Solvent-free selective oxidation of benzyl alcohol to benzaldehyde catalyzed by zinc mono-substituted phosphotungstic acid quaternary ammonium salt

Journal of Molecular Catalysis

Volumn 28, Issue 6, 2014, Pages 515-523

  Li, Gui Xian ^a   Bai, Hong Wei ^a   Ji, Dong ^a   Wei, Hui Juan ^a   Cao, Yan Wei ^a   Zhang, Yi Xin ^a  

^a LANZHOU UNIVERSITY OF TECHNOLOGY   (China)

Author keywords

Benzyl alcohol; Phosphotungstic acid quaternary ammonium salt; Solvent free oxidation; Transition metal Zn

Indexed keywords

CATALYST SELECTIVITY; CATALYTIC OXIDATION; FOURIER SERIES; FOURIER TRANSFORM INFRARED SPECTROSCOPY; OXIDATION; SALTS; SOLVENTS; TRANSITION METAL COMPOUNDS; TRANSITION METALS; ZINC; ZINC METALLOGRAPHY;

BENZYL ALCOHOL; FOURIER TRANSFORM INFRARED; PHOSPHOTUNGSTIC ACID; QUATERNARY AMMONIUM SALT; REACTION PARAMETERS; SELECTIVE OXIDATION; SOLVENT FREE CONDITIONS; SOLVENT-FREE OXIDATION;

CATALYST ACTIVITY;

EID: 84921856748     PISSN: 10013555     EISSN: None     Source Type: Journal    
DOI: None     Document Type: Article

References (38)

