Catalytic wet air oxidation of phenol with functionalized carbon materials as catalysts: Reaction mechanism and pathway

Journal of Environmental Sciences (China)

Volumn 26, Issue 8, 2014, Pages 1741-1749

  Wang, Jianbing ^a   Fu, Wantao ^a   He, Xuwen ^a   Yang, Shaoxia ^b   Zhu, Wanpeng ^b  

^a CHINA UNIVERSITY OF MINING AND TECHNOLOGY   (China)

^b TSINGHUA UNIVERSITY   (China)

Author keywords

Carbon materials; Catalytic wet air oxidation; Phenol; Radical; Reaction pathway

Indexed keywords

CARBON DIOXIDE; CARBOXYLIC ACIDS; CATALYST ACTIVITY; CATALYTIC OXIDATION; FREE RADICALS; OXIDATION; PHENOLS; REACTION INTERMEDIATES;

CARBON MATERIAL; CARBOXYLIC ACID GROUPS; CATALYTIC WET AIR OXIDATION; RADICAL; REACTION CONDITIONS; REACTION MECHANISM; REACTION PATHWAYS; STRONG OXIDANTS;

CARBON;

CARBOXYLIC ACID; CATALYST; FORMIC ACID; FREE RADICAL; OXALIC ACID; OXIDATION; PHENOL; REACTION RATE;

CARBON; PHENOL; RADICAL; WATER;

AIR; ARTICLE; CARBON MATERIALS; CATALYSIS; CATALYTIC WET AIR OXIDATION; CHEMICAL STRUCTURE; CHEMISTRY; OXIDATION REDUCTION REACTION; REACTION ANALYSIS; WATER POLLUTANT;

CARBON MATERIALS; CATALYTIC WET AIR OXIDATION; PHENOL; RADICAL; REACTION PATHWAY;

AIR; CARBON; CATALYSIS; MOLECULAR STRUCTURE; OXIDATION-REDUCTION; PHENOL; WATER; WATER POLLUTANTS, CHEMICAL;

EID: 84908108370     PISSN: 10010742     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.jes.2014.06.015     Document Type: Article

References (34)

