A three-dimensional simulation of the Antarctic ozone hole: Impact of anthropogenic chlorine on the lower stratosphere and upper troposphere

Journal of Geophysical Research Atmospheres

Volumn 102, Issue 7, 1997, Pages 8909-8930

  Brasseur, Guy P ^a   Tie, XueXi ^a   Rasch, Philip J ^a   Lefèvre, Frank ^b  

^a NATIONAL CENTER FOR ATMOSPHERIC RESEARCH   (United States)

^b CENTRE NATIONAL DE RECHERCHES MÉTÉOROLOGIQUES   (France)

Author keywords

[No Author keywords available]

Indexed keywords

ANTHROPOGENIC IMPACT; CHLORINE; CLOUD FORMATION; OZONE; POLAR STRATOSPHERIC CLOUD; STRATOSPHERE; TROPOSPHERE;

ANTARCTICA;

EID: 0031417255     PISSN: 01480227     EISSN: None     Source Type: Journal    
DOI: 10.1029/96jd03398     Document Type: Article

References (48)

1. Austin, J., and N. Butchart, Three-dimensional modelling study of the influence of planetary wave dynamics on polar ozone chemistry, J. Geophys. Res., 97, 10, 165-10,186, 1992.
2. Austin, J., and N. Butchart, Influence of climate change and timing of stratospheric warming on Arctic ozone depletion, J. Geophys. Res., 99, 1127-1145, 1994.
3. 2 climate, Nature, 360, 221-225, 1992.
4. Boville B., Middle atmosphere version of community climate model, 2, Annual cycle and interannual variability, J. Geophys. Res., 100, 9017-9040, 1995.
5. Brasseur, G., and P. C. Solomon, Aeronomy of the Middle Atmosphere, 2nd ed., D. Reidel, Norwell, Mass., 1986.
6. Brasseur, G., M. H. Hitchman, S. Walters, M. Dymek, E. Falise, and M. Pirre, An interactive chemical dynamical radiative two-dimensional model of the middle atmosphere, J. Geophys. Res., 95, 5639-5655, 1990.
7. Cariolle, D., A. Lasserre-Bigorry, and J. F. Boyer, A general circulation model simulation of the springtime Antarctic ozone decrease and its impact on midlatitudes, J. Geophys. Res., 95, 1883-1898, 1990.
8. Chipperfield, M. P., D. Carriolle, P. Simon, R. Ramaroson, and D. J. Lary, A three-dimensional modeling study of trace species in the Arctic lower stratosphere during winter 1989-1990, J. Geophys. Res., 98, 7199-7218, 1993.
9. Crutzen, J. P., and F. Arnold, Nitric acid cloud formation in the cold Antarctic stratosphere: A major cause for the springtime 'ozone hole,' Nature, 324, 651-655, 1986.
10. Danilin, M. J., and J. C. McConnell, Stratospheric effects of bromine activation on/in sulfate aerosols, J. Geophys. Res., 100, 11,237-11,243, 1995.
11. DeMore, W. B., et al., Chemical kinetics and photochemical data for use in stratospheric modeling, JPL Publ. 94-26, Jet Propul. Lab., Pasadena, Calif., 1994.
12. Dobson, G. M. B., Forty years' research on atmospheric ozone at Oxford: A history, Appl. Opt., 1, 387-405, 1968.
13. Dye, J. E., D. Baumgardner, B. W. Gandrud, S. R. Kawa, K. K. Kelly, M. Loewensein, G. V. Ferry, K. R. Chan, and B. L. Gary, Particle size distributions in Arctic polar stratospheric clouds, growth and freezing of sulfuric acid droplets, and implications for cloud formation, J. Geophys. Res., 97, 8015-8034, 1992.
14. Eckman, R. S., W. L. Grose, R. E. Turner, and W. T. Blackshear, Polar ozone depletion: A three-dimensional chemical modeling study of its long-term global impact, J. Geophys. Res., 101, 22,977-22,989, 1996.
15. Fox, L. E., D. R. Worsnop, M. S. Zahniser, S. C. Wofsy, Metastable phases in polar stratospheric aerosols, Science, 267, 351-355, 1995.
16. Fuchs, N. A., The Mechanics of Aerosols, 408 pp., Pergamon, Tarrytown, N. Y., 1964.
17. Granier, C., and G. Brasseur, Ozone and other trace gases in the Arctic and Antarctic regions: Three-dimensional model simulation, J. Geophys. Res., 96, 2995-3011, 1991.
18. Granier, C., and G. Brasseur, Impact of heterogeneous chemistry on model predictions of ozone changes, J. Geophys. Res., 97, 18,015-18,033, 1992.
19. Granier, C., J. F. Muller, S. Madronich, and G. Brasseur, Possible causes for the 1991-1993 decrease in global tropospheric CO abundance: A three-dimensional study, Atmos. Environ., 30, 1673-1682, 1996.
20. Grose, W. L., R. S. Eckman, R. E. Turner, and W. T. Blackshear, Antarctic ozone depletion and potential effects on the global ozone budget, in Dynamics, Chemistry and Photochemistry in the Middle Atmosphere of the Southern Hemisphere, edited by A. O'Neill and C. R. Mechoso, Kluwer Acad., Norwell, Mass., 1990.
