FTIR studies of the reaction of gaseous NO with HNO3 on porous glass: Implications for conversion of HNO3 to photochemically active NOx in the atmosphere

Journal of Physical Chemistry A

Volumn 104, Issue 43, 2000, Pages 9705-9711

  Mochida, Michihiro ^a,b   Finlayson Pitts, Barbara J ^a  

^a UNIVERSITY OF CALIFORNIA   (United States)

^b HOKKAIDO UNIVERSITY   (Japan)

Author keywords

[No Author keywords available]

Indexed keywords

IONS; NITRATES; NITRIC ACID; NITROGEN OXIDES; PHOTOCHEMICAL REACTIONS; POROUS MATERIALS;

HETEROGENEOUS REACTIONS;

FOURIER TRANSFORM INFRARED SPECTROSCOPY;

EID: 0034322505     PISSN: 10895639     EISSN: None     Source Type: Journal    
DOI: 10.1021/jp001471a     Document Type: Article

References (52)

1. Finlayson-Pitts, B. J.; Pitts, J. N. Chemistry of the Upper and Lower Atmosphere: Theory, Experiments and Applications; Academic Press: San Diego, 2000 and references therein.
2. Chatfield, R. B. Geophys. Res. Lett. 1994, 21, 2705-2708.
3. Rogaski, C. A.; Golden, D. M.; Williams, L. R. Geophys. Res. Lett. 1997, 24, 381-384.
4. Choi, W.; Leu, M. T. J. Phys. Chem. A. 1998, 102, 7618-7630.
5. Hauglustaine, D. A.; Ridley, B. A.; Solomon, S.; Hess, P. G.; Madronich, S. Geophys. Res. Lett. 1996, 23, 2609-2612.
6. Lary, D. J.; Lee, A. M.; Toumi, R.; Newchurch, M. J.; Pirre, M.; Renard, J. B. J. Geophys. Res. 1997, 102, 3671-3682.
7. Honrath, R. E.; Peterson, M. C.; Guo, S.; Dibb, J. E.; Shepson, P. B.; Campbell, B. Geophys. Res. Lett. 1999, 26, 695-698.
8. Jones, A. E.; Weller, R.; Wolff, E. W.; Jacobi, H. W. Geophys. Res. Lett. 2000, 27, 345-348.
9. Johnson, E. R. The Radiation-Induced Decomposition of Inorganic Molecular Ions; Gordon and Breach: New York, 1970.
10. Wagner, I.; Strehlow, H.; Busse, G. Z. Phys. Chem. 1980, 123, 1-33.
11. Vogt, R.; Finlayson-Pitts, B. J. J. Phys. Chem. 1995, 99, 17269-17272.
12. Smith, J. H. J. Am. Chem. Soc. 1947, 69, 1741-1747.
13. Jaffe, S.; Ford, H. W. J. Phys. Chem. 1967, 71, 1832-1836.
14. Kaiser, E. W.; Wu, C. H. J. Phys. Chem. 1977a, 81, 187-190.
15. Streit, G. E.; Wells, J. S.; Fehsenfeld, F. C.; Howard, C. J. J. Chem. Phys. 1979, 70, 3439-3443.
16. England, C.; Corcoran, W. H. Ind. Eng. Chem. Fundam. 1975, 14, 55-63.
17. Wallington, T. J.; Japar, S. M. J. Atmos. Chem. 1989, 9, 399-409.
18. Besemer, A. C.; Nieboer, H. Atmos. Environ. 1985, 19, 507-513.
19. Fairbrother, D. H.; Sullivan, D. J. D.; Johnston, H. S. J. Phys. Chem. A 1997, 101, 7350-7358.
20. Barney, W. S.; Finlayson-Pitts, B. J. J. Phys. Chem. A 2000, 104, 171-175.
21. Kiselev, A. V.; Lygin, V. I. Infrared Spectra of Surface Compounds; Wiley: New York, 1975.
22. Barney, W. S.; Wingen, L. M.; Lakin, M. J.; Brauers, T.; Stutz, J.; Finlayson-Pitts, B. J. J. Phys. Chem. A 2000, 104, 1692-1699.
