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Volumn 103, Issue 45, 1999, Pages 10053-10064

Dynamics of the Heterogeneous Electron-Transfer Reaction of Cytochrome C552 from Thermus Thermophilus, a Time-Resolved Surface-Enhanced Resonance Raman Spectroscopic Study

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Indexed keywords


EID: 0001079578     PISSN: 15206106     EISSN: None     Source Type: Journal    
DOI: 10.1021/jp991818d     Document Type: Article
Times cited : (32)

References (74)
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    • note
    • f in this potential range are much shorter. Thus, the adsorption equilibrium is not established in the time-resolved experiments so that in a good approximation the amount of adsorbed B1 can be regarded as constant.
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    • unpublished results
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    • 552 than for Cyt-c
    • 552 than for Cyt-c.
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    • red greater than +2.
    • red greater than +2.
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    • 552 in the present work. Moreover, anion binding cannot account for the nonlinearity of the Nernstian plot at positive potentials which, in contrast, is readily understood on the basis of the present PET model. In addition, this model may also explain (in part) errors associated with the ET rate constant determination. It may be that repetitive potential jumps cause irreversible changes of the charge distribution in the electrical double layer which in turn affect the potential drop at the redox site and thus the ET rate.
    • (1988) J. Biol. Chem. , vol.263 , pp. 11652
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    • note
    • cor as listed in Table 2. Using the uncorrected potentials, the reorganization energy was only slightly lower (0.13 eV) but the rms was worse.
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    • 9a
    • 9a


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