Rheological evidence for a dynamical crossover in polymer melts via nonequilibrium molecular dynamics

Physical Review Letters

Volumn 85, Issue 5, 2000, Pages 1128-1131

  Kröger, Martin ^a,b   Hess, Siegfried ^a  

^a TECHNISCHE UNIVERSITÄT BERLIN   (Germany)

^b ETH ZURICH   (Switzerland)

Author keywords

[No Author keywords available]

Indexed keywords

CHEMICAL BONDS; COMPUTER SIMULATION; DENSITY (SPECIFIC GRAVITY); DIFFUSION; MOLECULAR DYNAMICS; MOLECULAR ORIENTATION; MOLECULAR WEIGHT; RHEOLOGY; TEMPERATURE; VISCOELASTICITY;

DYNAMICAL CROSSOVER; ENTANGLEMENT MOLECULAR WEIGHT; FINITELY EXTENSIBLE NONLINEAR ELASTIC CHAIN MODEL; NONEQUILIBRIUM MOLECULAR DYNAMICS; POLYMER MELTS; POWER LAW BEHAVIOR; SHEAR RATES;

POLYMERS;

EID: 0038711087     PISSN: 00319007     EISSN: None     Source Type: Journal    
DOI: 10.1103/PhysRevLett.85.1128     Document Type: Article

References (29)

1. M. Kröger, W. Loose, and S. Hess, J. Rheol. 37, 1057 (1993).
2. T. Aoyagi and M. Doi, Comput. Theor. Polym. Sci. 10, 317 (2000).
3. J. Gao and J. H. Weiner, J. Chem. Phys. 90, 6749 (1989); M. Kröger, C. Luap, and R. Muller, Macromolecules 30, 526 (1997).
4. J. Gao and J. H. Weiner, J. Chem. Phys. 90, 6749 (1989); M. Kröger, C. Luap, and R. Muller, Macromolecules 30, 526 (1997).
5. T. P. Lodge, N. A. Rotstein, and S. Prager, Adv. Chem. Phys. 79, 1 (1990).
6. J. Klein, Nature (London) 271, 143 (1978); P. Schleger, B. Farago, C. Lartigue, A. Kollmar, and D. Richter, Phys. Rev. Lett. 81, 124 (1998).
7. J. Klein, Nature (London) 271, 143 (1978); P. Schleger, B. Farago, C. Lartigue, A. Kollmar, and D. Richter, Phys. Rev. Lett. 81, 124 (1998).
8. R. F. Landel, J. W. Berge, and J. D. Ferry, J. Colloid. Sci. 12, 400 (1957); H. H. Meyer, W. J. Pfeiffer, Jr., and J. D. Ferry, Biopolymers 5, 123 (1967).
9. R. F. Landel, J. W. Berge, and J. D. Ferry, J. Colloid. Sci. 12, 400 (1957); H. H. Meyer, W. J. Pfeiffer, Jr., and J. D. Ferry, Biopolymers 5, 123 (1967).
10. T. A. Witten, Rev. Mod. Phys. 71, S367 (1999); H. Voigt, Struktur und Dynamik von Kettenverschlaufungen in Polymersystemen (W&T Publishing, Berlin, 1996); R. Y. Qian, J. Macromol. Sci. Phys. B 38, 75 (1999); A. L. Kholodenko and T. A. Vilgis, Phys. Rep. 298, 254 (1998); J. Rault, J. Non-Newt. Fluid. Mech. 23, 229 (1987).
11. T. A. Witten, Rev. Mod. Phys. 71, S367 (1999); H. Voigt, Struktur und Dynamik von Kettenverschlaufungen in Polymersystemen (W&T Publishing, Berlin, 1996); R. Y. Qian, J. Macromol. Sci. Phys. B 38, 75 (1999); A. L. Kholodenko and T. A. Vilgis, Phys. Rep. 298, 254 (1998); J. Rault, J. Non-Newt. Fluid. Mech. 23, 229 (1987).
12. T. A. Witten, Rev. Mod. Phys. 71, S367 (1999); H. Voigt, Struktur und Dynamik von Kettenverschlaufungen in Polymersystemen (W&T Publishing, Berlin, 1996); R. Y. Qian, J. Macromol. Sci. Phys. B 38, 75 (1999); A. L. Kholodenko and T. A. Vilgis, Phys. Rep. 298, 254 (1998); J. Rault, J. Non-Newt. Fluid. Mech. 23, 229 (1987).
13. T. A. Witten, Rev. Mod. Phys. 71, S367 (1999); H. Voigt, Struktur und Dynamik von Kettenverschlaufungen in Polymersystemen (W&T Publishing, Berlin, 1996); R. Y. Qian, J. Macromol. Sci. Phys. B 38, 75 (1999); A. L. Kholodenko and T. A. Vilgis, Phys. Rep. 298, 254 (1998); J. Rault, J. Non-Newt. Fluid. Mech. 23, 229 (1987).
14. T. A. Witten, Rev. Mod. Phys. 71, S367 (1999); H. Voigt, Struktur und Dynamik von Kettenverschlaufungen in Polymersystemen (W&T Publishing, Berlin, 1996); R. Y. Qian, J. Macromol. Sci. Phys. B 38, 75 (1999); A. L. Kholodenko and T. A. Vilgis, Phys. Rep. 298, 254 (1998); J. Rault, J. Non-Newt. Fluid. Mech. 23, 229 (1987).
15. M. Kröger and H. Voigt, Macromol. Theory Simul. 3, 639 (1994).
16. K. Kremer, G. S. Grest, and I. Carmesin, Phys. Rev. Lett. 61, 566 (1988); K. Kremer and G. S. Grest, J. Phys. Chem. 92, 5057 (1990).
17. K. Kremer, G. S. Grest, and I. Carmesin, Phys. Rev. Lett. 61, 566 (1988); K. Kremer and G. S. Grest, J. Phys. Chem. 92, 5057 (1990).
18. J. Gao and J. H. Weiner, J. Chem. Phys. 103, 1621 (1995).
19. J. D. Ferry, Viscoelastic Properties of Polymers (J. Wiley & Sons, New York, 1980).
20. M. Pütz, K. Kremer, and G. S. Grest, Europhys. Lett. 49, 735 (2000).
21. M. Kröger and S. Hess, Physica (Amsterdam) 195A, 336 (1993); M. Kröger, Physica (Amsterdam) 249A, 332 (1998).
22. M. Kröger and S. Hess, Physica (Amsterdam) 195A, 336 (1993); M. Kröger, Physica (Amsterdam) 249A, 332 (1998).
23. M. Doi and S. F. Edwards, J. Chem. Soc. Faraday Trans. II 74, 1789 (1978); 74, 1818 (1978); 75, 38 (1979).
24. M. Doi and S. F. Edwards, J. Chem. Soc. Faraday Trans. II 74, 1789 (1978); 74, 1818 (1978); 75, 38 (1979).
25. M. Doi and S. F. Edwards, J. Chem. Soc. Faraday Trans. II 74, 1789 (1978); 74, 1818 (1978); 75, 38 (1979).
26. G. S. Grest, B. Dünweg, and K. Kremer, Comput. Phys. Commun. 55, 269 (1989).
27. M. Kröger, Comput. Phys. Commun. 118, 278 (1999).
28. L. J. Fetters, D. J. Lohse, S. T. Milner, and W. W. Graessley, Macromol. 32, 6847 (1999).
29. D. W. Mead, R. G. Larson, and M. Doi, Macromolecules 31, 7895 (1998).