23. Goodman, A. L.; Underwood, G. M.; Grassian, V. H. J. Phys. Chem. A. 1999, 103, 7217-7223.
24. Querry, M. R.; Tyler, I. L. J. Chem. Phys. 1980, 72, 2495-2499.
25. Biermann, U. M.; Luo, B. P.; Peter, T. J. Phys. Chem. A. 2000, 104, 783-793.
26. 4 is observed (Saliba, N.; Mochida, M.; Finlayson-Pitts, B. J. Geophys. Res. Lett. In press.).
27. Sharma, H. D.; Jervis, R. E.; Wong., K. Y. J. Phys. Chem. 1979, 74, 923-933.
28. Sakamaki, F.; Hatakeyama, S.; Akimoto, H. Int. J. Chem. Kinet. 1983, 15, 1013-1029.
29. Pitts, J.; J. N.; Sanhueza, E.; Atkinson, R.; Carter, W. P. L.; Winer, A. M.; Harris, G. W.; Plum, C. N. Int. J. Chem. Kinet. 1984a, 16, 919-939.
30. Svensson, R.; Ljungstrom, E.; Lindqvist, O. Atmos. Environ. 1987, 21, 1529-1539.
31. Jenkin, M. E.; Cox, R. A.; Williams, D. J. Atmos. Environ. 1988, 22, 487-498.
32. Febo, A.; Perrino, C. Atmos. Environ. 1991, 25A, 1055-1061.
33. Bambauer, A.; Brantner, B.; Paige, M.; Novakov, T. Atmos. Environ. 1994, 28, 3225-3232.
34. Mertes, S.; Wahner, A. J. Phys. Chem. 1995, 99, 14000-14006.
35. Kleffmann, J.; Becker, K. H.; Wiesen, P. Atmos. Environ. 1998a, 32, 2721-2729.
36. 2 in the cell, would be generated in 20 s, about 2 orders of magnitudes less than observed (Table 1).
37. Wayne, L. G.; Yost, D. M. J. Chem. Phys. 1951, 19, 41-47.
38. Graham, R. F.; Tyler, B. J. J. Chem. Soc., Faraday Trans. 1 1972, 68, 683-688.
39. Chan, W. H.; Nordstrom, R. J.; Calvert, J. G.; Shaw, J. H. Chem. Phys. Lett. 1976a, 37, 441-446.
40. Chan, W. H.; Nordstrom, R. J.; Calvert, J. G.; Shaw, J. H. Environ. Sci. Technol. 1976b, 10, 674-682.
41. Cox, R. A.; Derwent, R. G. J. Photochem. 1976/77, 6, 23-34.
42. Kaiser, E. W.; Wu, C. H. J. Phys. Chem. 1977b, 81, 1701-1706.
43. 2 would be generated in 20 s, much less than observed (Table 1).
44. Zhuravlev, L. T. Colloids Surf. 1993, 74, 71-90.
45. Sneh, O.; Cameron, M. A.; George, S. M. Surface Science 1996, 364, 61-78.
46. Brown, S. S.; Talukdar, R. K.; Ravishankara, A. R. J. Phys. Chem. A. 1999, 103, 3031-3037.
47. DeMore, W. B.; Sander, S. P.; Golden., D. M.; Hampson, R. F.; Kurylo, M. J.; Howard, C. J.; Ravishankara, A. R.; Kolb, C. E.; Molina, M. J. Chemical Kinetics and Photochemical Data for Use in Stratospheric Modeling, Evaluation No. 12. In JPL Publications; Jet Propulsion Laboratory: Pasadena, 1997; Vol. 97-4.
48. Dentener, F. J.; Carmichael, G. R.; Zhang, Y.; Lelieveld, J.;. Crutzen, P. J. J. Geophys. Res. 1996, 101, 22, 869-22, 889.
49. Sjodin, A.; Ferm, M. Atmos. Environ. 1985, 19, 985-992.
50. Notholt, J.; Hjorth, J.; Raes, F. Atmos. Environ. 1992, 26A, 211-217.
51. Winer, A. M.; Biermann, H. W. Rev. Chem. Intermed. 1994, 20, 423-445.
52. Calvert, J. G.; Yarwood, G.; Dunker, A. M. Res. Chem. Intermed. 1994, 20, 463-502.