Measurement of the initial phase of ozone decomposition in water and wastewater by means of a continuous quench-flow system: Application to disinfection and pharmaceutical oxidation

Water Research

Volumn 40, Issue 9, 2006, Pages 1884-1894

  Buffle, Marc Olivier ^a   Schumacher, Jochen ^b   Salhi, Elisabeth ^a   Jekel, Martin ^b   von Gunten, Urs ^a  

^a SWISS FEDERAL INSTITUTE OF AQUATIC SCIENCE AND TECHNOLOGY   (Switzerland)

^b TECHNISCHE UNIVERSITÄT BERLIN   (Germany)

Author keywords

AOP; Disinfection; Drinking water; Hydroxyl radicals; Kinetics; Ozone; Ozone demand; Pharmaceuticals; Quench flow system; Wastewater

Indexed keywords

DECOMPOSITION; DISINFECTION; DRUG PRODUCTS; OXIDATION; OZONE; OZONIZATION; POTABLE WATER; REACTION KINETICS; WASTEWATER; WASTEWATER TREATMENT;

HYDROXYL RADICALS; KINETICS; OZONE DEMAND; QUENCH-FLOW SYSTEM;

WATER TREATMENT;

CARBAMAZEPINE; OZONE; WATER;

DECOMPOSITION; DISINFECTION; DRUG PRODUCTS; OXIDATION; OZONE; OZONIZATION; POTABLE WATER; REACTION KINETICS; WASTEWATER; WASTEWATER TREATMENT; WATER TREATMENT;

DECOMPOSITION; DISINFECTION; DRUG; MICROBIAL ACTIVITY; OXIDATION; OZONE; WASTEWATER;

ARTICLE; CONTINUOUS QUENCH FLOW SYSTEM; DECOMPOSITION; DISINFECTION; EXPERIMENTATION; MICROORGANISM; OXIDATION; OXIDATION REDUCTION POTENTIAL; OZONATION; PRIORITY JOURNAL; WASTE WATER;

EID: 33645238669     PISSN: 00431354     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.watres.2006.02.026     Document Type: Article

References (34)

