Ammonia Electrosynthesis with High Selectivity under Ambient Conditions via a Li+ Incorporation Strategy

Journal of the American Chemical Society

Volumn 139, Issue 29, 2017, Pages 9771-9774

  Chen, Gao Feng ^a   Cao, Xinrui ^b   Wu, Shunqing ^b   Zeng, Xingye ^a   Ding, Liang Xin ^a   Zhu, Min ^a   Wang, Haihui ^a  

^a SOUTH CHINA UNIVERSITY OF TECHNOLOGY   (China)

^b XIAMEN UNIVERSITY   (China)

Author keywords

[No Author keywords available]

Indexed keywords

CATALYSTS; DENSITY FUNCTIONAL THEORY; ELECTROLYTIC REDUCTION; LITHIUM;

AMBIENT CONDITIONS; ATOMIC SCALE; DIIMIDE; ELECTRO REDUCTION; ELECTROCHEMICAL EVALUATIONS; HIGH POTENTIAL; HIGH SELECTIVITY; RATIONAL DESIGN;

CATALYST SELECTIVITY;

AMMONIA; ETHYLBENZENE; LITHIUM ION; NITROGEN;

ADSORPTION; ARTICLE; CATALYST; DENSITY FUNCTIONAL THEORY; ELECTROCHEMICAL ANALYSIS; ELECTROCHEMISTRY; ELECTROSYNTHESIS; HYDROGENATION; NITROGEN NUCLEAR MAGNETIC RESONANCE; POLYMERIZATION; PROTON NUCLEAR MAGNETIC RESONANCE; REDUCTION (CHEMISTRY); SYNTHESIS; X RAY PHOTOELECTRON SPECTROSCOPY;

EID: 85026312662     PISSN: 00027863     EISSN: 15205126     Source Type: Journal    
DOI: 10.1021/jacs.7b04393     Document Type: Article

References (32)

