Aqueous tetracycline degradation by H2O2 alone: Removal and transformation pathway

Chemical Engineering Journal

Volumn 307, Issue , 2017, Pages 15-23

  Chen, Yao Yao ^a   Ma, Yu Long ^a   Yang, Jin ^b   Wang, Li Qiong ^a   Lv, Jun Min ^a   Ren, Cui Juan ^a  

^a NINGXIA UNIVERSITY   (China)

^b BEIFANG UNIVERSITY OF NATIONALITIES   (China)

Author keywords

Degradation removal; H2O2; Tetracycline; Transformation pathway

Indexed keywords

ALKALINITY;

H2O2; INITIAL CONCENTRATION; OPERATIONAL PARAMETERS; OXIDATIVE TRANSFORMATIONS; REMOVAL EFFICIENCIES; TETRACYCLINE; TRANSFORMATION PATHWAYS; TRANSFORMATION PRODUCTS;

SOLUTIONS;

EID: 84983059076     PISSN: 13858947     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.cej.2016.08.046     Document Type: Article

References (27)

1. [1] Lindsey, M.E., Meyer, M., Thurman, E.M., Analysis of trace levels of sulfonamide and tetracycline antimicrobials in groundwater and surface water using solid-phase extraction and liquid chromatography/mass spectrometry. Anal. Chem. 73 (2001), 4640–4646.
2. [2] Liu, H., Zhang, G.P., Liu, C.Q., Li, L., Xiang, M., Characteristics of chloramphenicol and tetracyclines in municipal sewage and Nanming River of Guiyang City, China. Environ. Sci. 30 (2009), 687–692.
3. [3] Liu, Y.Q., He, X.X., Duan, X.D., Fu, Y.S., Dionysiou, D.D., Photochemical degradation of oxytetracycline: influence of pH and role of carbonate radical. Chem. Eng. J. 276 (2015), 113–121.
4. [4] Liu, Y.Q., He, X.X., Fu, Y.S., Dionysiou, D.D., Degradation kinetics and mechanism of oxytetracycline by hydroxyl radical-based advanced oxidation processes. Chem. Eng. J. 284 (2016), 1317–1327.
5. [5] Daghrir, R., Drogui, P., Tetracycline antibiotics in the environment: a review. Environ. Chem. Lett. 11 (2013), 209–227.
6. [6] Rahmah, A.U., Harimurti, S., Omar, A.A., Murugesan, T., Photochemical degradation of oxytetracycline hydrochloride in the presence of H2O2. National Postgraduate Conference, 2011, 1–4.
7. [7] Lee, H., Lee, E., Lee, C.H., Lee, K., Degradation of chlortetracycline and bacterial disinfection in livestock wastewater by ozone-based advanced oxidation. J. Ind. Eng. Chem. 17 (2011), 468–473.
8. [8] Hou, L.W., Wang, L.G., Royer, S., Zhang, H., Ultrasound-assisted heterogeneous Fenton-like degradation of tetracycline over a magnetite catalyst. J. Hazard. Mater. 302 (2016), 458–467.
9. [9] Neyens, E., Baeyens, J., A review of classic Fenton's peroxidation as an advanced oxidation technique. J. Hazard. Mater. 98 (2003), 33–50.
10. 4@C catalyzing heterogeneous UV-Fenton system for tetracycline removal with a focus on optimization by a response surface method. J. Photochem. Photobiol. A. 314 (2015), 178–188.
11. [11] Wu, H.H., Jiang, F.F., Lu, S.Y., Guan, Y.F., Deng, D.Y., Chen, X.L., Using goethite as a heterogeneous Fenton catalyst for the removal of tetracycline hydrochloride: effects of its adsorptive and reductive activities. Dong, F.Q., (eds.) Proceedings of the 11th International Congress for Applied Mineralogy (ICAM), 2015, Springer International Publishing, Switzerland, 405–423.
12. 2 advanced oxidation process. Iran. J. Environ. Health 12 (2014), 1–8.
13. 2, oxidation processes. J. Chem. Technol. Biot. 85 (2010), 1325–1333.
14. [14] Wang, Y., Zhang, H., Chen, L., Ultrasound enhanced catalytic ozonation of tetracycline in a rectangular air-lift reactor. Catal. Today. 175 (2011), 283–292.
15. [15] Lemke, T.L., Williams, D.A., Foye's Principles of Medicinal Chemistry. 6th ed., 2008.
16. [16] Hopkins, Z.R., Blaney, L., A novel approach to modeling the reaction kinetics of tetracycline antibiotics with aqueous ozone. Sci. Total. Environ. 468–469 (2014), 337–344.
17. [17] Palominos, R., Freer, J., Mondaca, M.A., Mansilla, H.D., Evidence for hole participation during the photocatalytic oxidation of the antibiotic flumequine. J. Photochem. Photobiol. A. 193 (2008), 139–145.
18. [18] Liu, Y.Q., He, X.X., Fu, Y.S., Dionysiou, D.D., Kinetics and mechanism investigation on the destruction of oxytetracycline by UV-254 nm activation of persulfate. J. Hazard. Mater. 305 (2016), 229–239.
19. 3 photocatalysis of tetracycline: kinetics, mechanisms and toxicity assessment. Chemosphere 93 (2013), 1–8.
20. [20] Ji, Y.F., Shi, Y.Y., Dong, W., Wen, X., Jiang, M.D., Lu, J.H., Thermo-activated persulfate oxidation system for tetracycline antibiotics degradation in aqueous solution. Chem. Eng. J. 298 (2016), 225–233.
21. [21] Niu, J.F., Li, Y., Wang, W.L., Light-source-dependent role of nitrate and humic acid in tetracycline photolysis: kinetics and mechanism. Chemosphere 92 (2013), 1423–1429.
22. [22] Wan, Y., Jia, A., Zhu, Z., Hu, J.Y., Transformation of tetracycline during chloramination: kinetics, products and pathways. Chemosphere 90 (2013), 1427–1434.
23. [23] Halling-Sørensen, B., Sengeløv, G., Tjørnelund, J., Toxicity of tetracyclines and tetracycline degradation products to environmentally relevant bacteria, including selected tetracycline-resistant bacteria. Arch. Environ. Contam. Toxicol. 42 (2002), 263–271.
24. [24] Dalmázio, I., Almeida, M.O., Augusti, R., Alves, T.M.A., Monitoring the degradation of tetracycline by ozone in aqueous medium via atmospheric pressure ionization mass spectrometry. J. Am. Soc. Mass. Spectrom. 18 (2007), 679–687.
25. [25] Khan, M.H., Bae, H., Jung, J.Y., Tetracycline degradation by ozonation in the aqueous phase: proposed degradation intermediates and pathway. J. Hazard. Mater. 181 (2010), 659–665.
26. [26] Cao, M.H., Wang, P.F., Ao, Y.H., Wang, C., Hou, J., Qian, J., Visible light activated photocatalytic degradation of tetracycline by a magnetically separable composite photocatalyst: graphene oxide/magnetite/cerium-doped titania. J. Colloid Interface Sci. 467 (2016), 129–139.
27. 2. Chem. Eng. J. 258 (2014), 18–25.