Influences of heat transport on the determination of reaction rates using the temperature scanning plug flow reactor

Chemical Engineering Science

Volumn 58, Issue 21, 2003, Pages 4903-4909

  Kolkowski, M ^a   Malachowski, J ^a   Keil, F J ^a   Liebner, C ^b   Wolf, D ^b   Baerns, M ^b  

^a HAMBURG UNIVERSITY OF TECHNOLOGY   (Germany)

^b LEIBNIZ INSTITUT FÜR KATALYSE E V AN DER UNIVERSITÄT ROSTOCK   (Germany)

Author keywords

Deriving reaction rates; Heat conduction; Heat transfer; Numerical analysis; Simulation; Temperature scanning reactor

Indexed keywords

AMMONIA; CHEMICAL REACTORS; HEAT TRANSFER; SYNTHESIS (CHEMICAL);

REACTANT MIXTURES;

RATE CONSTANTS;

HEAT TRANSFER; MATHEMATICAL ANALYSIS; PLUG FLOW; REACTOR; TEMPERATURE EFFECT; TRANSPORT;

EID: 0242572144     PISSN: 00092509     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.ces.2002.11.005     Document Type: Article

References (7)

1. Asprey S.P. Rice N.M. Wojciechowski B.W. The temperature scanning reactor II: Experimental procedures and data processing Catalysis Today 36 1997 209-226
2. Liebner, C., Wolf, D., Baerns, M., Kolkowski, M., - Keil, F. J. (2003). A high-speed method for obtaining kinetic data for exothermic or endothermic catalytic reactions under non-isothermal conditions illustrated for the ammonia synthesis. Applied Catalysis A, 240, 95-110.
3. Rice N.M. Wojciechowski B.W. The temperature scanning reactor II: Theory of operation Catalysis Today 36 1997 191-207
4. Sehested J. Jacobsen C.J.H. Toernqvist E. Rokni S. Stoltze P. Ammonia sythesis over a multipromoted iron catalyst: Extended set of activity measurements, microkinetic model, and hydrogen inhibition Journal of Catalysis 188 1999 83-89
5. Verein Deutscher Ingenieure (1991). VDI-Wärmeatlas: Berechnungsblätter für den Wärmeübergang (6th ed.). Ge1-Ge4, Mh4-Mh6, Mh9-Mh11. Düsseldorf: VDI-Verlag.
6. Wojciechowski B.W. The temperature scanning reactor I: Reactor types and modes of operation Catalysis Today 36 1997 167-190
7. Wojciechowski B.W. Rice N.M. Experimental methods in kinetic studies 1st ed. 2001 M. J. Wojciechowski Naples, FL