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Volumn 111, Issue 9, 1999, Pages 4121-4130

Two-dimensional vibrational spectroscopy. I. Theoretical calculation of the nonlinear Raman response function of CHCl3

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Indexed keywords


EID: 0001143103     PISSN: 00219606     EISSN: None     Source Type: Journal    
DOI: 10.1063/1.479709     Document Type: Article
Times cited : (45)

References (86)
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    • edited by S. H. Lin, A. A. Villaeys, and Y. Fujimura World Scientific, Singapore
    • M. Cho, in Advances in Multi-Photon Processes and Spectroscopy, edited by S. H. Lin, A. A. Villaeys, and Y. Fujimura (World Scientific, Singapore, 1999), p. 229. In this review article, four types of time- and frequency-domain two-dimensional vibrational spectroscopies were theoretically described. By using IR and off-resonant optical fields, it was shown that various 2D vibrational spectroscopic measurements could be carried out to selectively study those vibrational modes that are either IR-or Raman-active, or both. The complete frequency-domain analogs of the time-domain 2D vibrational spectroscopies were also discussed in detail and were theoretically described by using the quantum electrodynamics formalism.
    • (1999) Advances in Multi-Photon Processes and Spectroscopy , pp. 229
    • Cho, M.1
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    • note
    • In fact, both the nonlinearity of the molecular linear polarizability and the potential anharmonicity are originated from the electronic nature within the Born-Oppenheimer approximation. The approximated electronic wave function is parametrized by the nuclear coordinates to provide the potential energy surface. Thus, the mechanical as well as electronic anharmonicities are "electronic" in origin. However, the terminologies, mechanical and electronic anharmonicities, in a limited sense, are commonly used in the literature so they will be consistently used throughout this paper and the two companion papers.


* 이 정보는 Elsevier사의 SCOPUS DB에서 KISTI가 분석하여 추출한 것입니다.