Surface-Enhanced Spectroscopy for Higher-Order Light Scattering: A Combined Experimental and Theoretical Study of Second Hyper-Raman Scattering

Journal of Physical Chemistry Letters

Volumn 6, Issue 24, 2015, Pages 5067-5071

  Simmons, Philip D ^a   Turley, Hubert K ^b   Silverstein, Daniel W ^c   Jensen, Lasse ^c   Camden, Jon P ^b  

^a UNIVERSITY OF TENNESSEE   (United States)

^b UNIVERSITY OF NOTRE DAME   (United States)

^c PENNSYLVANIA STATE UNIVERSITY   (United States)

Author keywords

first principles theory; nonlinear spectroscopy; surface enhanced Raman scattering

Indexed keywords

CALCULATIONS; LIGHT SCATTERING; RAMAN SCATTERING;

FIRST-PRINCIPLES CALCULATION; FIRST-PRINCIPLES THEORY; NON-LINEAR PHENOMENA; NONLINEAR SPECTROSCOPY; QUANTITATIVE AGREEMENT; SURFACE ENHANCED RAMAN SCATTERING (SERS); SURFACE ENHANCED SPECTROSCOPY; THEORETICAL FRAMEWORK;

SURFACE SCATTERING;

EID: 84951859078     PISSN: None     EISSN: 19487185     Source Type: Journal    
DOI: 10.1021/acs.jpclett.5b02342     Document Type: Article

References (22)

1. Yu, J. H.; Kwon, S.-H.; Petrášek, Z.; Park, O. K.; Jun, S. W.; Shin, K.; Choi, M.; Park, Y. I.; Park, K.; Na, H. B. et al. High-Resolution Three-Photon Biomedical Imaging Using Doped Zns Nanocrystals Nat. Mater. 2013, 12, 359-366 10.1038/nmat3565
2. Hales, J. M.; Matichak, J.; Barlow, S.; Ohira, S.; Yesudas, K.; Brédas, J.-L.; Perry, J. W.; Marder, S. R. Design of Polymethine Dyes with Large Third-Order Optical Nonlinearities and Loss Figures of Merit Science 2010, 327, 1485-1488 10.1126/science.1185117
3. Iliopoulos, K.; Krupka, O.; Gindre, D.; Sallé, M. Reversible Two-Photon Optical Data Storage in Coumarin-Based Copolymers J. Am. Chem. Soc. 2010, 132, 14343-14345 10.1021/ja1047285
4. Samoc, M.; Morrall, J. P.; Dalton, G. T.; Cifuentes, M. P.; Humphrey, M. G. Two-Photon and Three-Photon Absorption in an Organometallic Dendrimer Angew. Chem. 2007, 119, 745-747 10.1002/ange.200602341
5. Milojevich, C. B.; Mandrell, B. K.; Turley, H. K.; Iberi, V.; Best, M. D.; Camden, J. P. Surface-Enhanced Hyper-Raman Scattering from Single Molecules J. Phys. Chem. Lett. 2013, 4, 3420-3423 10.1021/jz4017415
6. Zhang, Y.; Zhen, Y.-R.; Neumann, O.; Day, J. K.; Nordlander, P.; Halas, N. J. Coherent Anti-Stokes Raman Scattering with Single-Molecule Sensitivity Using a Plasmonic Fano Resonance Nat. Commun. 2014, 5, 4424 10.1038/ncomms5424
7. Roke, S.; Gonella, G. Nonlinear Light Scattering and Spectroscopy of Particles and Droplets in Liquids Annu. Rev. Phys. Chem. 2012, 63, 353-378 10.1146/annurev-physchem-032511-143748
8. Boyd, R. W. Nonlinear Optics, 3rd ed.; Academic Press: Burlington, MA, 2008.
9. Terhune, R.; Maker, P.; Savage, C. Measurements of Nonlinear Light Scattering Phys. Rev. Lett. 1965, 14, 681-684 10.1103/PhysRevLett.14.681
10. Long, D. A.; Stanton, L. Studies of Nonlinear Phenomena 1. Theory of Hyper Raman Effect Proc. R. Soc. London, Ser. A 1970, 318, 441-457 10.1098/rspa.1970.0153
11. Milojevich, C. B.; Silverstein, D. W.; Jensen, L.; Camden, J. P. Probing One-Photon Inaccessible Electronic States with High Sensitivity: Wavelength Scanned Surface Enhanced Hyper-Raman Scattering ChemPhysChem 2011, 12, 101-103 10.1002/cphc.201000868
12. Milojevich, C. B.; Silverstein, D. W.; Jensen, L.; Camden, J. P. Probing Two-Photon Properties of Molecules: Large Non-Condon Effects Dominate the Resonance Hyper-Raman Scattering of Rhodamine 6g J. Am. Chem. Soc. 2011, 133, 14590-14592 10.1021/ja2054622
13. Milojevich, C. B.; Silverstein, D. W.; Jensen, L.; Camden, J. P. Surface-Enhanced Hyper-Raman Scattering Elucidates the Two-Photon Absorption Spectrum of Rhodamine 6g J. Phys. Chem. C 2013, 117, 3046-3054 10.1021/jp3094098
14. Silverstein, D. W.; Milojevich, C. B.; Camden, J. P.; Jensen, L. Investigation of Linear and Nonlinear Raman Scattering for Isotopologues of Ru(Bpy)(3)(2+) J. Phys. Chem. C 2013, 117, 20855-20866 10.1021/jp4070505
15. Golab, J. T.; Sprague, J. R.; Carron, K. T.; Schatz, G. C.; Vanduyne, R. P. A Surface Enhanced Hyper-Raman Scattering Study of Pyridine Adsorbed onto Silver-Experiment and Theory J. Chem. Phys. 1988, 88, 7942-7951 10.1063/1.454251
16. Turley, H. K.; Camden, J. P. A Nonlinear Approach to Surface-Enhanced Sensing in the Short-Wave Infrared Chem. Commun. 2014, 50, 1472-1474 10.1039/C3CC49002E
17. Johnson, P. B.; Christy, R. W. Optical Constants of the Noble Metals Phys. Rev. B 1972, 6, 4370-4379 10.1103/PhysRevB.6.4370
18. Lee, P. C.; Meisel, D. Adsorption and Surface-Enhanced Raman of Dyes on Silver and Gold Sols J. Phys. Chem. 1982, 86, 3391-3395 10.1021/j100214a025
19. Valiev, M.; Bylaska, E. J.; Govind, N.; Kowalski, K.; Straatsma, T. P.; Van Dam, H. J. J.; Wang, D.; Nieplocha, J.; Apra, E.; Windus, T. L. et al. Nwchem: A Comprehensive and Scalable Open-Source Solution for Large Scale Molecular Simulations Comput. Phys. Commun. 2010, 181, 1477-1489 10.1016/j.cpc.2010.04.018
20. Aidas, K.; Angeli, C.; Bak, K. L.; Bakken, V.; Bast, R.; Boman, L.; Christiansen, O.; Cimiraglia, R.; Coriani, S.; Dahle, P. et al. The Dalton Quantum Chemistry Program System WIREs Comput. Mol. Sci. 2014, 4, 269-284 10.1002/wcms.1172
21. Silverstein, D. W.; Jensen, L. Vibronic Coupling Simulations for Linear and Nonlinear Optical Processes: Theory J. Chem. Phys. 2012, 136, 064111 10.1063/1.3684236
22. Silverstein, D.; Jensen, L. Tdspec: Time-Dependent Spectroscopic Simulations of Linear and Nonlinear Optical Processes; The Pennsylvania State University: University Park, PA, 2011.