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Volumn 111, Issue 22, 2007, Pages 6141-6145

Ultrafast electron-induced desorption of water from nanometer amorphous solid water films

Author keywords

[No Author keywords available]

Indexed keywords

DESORPTION; FILM THICKNESS; HYDROGEN BONDS; ULTRASHORT PULSES; VACUUM; WATER;

EID: 34250729192     PISSN: 15206106     EISSN: None     Source Type: Journal    
DOI: 10.1021/jp071226s     Document Type: Article
Times cited : (11)

References (22)
  • 1
    • 19944430597 scopus 로고    scopus 로고
    • Garrett, B. C.; Dixon, D. A.; Camaioni, D. M.; Chipman, D. M.; Johnson, M. A.; Jonah, C. D.; Kimmel, G. A.; Miller, J. H.; Rescigno, T. N.; Rossky, P. J.; Xantheas, S. S.; Colson, S. D.; Laufer, A. H.; Ray, D.; Barbara, P. F.; Bartels, D. M.; Becker, K. H.; Bowen, H.; Bradforth, S. E.; Carmichael, I.; Coe, J. V.; Corrales, L. R.; Cowin, J. P.; Dupuis, M.; Eisenthal, K. B.; Franz, J. A.; Gutowski, M. S.; Jordan, K. D.; Kay, B. D.; LaVerne, J. A.; Lymar, S. V.; Madey, T. E.; McCurdy, C. W.; Meisel, D.; Mukamel, S.; Nilsson, A. R.; Orlando, T. M.; Petrik, N. G.; Pimblott, S. M.; Rustad, J. R.; Schenter, G. K.; Singer, S. J.; Tokmakoff, A.; Wang, L. S.; Wittig, C.; Zwier, T. S. Chem. Rev. 2005, 105, 355.
    • Garrett, B. C.; Dixon, D. A.; Camaioni, D. M.; Chipman, D. M.; Johnson, M. A.; Jonah, C. D.; Kimmel, G. A.; Miller, J. H.; Rescigno, T. N.; Rossky, P. J.; Xantheas, S. S.; Colson, S. D.; Laufer, A. H.; Ray, D.; Barbara, P. F.; Bartels, D. M.; Becker, K. H.; Bowen, H.; Bradforth, S. E.; Carmichael, I.; Coe, J. V.; Corrales, L. R.; Cowin, J. P.; Dupuis, M.; Eisenthal, K. B.; Franz, J. A.; Gutowski, M. S.; Jordan, K. D.; Kay, B. D.; LaVerne, J. A.; Lymar, S. V.; Madey, T. E.; McCurdy, C. W.; Meisel, D.; Mukamel, S.; Nilsson, A. R.; Orlando, T. M.; Petrik, N. G.; Pimblott, S. M.; Rustad, J. R.; Schenter, G. K.; Singer, S. J.; Tokmakoff, A.; Wang, L. S.; Wittig, C.; Zwier, T. S. Chem. Rev. 2005, 105, 355.
  • 13
    • 34250716924 scopus 로고    scopus 로고
    • Private communication
    • Wolf, M. Private communication, 2006.
    • (2006)
    • Wolf, M.1
  • 14
    • 84906388320 scopus 로고    scopus 로고
    • For high electronic excitation of metal substrate-adsorbate systems, desorption is generally associated with a DIMET (desorption induced by multiple electronic transitions) picture of repeated electron attachment to a short-lived adsorbate electronic state. Such a picture is not expected to be applicable here, given the system properties. The multielectron effect here is presumably caused by the relatively high density of electrons injected into the water layer
    • For high electronic excitation of metal substrate-adsorbate systems, desorption is generally associated with a DIMET (desorption induced by multiple electronic transitions) picture of repeated electron attachment to a short-lived adsorbate electronic state. Such a picture is not expected to be applicable here, given the system properties. The multielectron effect here is presumably caused by the relatively high density of electrons injected into the water layer.
  • 17
    • 84906360028 scopus 로고    scopus 로고
    • Note that a similar fluence dependence and 2PC have previously been observed for femtosecond laser-induced water desorption from Ag nanoparticles (ref 22). On these grounds, phonon-mediated desorption was concluded in that study, in which TOF measurements were not reported. Our results show that these results may also be explained by an electron-mediated, many-electron process.
    • Note that a similar fluence dependence and 2PC have previously been observed for femtosecond laser-induced water desorption from Ag nanoparticles (ref 22). On these grounds, phonon-mediated desorption was concluded in that study, in which TOF measurements were not reported. Our results show that these results may also be explained by an electron-mediated, many-electron process.
  • 19
    • 84906402970 scopus 로고    scopus 로고
    • We carefully checked that the H2O does not contain traces of D2O
    • 2O.


* 이 정보는 Elsevier사의 SCOPUS DB에서 KISTI가 분석하여 추출한 것입니다.