Confirmation of a calorimetric peculiarity in the crossover region of glass transition in poly(n-hexyl methacrylate) by differential scanning calorimetry

Journal of Molecular Structure

Volumn 479, Issue 2-3, 1999, Pages 149-162

  Kahle, S ^a   Hempel, E ^a   Beiner, M ^a   Unger, R ^a   Schroter K ^a   Donth, E ^a  

^a MARTIN LUTHER UNIVERSITY HALLE WITTENBERG   (Germany)

Author keywords

Calorimetry; Cooperativity; Free volume; Glass transition; Vitrification

Indexed keywords

ANALYTIC METHOD; ARTICLE; DIFFERENTIAL SCANNING CALORIMETRY; ENTROPY; LIQUID CRYSTAL; SHEAR STRESS; THERMOGRAPHY; VISCOSITY;

EID: 0033608973     PISSN: 00222860     EISSN: None     Source Type: Journal    
DOI: 10.1016/S0022-2860(98)00866-7     Document Type: Article

References (65)

1. Barlow A.J., Lamb J., Matheson A.J. Proc. R. Soc. Lond. A. 292:1966;322.
2. Cukierman M., Lane J.W., Uhlmann D.R. J. Chem. Phys. 59:1973;3639.
3. Laughlin W.T., Uhlmann D.R. J. Phys. Chem. 76:1972;2317.
4. Stickel F., Fischer E.W., Richert R. J. Chem. Phys. 102:1995;6251.
5. Stickel F., Fischer E.W., Richert R. J. Chem. Phys. 104:1996;2043.
6. F. Stickel, Thesis, Universität Mainz, Shaker, Aachen, 1995.
7. Rössler E. Phys. Rev. Lett. 69:1992;1620.
8. Fujara F., Geil B., Sillescu H., Fleischer G. Z. Phys. B. 88:1992;195.
9. Sokolov A.P. Science. 273:1996;1675.
10. Sokolov A.P. Endeavour. 21:1997;109.
11. N.G. McCrum, B.E. Read, G. Williams, Anelastic and Dielectric Effects in Polymeric Solids, Wiley, London, 1967.
12. Johari G.P., Goldstein M. J. Chem. Phys. 53:1970;2372.
13. Johari G.P., Goldstein M. J. Chem. Phys. 74:1970;2034.
14. Johari G.P., Goldstein M. J. Chem. Phys. 55:1971;4245.
15. Johari G.P. Ann. New York Acad. Sci. 279:1976;117.
16. Adam G., Gibbs J.H. J. Chem. Phys. 43:1965;139.
17. Richert R., Angell C.A. J. Chem. Phys. 108:1998;2016.
18. Birge N.O., Nagel S.R. Phys. Rev. Lett. 54:1985;2674.
19. Korus J., Beiner M., Busse K., Kahle S., Unger R., Donth E. Thermochim. Acta. 304/305:1997;99.
20. Birge N.O., Dixon P.K., Menon N. Thermochim. Acta. 304/305:1997;51.
21. Garwe F., Schönhals A., Lockwenz H., Beiner M., Schröter K., Donth E. Macromolecules. 29:1996;247.
22. Hempel E., Beiner M., Renner T., Donth E. Acta Polymer. 47:1996;525.
23. S. Reissig, M. Beiner, S. Zeeb, S. Höring, E. Donth. Macromolecules, submitted.
24. Kahle S., Korus J., Hempel E., Unger R., Höring S., Schröter K., Donth E. Macromolecules. 30:1997;7214.
25. Kuebler S.C., Schaefer D.J., Boeffel C., Pawelzik U., Spiess H.W. Macromolecules. 30:1997;6597.
26. Beiner M., Kahle S., Hempel E., Schröter K., Donth E. Macromolecules. 31:1998;8973.
27. Korus J., Hempel E., Beiner M., Kahle S., Donth E. Acta Polymer. 48:1997;369.
28. J. Korus, Dissertation, Universität Halle, 1997.
29. Moynihan C.T., Easteal A.J., DeBolt M.A., Tucker J. J. Amer. Ceram. Soc. 59:1976;12.
