Kinetics and pathways of ibuprofen degradation by the UV/chlorine advanced oxidation process

Water Research

Volumn 90, Issue , 2016, Pages 301-308

  Xiang, Yingying ^a,b   Fang, Jingyun ^a   Shang, Chii ^b,c  

^a SUN YAT SEN UNIVERSITY   (China)

^b HONG KONG UNIVERSITY OF SCIENCE AND TECHNOLOGY   (Hong Kong)

^c Hong Kong Fire Services Department   (Hong Kong)

Author keywords

Chlorine atoms; Hydroxyl radicals; Ibuprofen; Pharmaceutical and personal care products (PPCPs); UV chlorine advanced oxidation process; Water treatment

Indexed keywords

CARBOXYLATION; KINETICS; OXIDATION; POTABLE WATER; RATE CONSTANTS; WATER TREATMENT;

ADVANCED OXIDATION PROCESSES; CHLORINE ATOM; FIRST-ORDER RATE CONSTANTS; HYDROXYL RADICALS; IBUPROFEN; ORGANIC CHLORINE; PHARMACEUTICAL AND PERSONAL CARE PRODUCT; PHARMACEUTICAL AND PERSONAL CARE PRODUCTS; REACTIVE SPECIES; UV/CHLORINE ADVANCED OXIDATION PROCESS;

CHLORINE;

CHLORINE; DRINKING WATER; HYDROGEN PEROXIDE; HYDROXYL RADICAL; IBUPROFEN; PIRENZEPINE; REACTIVE CHLORINE SPECIES; UNCLASSIFIED DRUG; OXYGEN; WATER POLLUTANT;

CHLORINE; CONCENTRATION (COMPOSITION); DEGRADATION; DRUG; HYDROXYL RADICAL; OXIDATION; PPCP; REACTION KINETICS; ULTRAVIOLET RADIATION; WATER TREATMENT;

ADVANCED OXIDATION PROCESS; ARTICLE; CHLORINATION; CONTROLLED STUDY; DECARBOXYLATION; DEGRADATION KINETICS; DEMETHYLATION; DRUG DEGRADATION; HYDROXYLATION; OXIDATION; PRIORITY JOURNAL; ULTRAVIOLET RADIATION; ANALYSIS; CHEMISTRY; DISINFECTION; HALOGENATION; KINETICS; PH; PHOTOCHEMISTRY; PROCEDURES; SEWAGE; TEMPERATURE; WATER MANAGEMENT; WATER POLLUTANT;

CHLORINE; DISINFECTION; DRINKING WATER; HALOGENATION; HYDROGEN PEROXIDE; HYDROGEN-ION CONCENTRATION; HYDROXYL RADICAL; IBUPROFEN; KINETICS; OXYGEN; PHOTOCHEMISTRY; TEMPERATURE; ULTRAVIOLET RAYS; WASTE DISPOSAL, FLUID; WATER POLLUTANTS, CHEMICAL; WATER PURIFICATION;

EID: 84952683767     PISSN: 00431354     EISSN: 18792448     Source Type: Journal    
DOI: 10.1016/j.watres.2015.11.069     Document Type: Article

References (42)