1. Pickett, C. J.; Talarmin, J. Nature 1985, 317, 652 10.1038/317652a0
2. Christensen, C. H.; Johannessen, T.; Sørensen, R. Z.; Nørskov, J. K. Catal. Today 2006, 111, 140 10.1016/j.cattod.2005.10.011
3. Rosca, V.; Duca, M.; de Groot, M. T.; Koper, M. T. Chem. Rev. 2009, 109, 2209 10.1021/cr8003696
4. Service, R. F. Science 2014, 345, 610 10.1126/science.345.6197.610
5. Brown, K. A.; Harris, D. F.; Wilker, M. B.; Rasmussen, A.; Khadka, N.; Hamby, H.; Keable, S.; Dukovic, G.; Peters, J. W.; Seefeldt, L. C.; King, P. W. Science 2016, 352, 448 10.1126/science.aaf2091
6. Ertl, G. Angew. Chem., Int. Ed. 2008, 47, 3524 10.1002/anie.200800480
7. Honkala, K.; Hellman, A.; Remediakis, I. N.; Logadottir, A.; Carlsson, A.; Dahl, S.; Christensen, C. H.; Nørskov, J. K. Science 2005, 307, 555 10.1126/science.1106435
8. Chirik, P. J. Nat. Chem. 2009, 1, 520 10.1038/nchem.386
9. Van Der Ham, C. J.; Koper, M. T.; Hetterscheid, D. G. Chem. Soc. Rev. 2014, 43, 5183 10.1039/C4CS00085D
10. Spatzal, T.; Aksoyoglu, M.; Zhang, L.; Andrade, S. L.; Schleicher, E.; Weber, S.; Rees, D. C.; Einsle, O. Science 2011, 334, 940 10.1126/science.1214025
11. Lancaster, K. M.; Roemelt, M.; Ettenhuber, P.; Hu, Y.; Ribbe, M. W.; Neese, F.; Bergmann, U.; DeBeer, S. Science 2011, 334, 974 10.1126/science.1206445
12. Giddey, S.; Badwal, S. P. S.; Kulkarni, A. Int. J. Hydrogen Energy 2013, 38, 14576 10.1016/j.ijhydene.2013.09.054
13. Marnellos, G.; Stoukides, M. Science 1998, 282, 98 10.1126/science.282.5386.98
14. Murakami, T.; Nishikiori, T.; Nohira, T.; Ito, Y. J. Am. Chem. Soc. 2003, 125, 334 10.1021/ja028891t
15. Kugler, K.; Luhn, M.; Schramm, J. A.; Rahimi, K.; Wessling, M. Phys. Chem. Chem. Phys. 2015, 17, 3768 10.1039/C4CP05501B
16. Milton, R. D.; Cai, R.; Abdellaoui, S.; Leech, D.; De Lacey, A. L.; Pita, M.; Minteer, S. D. Angew. Chem., Int. Ed. 2017, 56, 2680 10.1002/anie.201612500
17. Kordali, V.; Kyriacou, G.; Lambrou, C. Chem. Commun. 2000, 17, 1673 10.1039/b004885m
18. Lan, R.; Tao, S. RSC Adv. 2013, 3, 18016 10.1039/c3ra43432j
19. Bao, D.; Zhang, Q.; Meng, F. L.; Zhong, H. X.; Shi, M. M.; Zhang, Y.; Yan, J. M.; Jiang, Q.; Zhang, X. B. Adv. Mater. 2017, 29, 1604799 10.1002/adma.201604799
20. Chen, S.; Perathoner, S.; Ampelli, C.; Mebrahtu, C.; Su, D.; Centi, G. Angew. Chem. 2017, 129, 2743 10.1002/ange.201609533
21. Seh, Z. W.; Kibsgaard, J.; Dickens, C. F.; Chorkendorff, I.; Nørskov, J. K.; Jaramillo, T. F. Science 2017, 355, eaad4998 10.1126/science.aad4998
22. Wu, H.; Shevlin, S. A.; Meng, Q.; Guo, W.; Meng, Y.; Lu, K.; Wei, Z.; Guo, Z. Adv. Mater. 2014, 26, 3338 10.1002/adma.201305452
23. Song, Z.; Xu, T.; Gordin, M. L.; Jiang, Y. B.; Bae, I. T.; Xiao, Q.; Zhan, H.; Liu, J.; Wang, D. Nano Lett. 2012, 12, 2205 10.1021/nl2039666
24. Wang, S.; Xia, L.; Yu, L.; Zhang, L.; Wang, H.; Lou, X. W. Adv. Energy Mater. 2016, 6, 1502217 10.1002/aenm.201502217
25. Wang, Y.; Cui, X.; Zhang, Y.; Zhang, L.; Gong, X.; Zheng, G. Adv. Mater. 2016, 28, 7626 10.1002/adma.201602583
26. Deng, W.; Shen, Y.; Qian, J.; Yang, H. Chem. Commun. 2015, 51, 5097 10.1039/C5CC00073D
27. Song, Z.; Zhan, H.; Zhou, Y. Angew. Chem. 2010, 122, 8622 10.1002/ange.201002439
28. Kadiyala, A. K.; Sharma, M.; Bijwe, J. Mater. Des. 2016, 109, 622 10.1016/j.matdes.2016.07.108
29. Lin, D.; Zhuo, D.; Liu, Y.; Cui, Y. J. Am. Chem. Soc. 2016, 138, 11044 10.1021/jacs.6b06324
30. Chen, G.-F.; Ma, T. Y.; Liu, Z.-Q.; Li, N.; Su, Y.-Z.; Davey, K.; Qiao, S. Z. Adv. Funct. Mater. 2016, 26, 3314 10.1002/adfm.201505626
31. Köleli, F.; Kayan, D. B. J. Electroanal. Chem. 2010, 638, 119 10.1016/j.jelechem.2009.10.010
32. Shipman, M. A.; Symes, M. D. Catal. Today 2017, 286, 57 10.1016/j.cattod.2016.05.008