Dielectric study on the heterogeneous dynamics of miscible polyisoprene/poly(vinyl ethylene) blends: Estimation of the relevant length scales for the segmental relaxation dynamics

Macromolecules

Volumn 36, Issue 10, 2003, Pages 3699-3708

  Hirose, Yuji ^a   Urakawa, Osamu ^a   Adachi, Keiichiro ^a  

^a OSAKA UNIVERSITY   (Japan)

Author keywords

[No Author keywords available]

Indexed keywords

DONTH MODEL; HETEROGENEOUS DYNAMICS; POLYVINYL ETHYLENE BLENDS; SEGMENTAL MOTIONS; SEGMENTAL RELAXATION DYNAMICS;

BLOCK COPOLYMERS; COMPUTER SIMULATION; DIELECTRIC PROPERTIES; MOLECULAR DYNAMICS; POLYETHYLENES; POLYISOPRENES; RELAXATION PROCESSES; SOLUBILITY;

POLYMER BLENDS;

EID: 0037768390     PISSN: 00249297     EISSN: None     Source Type: Journal    
DOI: 10.1021/ma0217940     Document Type: Article

References (45)

1. Utracki, L. A. Polymer alloys and Blends: Thermodynamics and Rheology; Carl Hanser Verlag; Munich, Germany, 1989
2. Colby, R. H. Polymer 1989, 30, 1275.
3. Roovers, J.; Toporowski, P. M. Macromolecules 1992, 25, 1096-1102.
4. Roovers, J.; Toporowski, P. M. Macromolecules 1992, 25, 3454-3461.
5. Pathak, J. A.; Colby, R. H. Floudas, G.; Jerome, R. Macromolecules 1999, 32, 2553-2561.
6. Alegria, A.; Colmenero, J.; Ngai, K. L.; Roland, C. M. Macromolecules 1994, 27, 4486-4492.
7. Alvarez, F.; Alegria, A.; Colmenero, J. Macromolecules 1997, 30, 597-604.
8. Arbe, A.; Alegria, A.; Colmenero, J.; Hoffmann, S.; Willner, L.; Richter, D. Macromolecules 1999, 32, 7572-7581.
9. Roland, C. M.; Ngai, K. L. Macromolecules 1991, 24, 2261-2265.
10. Roland, C. M.; Ngai, K. L. Macromolecules 1992, 25, 363-367.
11. Ngai, K. L.; Roland, C. M.; O'Reilly, J. M.; Sedita, J. S. Macromolecules 1992, 25, 3906-3909.
12. Cendoya, I.; Alegria, A.; Alberdi, J. M.; Colmenero, J.; Grimm, H.; Richter, D.; Frick, B. Macromolecules 1999, 32, 4065-4078.
13. Zetsche, A.; Fischer, E. W. Acta Polym. 1994, 45, 168-175.
14. Kanatakis, J.; Fytas, G.; Hadjichristidis, N. Macromolecules 1991, 24, 1806-1812.
15. Kanatakis, J.; Fytas, G.; Kremer, F.; Pakula, T. Macromolecules 1992, 25, 3484-3491.
16. Miller, J. B.; McGrath, K. J.; Roland, C. M.; Trask, C. A.; Garroway, A. N. Macromolecules 1990, 23, 4543-4547.
17. Chin, Y. H.; Zhang, C.; Wang, P.; Inglefield, P. T.; Jones, A. A.; Kambour, R. P.; Bendler, J. T.; White, D. M. Macromolecules 1992, 25, 3031-3038.
18. Chung, G.-C.; Kornfield, J. A.; Smith, S. D. Macromolecules 1994, 27, 964-973.
19. Chung, G.-C.; Kornfield, J. A.; Smith, S. D. Macromolecules 1994, 27, 5729-5741.
20. Min, B.; Qiu, X. H.; Ediger, M. D.; Pitsikalis, M.; Hadjichristidis, N. Macromolecules 2001, 34, 4466-4475.
21. Lutz, T. R.; He, Y.; Ediger, M. D.; Cao, H.; Lin, G.; Jones, A. A. Submitted to Macromolecules.
22. Arendt, B. H.; Krishnamoorti, R.; Kornfield, J. A.; Smith, S. D. Macromolecules 1997, 30, 1127-1137.
23. Kamath, S.; Colby, R. H.; Kumar, S. K.; Karatasos, K.; Floudas, G.; Fytas, G.; Roovers, J. E. L. J. Chem. Phys. 1999, 111, 6121-6128.
24. Hoffmann, S.; Willner, L.; Richter, D.; Arbe, A. Colmenero, J.; Farago, F. Phys. Rev. Lett. 2000, 85, 772-775.
25. Arendt, B. H.; Krishnamoorti, R.; Kannan, R. M.; Seitz, K.; Kornfield, J. A.; Roovers, J. Macromolecules 1997, 30, 1138-1145.
26. Katana, G.; Fischer, E. W.; Hack, Th.; Abetz, V.; Kremer, F. Macromolecules 1995, 28, 2714-2722.
27. Milhaupt, J. M.; Lodge, T. P.; Smith, S. D.; Hamersky, M. W. Macromolecules 2001, 34, 5561-5570.
28. Urakawa, O.; Fuse, Y.; Hori, H.; Tran-Cong, Q.; Yano, O. Polymer 2001, 42, 765-773.
29. Roland, C. M. Macromolecules 1987, 20, 2557.
30. Roland, C. M. J. Polym. Sci., Polym. Phys. Ed. 1988, 26, 839.
31. Tomlin, D. W.; Roland, C. M. Macromolecules 1992, 25, 2994-2996.
32. Kumar, S. K.; Colby, R. H.; Anastasiadis, S. H.; Fytas, G. J. Chem. Phys. 1996, 105, 3777-3788.
33. Lodge, T. P.; McLeish, T. C. B. Macromolecules 2000, 33, 5278-5284.
34. Donth, E. J. Non Cryst. Solids 1982, 53, 325-330.
35. Adam, G.; Gibbs, J. H. J. Chem. Phys. 1965, 43, 139-146.
36. Adachi, K.; Kotaka, T. Prog. Polym. Sci. 1993, 18, 585-622.
37. Halasa, A. F.; Lohr, D. F.; Hall, J. E. J. Polym. Sci., Polym. Chem. Ed. 1981, 19, 1357-1360.
38. Fox, T. G. Bull. Am. Phys. Soc. 1956, 1, 123.
39. Gordon, M.; Taylor, J. S. J. Appl. Chem. 1952, 2, 495.
40. Kwei, T. K. J. Polym. Sci., Polym. Lett. Edn. 1984, 22, 307.
41. Ferry, J. D. Viscoelastic Properties of Polymers; Wiley: New York, 1980.
42. Adachi, K.; Hirano, H. Macromolecules 1998, 31, 3958-3962.
43. Schonhals, A. In Dielectric Spectroscopy of Polymeric Materials; Runt, J. P., Fitzgerald, J. J., Eds.; American Chemical Society: Washington, DC, 1997; Chapter 3.
44. eff's for the normal mode and segmental mode relaxation times of pure PI (by using the data in ref 43) were resolved to be less than 2 K.
45. Adachi, K.; Nishi, I.; Itoh, S.; Kotaka, T. Macromolecules 1990, 23, 2550.