, 33.
16. Dahl, S.; Logadottir, A.; Jacobsen, C. J. H.; Norskov, J. K. Appl. Catal., A 2001, 222, 19.
17. Cattania, M. G.; Parmigiani, F.; Ragaini, V. Surf. Sci. 1989, 211/212, 1097.
18. Szmigiel, D.; Bielawa, H.; Kurtz, M.; Hinrichsen, O.; Rosowski, F.; Muhler, M.; Rarog, W.; Jodzis, S.; Kowalczyk, Z.; Znak, L.; Zielinski, J. J. Catal. 2002, 205, 205.
19. McClaine, B. C.; Davis, R. J. J. Catal. 2002, 210, 387.
20. Bukhtiyarov, V. I.; Slin'ko, M. G. Russ. Chem. Rev. 2001, 70, 147.
21. Rosowski, F.; Hornung, A.; Hinrichsen, O.; Herein, D.; Muhler, M.; Ertl, G. Appl. Catal., A 1997, 151, 443.
22. Briggs, D.; Seach, M. P. Practical Surface Analysis; Wiley: Chichester, U.K., 1992; Vol. 1.
23. Kuznetsov, L. D.; Dmitrenko, L. M.; Rabina, P. D.; Sokolinsky, Y. A. Ammonia synthesis; Khimia: Moscow, 1982 (in Russian).
24. Anderson, J. R. Structure of Metallic Catalysts; Academic Press: London, 1975.
25. Barr, T. L. Crit. Rev. Anal. Chem. 1991, 22, 229.
26. Barr, T. L.; Hoppe, E.; Dugall, T.; Shah P.; Seal S. J. Electron Spectrosc. Relat. Phenom. 1999, 98/99, 95.
27. Bukhtiyarov, V. I.; Prosvirin, I. P.; Kvon, R. I. J. Electron Spectrosc. Relat. Phenom. 1996, 77, 7.
28. Larichev, Y. V.; Moroz, B. L.; Prosvirin, I. P.; Bukhtiyarov, V. I.; Likholobov, V. A. Chem. Sustainable Dev. 2003, 11, 155.
29. Bartzold, R. C Surf. Sci. 1981, 106, 243.
30. Wagner, C D.; Gale, C D.; Raymond, R. H. Anal. Chem. 1979, 57, 466.
31. Lewis, R. T.; Kelly, M. A. J. Electron Spectrosc. Relat. Phenom. 1980, 20, 105.
32. Werthiem, G. K. Z. Phys. B 1987, 66, 53.
33. Nefedov, V. I.; Gati, D.; Dzhurinskii, B. F.; Serguhin, N. P.; Salyn, Y. V. Russ. J. Inorg. Chem. 1975, 20, 2307.
34. Yang, S. J.; Bates, C W. Appl. Phys. Lett. 1980, 36, 675, and literature cited therein.
35. Ebbinghaus, G.; Simon, A. Chem. Phys. 1979, 43, 117.
36. Ayyoob, M.; Hedge, M. S. Surf. Sci. 1983, 133, 516.
37. Podgornov, E. A.; Prosvirin, I. P.; Bukhtiyarov, V. I. J. Mol. Catal. A: Chem. 2000, 158, 337.
38. Hwang, C C.; An, K. S.; Park, R. J.; Kim, J. S.; Lee, J. B.; Park, C. Y.; Lee, S. B.; Kimura, A.; Kakizaki, A. J. Electron Spectrosc. Relat. Phenom. 1998, 88, 733.
39. Hrbek, J.; Yang, Y. W.; Rodriguez, J. A. Surf. Sci. 1993, 296, 164.
40. Tanabe, K., In Catalysis: Science and Technology; Anderson, J. R., Boudart, M., Eds.; Springer: Berlin, 1981; Vol. 2, p 231.
41. Ebbinghaus, G.; Braun, W.; Simon, A.; Berresheim, K. Phys. Rev. Lett. 1976, 37, 1770.
42. Aika, K.; Shimazaki, K.; Hattori, Y.; Ohya, A.; Ohshima, S.; Shirota, K.; Ozaki, A. J. Catal. 1985, 92, 296.
43. Bates, C W. Phys. Rev. Lett. 1981, 47, 204, and literature cited therein.
44. Shitova, N. B.; Dobrynkin, N. M.; Noskov, A. S.; Prosvirin, I. P.; Bukhtiyarov, V. I.; Kochubei, D. I.; Tsyrul'nikov, P. G.; Shlyapin, D. A. Kinetica i Kataliz (Kinetics &Catalysis) 2004, 45, 414.
45. Larichev, Y. V.; Prosvirin, I. P.; Shlyapin, D. A.; Shitova, N. B.; Tsyrul'nikov, P. G.; Bukhtiyarov, V. I. Kinetica i Kataliz (Kinetics & Catalysis) 2005, 46, 597.