1. Barakat M.A., Tseng J.M., Huang C.P. Hydrogen peroxide-assisted photocatalytic oxidation of phenolic compounds. Appl. Catal. B Environ. 2005, 59(1-2):99-104.
2. Beitz T., Bechmann W., Mitzner R. Investigations of reactions of selected azaarenes with radicals in water. 2. Chlorine and bromine radicals. J. Phys. Chem. A 1998, 102(34):6766-6771.
3. Bolton J.R., Linden K.G. Standardization of methods for fluence (UV Dose) determination in bench-scale UV experiments. J. Environ. Eng. 2003, 129(3):209-215.
4. 2 in aqueous solution up to 200 °C. A pulse radiolysis study. J. Chem. Soc. Faraday Trans. 1 1988, 84(4):1113-1121.
5. Christen V., Hickmann S., Rechenberg B., Fent K. Highly active human pharmaceuticals in aquatic systems: a concept for their identification based on their mode of action. Aquat. Toxicol. 2010, 96(3):167-181.
6. 2/UV process in a completely mixed batch reactor. Water Res. 1999, 33(10):2315-2328.
7. Da Silva J.C.C., Teodoro J.A.R., Afonso R.J.D.C., Aquino S.F., Augusti R. Photolysis and photocatalysis of ibuprofen in aqueous medium: characterization of by-products via liquid chromatography coupled to high-resolution mass spectrometry and assessment of their toxicities against Artemia Salina. J. Mass Spectrom. 2014, 49(2):145-153.
8. Deng Z., Yang X., Shang C., Zhang X. Electrospray ionization-tandem mass spectrometry method for differentiating chlorine substitution in disinfection byproduct formation. Environ. Sci. Technol. 2014, 48(9):4877-4884.
9. Fang J., Fu Y., Shang C. The roles of reactive species in micropollutant degradation in the UV/free chlorine system. Environ. Sci. Technol. 2014, 48(3):1859-1868.
10. -) with 254 nm ultraviolet light. J. Environ. Eng. Sci. 2007, 6(3):277-284.
11. Garoma T., Gurol M.D. Modeling aqueous ozone/UV process using oxalic acid as probe chemical. Environ. Sci. Technol. 2005, 39(20):7964-7969.
12. Grebel J.E., Pignatello J.J., Mitch W.A. Effect of halide ions and carbonates on organic contaminant degradation by hydroxyl radical-based advanced oxidation processes in saline waters. Environ. Sci. Technol. 2010, 44(17):6822-6828.
13. - and Cl in aqueous solution. PCCP 2007, 9(30):3935-3964.
14. 2 and some ions. Langmuir 2002, 18(8):3247-3254.
15. Huerta-Fontela M., Galceran M.T., Ventura F. Occurrence and removal of pharmaceuticals and hormones through drinking water treatment. Water Res. 2011, 45(3):1432-1442.
16. Jin J., El-Din M.G., Bolton J.R. Assessment of the UV/Chlorine process as an advanced oxidation process. Water Res. 2011, 45(4):1890-1896.
17. 2. Water Res. 2011, 45(13):3811-3822.
18. 4 titration. Anal. Chem. 1994, 66(18):2921-2925.
19. Lee Y., von Gunten U. Oxidative transformation of micropollutants during municipal wastewater treatment: comparison of kinetic aspects of selective (chlorine, chlorine dioxide, ferrateVI, and ozone) and non-selective oxidants (hydroxyl radical). Water Res. 2010, 44(2):555-566.
20. Li X., Wang Y., Yuan S., Li Z., Wang B., Huang J., Deng S., Yu G. Degradation of the anti-inflammatory drug ibuprofen by electro-peroxone process. Water Res. 2014, 63:81-93.
21. Mack J., Bolton J.R. Photochemistry of nitrite and nitrate in aqueous solution: a review. J. Photochem. Photobiol. A Chem. 1999, 128(1-3):1-13.
22. Madhavan J., Grieser F., Ashokkumar M. Combined advanced oxidation processes for the synergistic degradation of ibuprofen in aqueous environments. J. Hazard. Mater 2010, 178(1-3):202-208.
23. 2 and simulated solar irradiation. Water Res. 2008, 42(3):585-594.
24. Nowell L.H., Hoigné J. Photolysis of aqueous chlorine at sunlight and ultraviolet wavelengths-II. Hydroxyl radical production. Water Res. 1992, 26(5):599-605.
25. Pinkston K.E., Sedlak D.L. Transformation of aromatic ether- and amine-containing pharmaceuticals during chlorine disinfection. Environ. Sci. Technol. 2004, 38(14):4019-4025.
26. Plewa M.J., Wagner E.D., Metz D.H., Kashinkunti R., Jamriska K.J., Meyer M. Differential toxicity of drinking water disinfected with combinations of ultraviolet radiation and chlorine. Environ. Sci. Technol. 2012, 46(14):7811-7817.
27. Rao B., Estrada N., McGee S., Mangold J., Gu B., Jackson W.A. Perchlorate production by photodecomposition of aqueous chlorine solutions. Environ. Sci. Technol. 2012, 46(21):11635-11643.
28. Rosenfeldt E.J., Linden K.G. Degradation of endocrine disrupting chemicals bisphenol A, ethinyl estradiol, and estradiol during UV photolysis and advanced oxidation processes. Environ. Sci. Technol. 2004, 38(20):5476-5483.
29. Rosenfeldt E., Boal A.K., Springer J., Stanford B., Rivera S., Kashinkunti R.D., Metz D.H. Comparison of UV-mediated advanced oxidation. J. Am. Water Works Assoc. 2013, 105(7):29-33.
30. Ruggeri G., Ghigo G., Maurino V., Minero C., Vione D. Photochemical transformation of ibuprofen into harmful 4-isobutylacetophenone: pathways, kinetics, and significance for surface waters. Water Res. 2013, 47(16):6109-6121.
31. Shu Z., Li C., Belosevic M., Bolton J.R., El-Din M.G. Application of a solar UV/chlorine advanced oxidation process to oil sands process-affected water remediation. Environ. Sci. Technol. 2014, 48(16):9692-9701.
32. Sichel C., Garcia C., Andre K. Feasibility studies: UV/chlorine advanced oxidation treatment for the removal of emerging contaminants. Water Res. 2011, 45(19):6371-6380.
33. USEPA Standard Methods for the Examination of Water and Wastewater 1998, American Public Health Assoc, Washington. DC. USA. 20th ed.
34. Vione D., Maddigapu P.R., De Laurentiis E., Minella M., Pazzi M., Maurino V., Minero C., Kouras S., Richard C. Modelling the photochemical fate of ibuprofen in surface waters. Water Res. 2011, 45(20):6725-6736.
35. Vieno N.M., Härkki H., Tuhkanen T., Kronberg L. Occurrence of pharmaceuticals in river water and their elimination in a pilot-scale drinking water treatment plant. Environ. Sci. Technol 2007, 41(14):5077-5084.
36. Wang D., Bolton J.R., Hofmann R. Medium pressure UV combined with chlorine advanced oxidation for trichloroethylene destruction in a model water. Water Res. 2012, 46(15):4677-4686.
37. Watts M.J., Linden K.G. Chlorine photolysis and subsequent OH radical production during UV treatment of chlorinated water. Water Res 2007, 41(13):2871-2878.
38. 2 processes. J. Water Supply Res. T 2007, 56(8):469-477.
39. 2. Water Res. 2013, 47(15):5876-5888.
40. 2. Water Res. 2009, 43(6):1766-1774.
41. Zhai H., Zhang X. A new method for differentiating adducts of common drinking water DBPs from higher molecular weight DBPs in electrospray ionization-mass spectrometry analysis. Water Res. 2009, 43(8):2093-2100.
42. Zhao Q., Shang C., Zhang X., Ding G., Yang X. Formation of halogenated organic byproducts during medium-pressure UV and chlorine coexposure of model compounds, NOM and bromide. Water Res. 2011, 45(19):6545-6554.