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The Lorentz isotropic local field correction, f = (∈ + 2)/3, has been used for photosynthetic complexes with a static dielectric constant ∈ of about 2.
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11644260702
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note
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In arriving at a value for fΔμ⊥ that part of the theory of ref 16 that assumes that the variance of Δμ is zero was used. However, in that reference it is shown that the introduction of a Gaussian distribution for Δμ makes only a small difference when F of eq 3 is ≲3.5.
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52
-
-
11644262098
-
-
note
-
The double hole structure of the 825 nm band can be understood in terms of energy transfer from two higher energy subunits to the lowest energy subunit.
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53
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56
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11644265676
-
-
note
-
Coupling energies of Pearlstein were uniformly reduced by about a factor of 2. It was argued that the energy disorder relative to the excitonic couplings between subunits of the trimer is sufficiently large to cause localization on a single subunit.
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57
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33751553603
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Altmann, R.B.1
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64
-
-
85088545739
-
-
note
-
y excitations of the B800 ring are essentially localized on single B800 molecules. The situation for the B850 and B875 rings is different, vide supra.
-
-
-
-
65
-
-
0030584679
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67
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85088546580
-
-
note
-
int.
-
-
-
-
68
-
-
11644258836
-
-
note
-
Here we are free to associate the dimer with the basic α,β polypeptide pair.
-
-
-
-
71
-
-
11644317493
-
-
note
-
These findings for localization are valid for weak energy disorder, which means that the disorder-induced matrix elements between energetically different exciton levels are comparable to or smaller than the spacings between the levels. Low-temperatuare absorption and hole-burned spectra are consistent with weak energy disorder.48
-
-
-
-
73
-
-
11644317392
-
-
note
-
This assumption is made even when the S/N ratio of the absorption band is high enough to yield acceptable first and second derivatives.
-
-
-
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