30. Narayanaswamy O.S. J. Am. Ceram. Soc. 54:1971;491.
31. S. Kahle, Dissertation, Universität Halle, 1997.
32. Moynihan C.T., Macedo P.B., Montrose C.J., Gupta P.K., DeBolt M.A., Dill J.F., Dom B.E., Drake P.W., Easteal A.J., Eltermann P.B., Moeller R.P., Sasabe H., Wilder J.A. Ann. New York Acad. Sci. 279:1976;15.
33. Brunacci A., Cowie J.M.G., Ferguson R., Gómez Ribelles J.L., Vidaurre Garayo A. Macromolecules. 29:1996;7976.
34. Gómez Ribelles J.L., Monleón Pradas M., Vidaurre Garayo A., Romero Colomer F., Más Estellés J., Meseguer Dueñas J.M. Macromolecules. 28:1995;5878.
35. Donth E., Beiner M., Reissig S., Korus J., Garwe F., Vieweg S., Kahle S., Hempel E., Schröter K. Macromolecules. 29:1996;6589.
36. E. Donth, Relaxation and Thermodynamics in Polymers. Glass Transition, Akademie-Verlag, Berlin, 1992.
37. Havriliak S., Negami S. J. Polym. Sci. C. 14:1966;99.
38. Kishimoto K., Suga H., Seki S. Bull. Chem. Soc. Jpn. 46:1973;3020.
39. Donth E. J. Non-Cryst. Solids. 53:1982;325.
40. E. Donth, Glasübergang, Akademie-Verlag, Berlin, 1981.
41. Donth E. J. Polym. Sci. B: Polym. Phys. 34:1996;2881.
42. Murthy S.S.N. J. Chem. Soc. Faraday Trans. 85:1989;581.
43. Murthy S.S.N. J Mol. Liquids. 44:1989;51.
44. A. Schönhals, in: M. Giordano et al. (Eds.), Non Equilibrium Phenomena in Supercooled Fluids, Glasses and Amorphous Materials, World Scientific, Singapore, 1997, p. 210.
45. W. Götze, in: J.P. Hansen, D. Levesque, J. Zinn-Justin (Eds.), Liquids, Freezing and the Glass Transition, Proc. Les Houches Summer School, North Holland, Amsterdam, 1989, p. 1.
46. Götze W., Sjögren L. Rep. Prog. Phys. 55:1992;241.
47. Goldstein M. J. Chem. Phys. 51:1969;3728.
48. Donth E. Acta Polymer. 30:1979;481.
49. Donth E. J. Phys. I France. 6:1996;1189.
50. W. Feller, An Introduction to Probability Theory and Its Applications, 2nd ed., Wiley, New York, 1971, pp.169-176, 569-570, 574-581.
51. Glarum S.H. J. Chem. Phys. 33:1960;639.
52. Shlesinger M.F. Ann. Rev. Phys. Chem. 39:1988;269.
53. E. Donth, Acta Polymer, submitted.
54. Donth E., Kahle S., Korus J., Beiner M. J. Phys. I France. 7:1997;581.
55. Williams G. Trans. Faraday Soc. 62:1966;2091.
56. Suga H., Seki S. J. Non-Cryst. Solids. 16:1974;171.
57. J.D. Ferry, Viscoelastic Properties of Polymers, Wiley, New York, 1961.
58. N.W. Tschoegl, The Phenomenological Theory of Linear Viscoelastic Behavior, Springer, Berlin, 1989.
59. Kahle S., Schulz M., Donth E. J. Non-Cryst. Solids. 238:1998;234.
60. Hodge I.M. J. Non-Cryst. Solids. 169:1994;211-266.
61. Hodge I.M. Macromolecules. 20:1987;2897.
62. Hodge I.M. Macromolecules. 16:1983;898.
63. Hutchinson J.M., Ruddy M. J. Polym. Sci. 26:1988;2341.
64. W.M. Prest Jr., F.J. Roberts, I.M. Hodge, in: J.C. Buck (Ed.), Proceedings of 12th NATAS Conference, NATAS, 1983, p.119.
65. Privalko V.P., Demchenko S.S., Lipatov Y.S. Macromolecules. 19:1986;901.