1. Farsani M R, Jalilian F, Yadollahi B, et al. A comparative study on Keggin and Wells-Dawson sandwich type polyoxometallates in the oxidation of alcohols with 30% hydrogen peroxide[J]. Polyhedron, 2014, 76: 102-107.
2. Zhan Guo-wu, Hong Ying-ling, Lu Fen-fen, et al. Kinetics of liquid phase oxidation of benzyl alcohol with hydrogen peroxide over bio-reduced Au/TS-1 catalysts[J]. J Mol Catal A: Chem, 2013, 366: 215-221.
3. 2/pyridine complex catalytic oxidation of benzylic compounds and alcohols with molecular oxygen[J]. J Mol Catal(China), 2012, 26(1): 19-25.
4. Yang Wei-jun, Zhang Lei, Li Yong-jin, et al. Effect of phenyl Cl substituent position on the catalytic performance for olefin epoxidation of tetraphenyl metalloporphyrins[J]. J Mol Catal(China), 2012, 26(4): 314-321.
5. García-Suárez E J, Tristany M, García A B, et al. Carbon-supported Ru and Pd nanoparticles: Efficient and recyclable catalysts for the aerobic oxidation of benzyl alcohol in water[J]. Micro Mes Mat, 2012, 153: 155-162.
6. Kong Xiang-guo, Hu Bo, Zhuo Guang-lan, et al. The selective oxidation of styrene to benzaldehyde by modified VPO catalyst[J]. J Mol Catal(China), 2012, 27(1): 23-29.
7. Li Yan-fei, Gao Bao-jiao, Yu Yi-ling, et al. Preparation of N,N-bidentate schiff Bare-type oxovanadium(IV) complex immobilized on CPS micropheres andcatalytic property in oxidation of ethylbenzene by molecular oxygen[J]. J Mol Catal(China), 2013, 27(3): 271-278.
8. Zhang Cheng-ming, Sun Kun-peng, Xu Xian-lun. Preparation of CuMn-containing hydrotalcites and it's solvent-free catalytic oxidation of benzyl alcohol[J]. J Mol Catal(China), 2010, 24(4): 304-308.
9. Wang Fang, Liu Jun-hua, Li Wei-min, et al. One-pot synthesis of Au-silica catalysts and their catalytic performance over styrene epoxidation[J]. J Mol Catal(China), 2013, 27(4): 333-341.
10. Qiang Bin, Kong Xiang-guo, Zhuo Guang-lan, et al. Selective oxidation of styrene to berzaldehyde over supported VPO catalyst[J]. J Mol Catal(China), 2013, 27(6): 522-529.
11. 2 in alkaline medium for selective oxidation of alcohol[J]. Micro Mes Mat, 2007, 101(1/2): 256-263.
12. Tong Xin-li, Sun Yong-fa, Yan Yong-tao, et al. Transition metal-free catalytic oxidation of aromatic alcohols with molecular oxygen in the presence of a catalytic amount of N-bromosuccinimide[J]. J Mol Catal A: Chem, 2014, 391: 1-6.
13. Yu Yi-ling, Gao Bao-jiao, Li Yan-fei, et al. Catalytic property of co-catalyst of TEMPO/immobilized Schiff base copper complex in oxidation of benzyl alcohol by molecular oxygen[J]. J Mol Catal(China), 2014, 28(3): 210-217.
14. Wang Xiao-li, Wu Gong-de, Ding Ke-qiang, et al. Selective oxidation of benzyl alcohol over the immobilized Schiff base complex: effect of preparation parameters on its structure and catalytic performance[J]. J Mol Catal(China), 2011, 25(4): 308-315.
15. 2/TEMPO/piperidine) for the oxidation of primary benzylic alcohols to aldehydes by oxygen[J]. J Mol Catal(China), 2014, 28(4): 317-328.
16. Wang De-sheng, Yan Liang, Wang Xiao-lai. A research progress of heteropolya- cids catalyst[J]. J Mol Catal(China), 2012, 26(4): 366-375.
17. Li Gui-xian, Ding Yong, Wang Jian-ming, et al. New progress of Keggin and Wells-Dawson type polyoxometalates catalyze acid and oxidative reactions[J]. J Mol Catal A: Chem, 2007, 262(1/2): 67-76.
18. Simões M M, Santos I C, Balula M S S, et al. Oxidation of cycloalkanes with hydrogen peroxide in the presence of Keggin-type polyoxotungstates[J]. Catal Today, 2004, 91/92: 211-214.
19. Pope M T, Müller A. Polyoxometalate chemistry: An old field with new dimensions in several disciplines[J]. Angew Chem Inter Ed Eng, 1991, 30(1): 34-48.
20. Leng Yi-xin, Gao Zai-ling, Su Ji-guang. Synthesis of maleic anhydride by oxidizing furfural over phosphorusmolybdenumic acid supported on silica gel[J]. J Mol Catal(China), 2012, 26(3): 246-251.
21. Zhao Mei-ting, Zhou Jian-wei, Li Zhen, et al. Polyoxometalates based supported ionic liquid catalysis for alcohol oxidation with hydrogen peroxide [J]. J Mol Catal(China), 2011, 25(2): 97-104.
22. Nadealian Z, Mirkhani V, Yadollahi B, et al. Selective oxidation of alcohols to aldehydes using inorganic-organic hybrid catalyst based on zinc substituted polyoxometalate and ionic liquid[J]. J Coord Chem, 2012, 65(6): 1071-1081.
23. Wang Jian-min, Yan Liang, Li Gui-xian, et al. Mono-substituted Keggin-polyoxometalate complexes as effective and recyclable catalyst for the oxidation of alcohols with hydrogen peroxide in biphasic system[J]. Tetra Lett, 2005, 46(41): 7023-7027.
24. Jing Li, Shi Jing, Zhang Fu-min, et al. Polyoxometalate-based amphiphilic catalysts for selective oxidation of benzyl alcohol with hydrogen peroxide under organic solvent-free conditions[J]. Ind Eng Chem Res, 2013, 52(30): 10095-10104.
25. Pathan S, Patel A. Solvent free clean selective oxidation of alcohols catalyzed by mono transition metal (Co, Mn, Ni)-substituted Keggin-phosphomolybdates using hydrogen peroxide[J]. Appl Catal A: Gen, 2013, 459: 59-64.
26. Weakley T, Malik S. Heteropolyanions containing two different heteroatoms-I[J]. Inorg Nucl Chem, 1967, 29(12): 2935-2944.
27. Tourné C M, Tourné G F, Malik S, et al. Triheteropolyanions containing copper (II), manganese (II), or manganese (III)[J]. Inorg Nucl Chem, 1970, 32(12): 3875-3890.
28. Ma Jian-wei, Ye Xing-kai, Wu Yue. Study on the catalytic property of heteropoly compound[J]. Chin J Catal, 1991, 12(6): 443-450.
29. 11Z[J]. J Fuel Chem Technol, 2001, 29: 205-207.
30. Varadwaj G, Rana S, Parida K. Cs salt of Co substituted lacunary phosphotungstate supported K10 montmorillonite showing binary catalytic activity [J]. Chem Eng J, 2013, 215/216: 849-858.
31. 11 heteropolyanion[J]. Chem J Chin U, 1994, 15(5): 642-645.
32. Yan Xue-hai, Zhu Peng-li, Fei Jin-bo, et al. Self-Assembly of peptide-inorganic hybrid spheres for adaptive encapsulation of guests[J]. Adv Mater, 2010, 22(11): 1283-1287.
33. Misono M. Unique acid catalysis of heteropoly compounds (heteropolyoxometalates) in the solid state[J]. Chem Comm, 2001, 2001(13): 1141-1152.
34. 2[J]. J Mol Catal A: Chem, 2012, 358: 67-72.
35. Pathan S, Patel A. Keggin type transition metal substituted phosphomolybdates: heterogeneous catalysts for selective aerobic oxidation of alcohols and alkenes under solvent free condition [J]. Catal Sci Technol, 2014, 4(3): 648-656.
36. Lin Xin-rong, Xu Jin-yu, Liu Hui-zhang, et al. Studies on styrene oxidation reaction catalyzed by ruthenium substituted polyoxotungstates: Kinetics and phase transfer effect[J]. J Mol Catal A: Chem, 2000, 161(1/2): 163-169.
37. Patel A, Patel K. Cs salt of di-manganese (II) substituted phosphotungstate: One pot synthesis, structural, spectroscopic characterization and solvent free liquid phase oxidation of styrene using different oxidants[J].Polyhedron, 2014, 69: 110-118.
38. Chaudhari M P, Sawant S B. Kinetics of heterogeneous oxidation of benzyl alcohol with hydrogen peroxide[J]. Chem Eng J, 2005, 106(2): 111-118.