1. Acero J.L., Stemmler K., and von Gunten U. Degradation kinetics of atrazine and its degradation products with ozone and OH radicals: A predictive tool for drinking water treatment. Environ. Sci. Technol. 34 4 (2000) 591-597
2. Acero J.L., and von Gunten U. Characterization of oxidation processes: ozonation and the AOP O3/H2O2. J. AWWA 93 10 (2001) 99-100
3. Acero J.L., Haderlein S.B., Schmidt T.C., Suter M.J.-F., and von Gunten U. MTBE oxidation by conventional ozonation and the combination ozone/hydrogen peroxide: Efficiency of the process and bromate formation. Environ. Sci. Technol. 35 21 (2001) 4252-4259
4. Bader H., and Hoigné J. Determination of ozone in water by the indigo method. Wat. Res. 15 (1981) 449-456
5. Buffle, M.-O., Chiu, K.-P., Taghipour, F., 2000. UV Reactor conceptualization and performance optimization with computer modeling. In:Disinfection 2000: Disinfection of Wastes in the New Millenium, 15-18 March 2000, New Orleans, LA, USA.
6. Buffle M.-O., Galli S., and von Gunten U. Enhanced bromate control during ozonation: the chlorine-ammonia process. Environ. Sci. Technol. 38 19 (2004) 5187-5195
7. {radical dot} generation. Ozone Sci. Eng., in press.
8. {radical dot} generation during the initial phase of natural water ozonation. Environ. Sci. Technol., in press.
9. Cho M., Kim H., Cho S.H., and Yoon J. Investigation of ozone reaction in river waters causing instantaneous ozone demand. Ozone Sci. Eng. 25 (2003) 251-259
10. Dodd M.C., Buffle M.-O., and von Gunten U. Oxidation of antibacterial molecules by aqueous ozone: moiety-specific reaction kinetics and application ozone-based wastewater treatment. Environ. Sci. Technol. 40 6 (2006) 1969-1977
11. Elovitz M.S., and von Gunten U. Hydroxyl radical/ozone ratios during ozonation processes. I.The Rct concept. Ozone Sci. Eng. 21 3 (1999) 239-260
12. Elovitz M.S., von Gunten U., and Kaiser H.-P. Hydroxyl radical/ozone ratios during ozonation processes. II. The effect of temperature, pH, alkalinity and DOM properties. Ozone Sci. Eng. 22 (2000) 123-150
13. Ferrari B., Paxeus N., Lo Giudice R., Pollio A., and Garric J. Ecotoxicological impact of pharmaceuticals found in treated wastewaters: study of carbamazepine, clofibric acid, and diclofenac. Ecotox. Environ. Safe. 55 3 (2003) 359-370
14. Goni-Urriza M., Capdepuy M., Arpin C., Raymond N., Caumette P., and Quentin C. Impact of an urban effluent on antibiotic resistance of riverine Enterobacteriaceae and Aeromonas spp. Appl. Environ. Microbiol. 66 1 (2000) 125-132
15. Hoigné J. Characterization of water quality criteria for ozonation processes. Part1: Minimal set of analytical data. Ozone Sci. Eng. 16 (1994) 113-120
16. Hoigné J., and Bader H. Rate constants of reactions of ozone with organic and inorganic compounds in water-II Dissociating organic compounds. Wat. Res. 17 (1983) 185-194
17. Hoigné J., and Bader H. Characterization of water quality criteria for ozonation processes. Part2: Lifetime of added ozone. Ozone Sci. Eng. 16 (1994) 121-134
18. Huber M.M., Canonica S., Park G.-Y., and von Gunten U. Oxidation of pharmaceuticals during ozonation and advanced oxidation processes. Environ. Sci. Technol. 37 5 (2003) 1016-1024
19. Huber M.M., Ternes T.A., and von Gunten U. Removal of estrogenic activity and formation of oxidation products during ozonation of 17a-ethinylestradiol. Environ. Sci. Technol. 38 19 (2004) 5177-5186
20. Huber, M. M., Göbel, A., Joss, A., Hermann, N., Loeffler, D., McArdell, C. S., Ried, A., Siegrist, H., Ternes, T., von Gunten, U., 2005. Oxidation of pharmaceuticals during ozonation of municipal wastewater effluents: a pilot study. Environ. Sci. Technol. in press.
21. Joss A., Andersen H., Ternes T., Richle P.R., and Siegrist H. Removal of estrogens in municipal wastewater treatment under aerobic and anaerobic conditions: consequences for plant optimization. Environ. Sci. Technol. 38 11 (2004) 3047-3055
22. Kolpin D.W., Furlong E.T., Meyer M.T., Thurman E.M., Zaugg S.D., Barber L.B., and Buxton H.T. Pharmaceuticals, hormones, and other organic wastewater contaminants in US streams, 1999-2000: a national reconnaissance. Environ. Sci. Technol. 36 6 (2002) 1202-1211
23. Laville N., Ait-Aissa S., Gomez E., Casellas C., and Porcher J.M. Effects of human pharmaceuticals on cytotoxicity, EROD activity and ROS production in fish hepatocytes. Toxicology 196 1-2 (2004) 41-55
24. Mackey E.D., Hargy T.M., Wright H.B., Malley Jr. J.P., and Cushing R.S. Treatment technologies: comparing cryptosporidium and MS2 bioassays-implications for UV reactor validation. J. AWWA 94 2 (2002) 62-69
25. Mvula E., and von Sonntag C. Ozonolysis of phenols in aqueous solution. Org. Biomol. Chem. 1 10 (2003) 1749-1756
26. Paraskeva P., and Graham N.J.D. Ozonation of municipal wastewater effluents. Water. Environ. Res. 74 6 (2002) 569-581
27. Purdom C.E., Hardiman P.A., Bye V.J., Eno N.C., Tyler C.R., and Sumpter J.P. Estrogenic effects of effluents from sewage treatment works. Chem. Ecol. 8 4 (1994) 275-285
28. Rakness K.L., Corsaro K.M., Hale G., and Blank B.D. Watewater disinfection with ozone-Process control and operating results. Ozone Sci. Eng. 15 (1993) 497-514
29. Schumacher, J., Pi, Y. Z., Jekel, M., 2004. Ozonation of persistent DOC in municipal WWTP effluent for groundwater recharge. Water Sci. Technol. 49 (4, Oxidation Technologies for Water and Wastewater Treatment III), 305-310.
30. Schwartz T., Kohnen W., Jansen B., and Obst U. Detection of antibiotic-resistant bacteria and their resistance genes in wastewater, surface water, and drinking water biofilms. FEMS Microbiol. Ecol. 43 3 (2003) 325-335
31. Ternes T.A. Occurence of drugs in german sewage treatment plants and rivers. Water. Res. 32 11 (1998) 3245-3260
32. Thorpe K.L., Cummings R.I., Hutchinson T.H., Scholze M., Brighty G., Sumpter J.P., and Tyler C.R. Relative potencies and combination effects of steroidal estrogens in fish. Environ. Sci. Technol. 37 6 (2003) 1142-1149
33. von Gunten U. Ozonation of drinking water: Part II. Disinfection and by-product formation in presence of bromide, iodide and chlorine. Water. Res. 37 (2003) 1469-1487
34. Xu P., Janex M.-L., Savoye P., Cockx A., and Lazarova V. Wastewater disinfection by ozone: main parameters for process design. Water. Res. 36 4 (2002) 1043-1055