21. Hack, J. J., B. A. Boville, B. P. Briegleb, J. T. Kiehl, P. J. Rasch, and D. L. Williamson, Description of the NCAR community climate model (CCM2), Tech. Note, NCAR/TN-382+STR, 108 pp., Natl. Cent, for Atmos. Res., Boulder, Colo., 1993.
22. Hanson, D., and K. Mauersberger, Laboratory studies of the nitric acid trihydrate: Implications for the south polar stratosphere, Geophys. Res. Lett., 15, 855-858, 1988.
23. 5 on polar stratospheric cloud materials, J. Geophys. Res., 96, 5081-5090, 1991.
24. Hanson, D. R., A. R. Ravishankara, Heterogeneous chemistry of bromine species in sulfuric acid under stratospheric conditions, Geophys. Res. Lett., 22, 385-388, 1995.
25. Hanson, D. R., A. R. Ravishankara, and S. Solomon, Heterogeneous reactions in sulfuric acid aerosols: A framework for model calculations, J. Geophys. Res., 99, 3615-3629, 1994.
26. Hofmann, D. J., S. J. Oltmans, J. A. Lathrop, J. M. Harris, and H. Volmel, Record low ozone at the South Pole in the spring of 1993, Geophys. Res. Lett., 21, 421-424, 1994.
27. Holtslag, A. A. M., and B. A. Boville, Local versus nonlocal boundarylayer diffusion in a global climate model, J. Clim., 6, 1825-1842, 1993.
28. 2o, J. Phys. Chem., 74, 2984-2989, 1970.
29. Kasten, F., Falling speed of aerosol particles, J. Appl. Meteorol., 7, 944-947, 1968.
30. Kiehl, J. T., B. A. Boville, and B. P. Briegleb, Response of a general circulation model to a prescribed Antarctic ozone hole, Nature, 332, 501-504, 1988.
31. Lary, D. J., M. P. Chipperfield, and R. Toumi, Heterogeneous atmospheric bromine chemistry, J. Geophys. Res., 101, 1489-1504, 1996.
32. Lefèvre, F., G. P. Brasseur, I. Folkins, A. K. Smith, and P. Simon, Chemistry of the 1991-1992 stratospheric winter: Three-dimensional model simulation, J. Geophys. Res., 99, 8183-8195, 1994.
33. Madronich, S., and C. Granier, Tropospheric chemistry changes due to increased UV-B radiation, in Stratospheric Ozone Depletion/UV-B Radiation in the Biosphere, NATO ASISer. I, vol. 18, edited by R. H. Biggs and M. E. B. Joyner, pp. 3-10, Springer-Verlag, New York, 1994.
34. Mahlman, J. D., J. P. Pinto, and L. J. Umscheid, Transport, radiative, and dynamical effects of the Antarctic ozone hole: A GFDL "SKYHI" model experiment, J. Atmos. Sci., 51, 489-508, 1994.
35. McFarlane, N. A., The effect of orographically excited gravity wave drag on the general circulation of lower stratosphere and troposphere, J. Atmos. Sci., 44, 1775-1800, 1988.
36. 2O system: Implications for polar stratospheric clouds, Science, 261, 1418, 1993.
37. Moore, S. B., L. F. Keyser, M. T. Leu, R. P. Turco, and R. H. Smith, Heterogeneous reactions on nitric acid trihydrates, Nature, 345, 333-335, 1990.
38. Portmann, R. W., S. Solomon, R. R. Garcia, L. W. Thomason, L. R. Poole, and M. P. McCormick, Role of aerosol variations in atmospheric ozone depletion in polar regions, J. Geophys. Res., 101, 22,991-23,006, 1996.
39. Prather, M., M. M. Garcia, R. Suozzo, and D. Rind, Global impact on the Antarctic ozone hole: Dynamical dilution with a three-dimensional chemical transport model, J. Geophys. Res., 95, 3449-3471, 1990.
40. Rasch, P. J., and D. L. Williamson, Sensitivity of a general circulation model climate to the moisture transport formulation, J. Geophys. Res., 96, 13,123-13,137, 1991.
41. Rasch, P. J., B. A. Boville, G. P. Brasseur, A three-dimensional general circulation model with coupled chemistry for the middle atmosphere, J. Geophys. Res.. 100, 9041-9071, 1995.
42. 3, and aerosol by the UARS CLASH Experiment between January 1992 and April 1993, J. Atmos. Sci., 51, 2877-2902, 1994.
43. 2O, on ice and nitric acid trihydrate, J. Phys. Chem., 94, 3255-3260, 1990.
44. Tabazadeh, A., R. P. Turco, K. Drdla, and M. Z. Jacobson, A study of type I polar stratospheric cloud formation, Geophys. Res. Lett., 21, 1619-1622, 1994.
45. Tolbert, M. A., Sulfate aerosols and polar stratospheric cloud formation, Science, 264, 527-528, 1994.
46. Toon, O. B., and M. A. Tolbert, Spectroscopic evidence against nitric acid trihydrate in polar stratospheric clouds. Nature, 375, 218-220, 1995.
47. 3 and HCl in the winter polar stratospheres, Geophys Res. Lett., 13, 1284-1287, 1986.
48. World Meteorological Organization (WMO), Scientific Assessment of Ozone Depletion: 1991, Geneva, 1992.