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It is important to distinguish here between uncertainty in a measurement from uncertainty in a model. Both lead to uncertainty in population, but usually only the former source of uncertainty is represented in experimental error bars. The present work, being model independent, suffers only from experimental error.
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Any target atom or molecule undergoing charge transfer is effectively "destroyed." However, singly charged ions interact much less strongly with the target than do near-resonant photons, which are highly perturbative. Thus only a very small fraction of the target is modified through interaction with an ion beam.
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0942270169
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note
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The capture cross sections discussed here refer to randomly oriented targets since both the trapping and repumping beams are incident from all three orthogonal directions.
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In the system used in this work, an acousto-optical modulator (AOM) was used to chop the lasers. The temporal response of the AOM was about 15 ns. A Pockels cell could have easily been used in place of the AOM, leaving the TOF resolution as the "hard limit" to our temporal evolution measurements.
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