1. Barbier J., Delanoë F., Jabouille F., Duprez D., Blanchard G., Isnard P. Total oxidation of acetic acid in aqueous solution over noble metal catalysts. J. Catal. 1998, 177(2):378-385.
2. Boehm H.P. Surface oxides on carbon and their analysis: a critical assessment. Carbon 2002, 40(2):145-149.
3. Dandekar A., Baker R.T.K., Vannice M.A. Characterization of activated carbon, graphitized carbon fibers and synthetic diamond powder using TPD and DRIFTS. Carbon 1998, 36(12):1821-1831.
4. Duprez D., Delanoe F., Barbier J., Isnard P., Blanchard G. Catalytic oxidation of organic compounds in aqueous media. Catal. Today 1996, 29(1-4):317-322.
5. Fortuny A., Bengoa C., Font J., Fabregat A. Bimetallic catalysts for continuous catalytic wet air oxidation of phenol. J. Hazard. Mater. 1999, 64(2):181-193.
6. Gallezot P., Chaumet S., Perrard A., Isnard P. Catalytic wet air oxidation of acetic acid on carbon-supported ruthenium catalysts. Catal. Today 1997, 168(1):104-109.
7. Huang S.Y., Zhang C.B., He H. In situ adsorption-catalysis system for the removal of o-xylene over an activated carbon supported Pd catalyst. J. Environ. Sci. 2009, 21(7):985-990.
8. Kim U.J., Furtado C.A., Liu X.M., Chen G.G., Eklund P.C. Raman and IR spectroscopy of chemically processed single-walled carbon nanotubes. J. Am. Chem. Soc. 2005, 127(44):15437-15445.
9. Kim S.K., Kim K.H., Ihm S.K. The characteristics of wet air oxidation of phenol over CuOx/Al2O3 catalysts: effect of copper loading. Chemosphere 2007, 68(2):287-292.
10. Kouklin N., Tzolov M., Straus D., Yin A., Xu J.M. Infrared absorption properties of carbon nanotubes synthesized by chemical vapor deposition. Appl. Phys. Lett. 2004, 85(19):4463-4465.
11. Li N., Descorme C., Besson M. Catalytic wet air oxidation of 2-chlorophenol over Ru loaded CexZr1-xO2 solid solutions. Appl. Catal. B Environ. 2007, 76(1-2):92-100.
12. Liu Y., Sun D.Z., Cheng L., Li Y.P. Preparation and characterization of Fe2O3-CeO2-TiO2/γ-A12O3 catalyst for degradation dye wastewater. J. Environ. Sci. 2006, 18(6):1189-1192.
13. Liu Z.Q., Ma J., Cui Y.H. Carbon nanotube supported platinum catalysts for the ozonation of oxalic acid in aqueous solutions. Carbon 2008, 46(6):890-897.
14. Liu Z.Q., Ma J., Cui Y.H., Zhao L., Zhang B.P. Factors affecting the catalytic activity of multi-walled carbon nanotube for ozonation of oxalic acid. Sep. Purif. Technol. 2011, 78(2):147-153.
15. Liu X.T., Wang M.S., Zhang S.J., Pan B.C. Application potential of carbon nanotubes in water treatment: a review. J. Environ. Sci. 2013, 25(7):1263-1280.
16. Luck F. Wet air oxidation: past, present and future. Catal. Today 1999, 53(1):81-91.
17. Morales-Torres S., Silva A.M.T., Pérez-Cadenas A.F., Faria J.L., Maldonado-Hódar F.J., Figueiredo J.L., et al. Wet air oxidation of trinitrophenol with activated carbon catalysts: effect of textural properties on the mechanism of degradation. Appl. Catal. B Environ. 2010, 100(1-2):310-317.
18. Pyun J. Graphene oxide as catalyst: application of carbon materials beyond nanotechnology. Angew. Chem. Int. Ed. 2011, 50(1):46-48.
19. Rivas F.J., Kolaczkowski S.T., Beltrán F.J., McLurgh D.B. Development of a model for the wet air oxidation of phenol based on a free radical mechanism. Chem. Eng. Sci. 1998, 53(14):2575-2586.
20. Santiago M., Stüber F., Fortuny A., Fabregat A., Font J. Modified activated carbons for catalytic wet air oxidation of phenol. Carbon 2005, 43(10):2134-2145.
21. Santos A., Yustos P., Quintanilla A., Rodriguez S., Garcia-Ochoa F. Route of the catalytic oxidation of phenol in aqueous phase. Appl. Catal. B Environ. 2002, 39(2):97-113.
22. Serp P., Corrias M., Kalck P. Carbon nanotubes and nanofibers in catalysis. Appl. Catal. A Gen. 2003, 253(2):337-358.
23. Soria-Sánchez M., Maroto-Valiente A., Álvarez-Rodríguez J., Muñoz-Andrés V., Rodríguez-Ramos I., Guerrero-Ruíz A. Carbon nanostructured materials as direct catalysts for phenol oxidation in aqueous phase. Appl. Catal. B Environ. 2011, 104(1-2):101-109.
24. Stuber F., Font J., Fortuny A., Bengoa C., Eftaxias A., Fabregat A. Carbon materials and catalytic wet air oxidation of organic pollutants in wastewater. Top. Catal. 2005, 45(1-4):3-50.
25. Suarez-Ojeda M.E., Stüber F., Fortuny A., Fabregat A., Carrera J., Font J. Catalytic wet air oxidation of substituted phenols using activated carbon as catalyst. Appl. Catal. B Environ. 2005, 58(1-2):105-114.
26. Suarez-Ojeda M.E., Fabregat A., Stüber F., Fortuny A., Carrera J., Font J. Catalytic wet air oxidation of substituted phenols: temperature and pressure effect on the pollutant removal, the catalyst preservation and the biodegradability enhancement. Chem. Eng. J. 2007, 132(1-3):105-115.
27. Xu Y., Li X.Y., Cheng X., Sun D.Z., Wang X.Y. Degradation of cationic red GTL by catalytic wet air oxidation over Mo-Zn-Al-O catalyst under room temperature and atmospheric pressure. Environ. Sci. Technol. 2012, 46(5):2856-2863.
28. Yamakoshi Y., Umezawa N., Rui A., Arakane K., Miyakta N., Goda Y., et al. Active oxygen species generated from photoexcited fullerene (C60) as potential medicines: O2- versus O2. J. Am. Chem. Soc. 2003, 125(42):12803-12809.
29. Yang S.X., Feng Y.J., Wan J.F., Lin Q.Y., Zhu W.P., Jiang Z.P. Pretreatment of apramycin wastewater by catalytic wet air oxidation. J. Environ. Sci. 2005, 17(4):623-626.
30. Yang M., Xu A.H., Du H.Z., Sun C.L., Li C. Removal of salicylic acid on perovskite-type oxide LaFeO3 catalyst in catalytic wet air oxidation process. J. Hazard. Mater. 2007, 139(1):86-92.
31. Yang S.X., Zhu W.P., Li X., Wang J.B., Zhou Y.R. Multi-walled carbon nanotubes (MWNTs) as an efficient catalyst for catalytic wet air oxidation of phenol. Catal. Commun. 2007, 8(12):2059-2063.
32. Yang S.X., Li X., Zhu W.P., Wang J.B., Descorme C. Catalytic activity, stability and structure of multi-walled carbon nanotubes in the wet air oxidation of phenol. Carbon 2008, 46(3):445-452.
33. Yang S.X., Besson M., Descorme C. Catalytic wet air oxidation of formic acid over Pt/CexZr1-xO2 catalysts at low temperature and atmospheric pressure. Appl. Catal. B Environ. 2010, 100(1-2):282-288.
34. Zhu W.P., Bin Y.J., Li Z.H., Jiang Z.P., Yin T. Application of catalytic wet air oxidation for the treatment of H-acid manufacturing process wastewater. Water Res. 2002, 36(8):1947-1954.