Pd-Au/C catalysts with different alloying degrees for ethanol oxidation in alkaline media

Electrochimica Acta

Volumn 144, Issue , 2014, Pages 50-55

  Qin, Yuan Hang ^a,b   Li, Yunfeng ^b   Lv, Ren Liang ^a   Wang, Tie Lin ^a   Wang, Wei Guo ^a   Wang, Cun Wen ^a  

^a WUHAN INSTITUTE OF TECHNOLOGY   (China)

^b University of Missouri   (United States)

Author keywords

alloy; ethanol oxidation; gold; palladium

Indexed keywords

ALLOYING; CATALYST ACTIVITY; CATALYTIC OXIDATION; ETHANOL; GOLD; HIGH RESOLUTION TRANSMISSION ELECTRON MICROSCOPY; OXIDATION; PALLADIUM; REDUCING AGENTS; SODIUM BOROHYDRIDE; TRANSMISSION ELECTRON MICROSCOPY; X RAY DIFFRACTION; X RAY PHOTOELECTRON SPECTROSCOPY;

CORE SHELL STRUCTURE; ELECTROCHEMICAL CHARACTERIZATIONS; ENHANCED ADSORPTIONS; ETHANOL OXIDATION; ETHANOL OXIDATION REACTION; HOMOGENOUS STRUCTURE; SHELL STRUCTURE; TRI-SODIUM CITRATES;

PALLADIUM ALLOYS;

EID: 84906957959     PISSN: 00134686     EISSN: None     Source Type: Journal    
DOI: 10.1016/j.electacta.2014.08.078     Document Type: Article

References (28)

1. W. Du, K.E. Mackenzie, D.F. Milano, N.A. Deskins, D. Su, and X. Teng Palladium-tin alloyed catalysts for the ethanol oxidation reaction in an alkaline medium ACS Catal. 2 2012 287 297
2. Y.-H. Qin, H.-C. Li, H.-H. Yang, X.-S. Zhang, X.-G. Zhou, L. Niu, and W.-K. Yuan Effect of electrode fabrication methods on the electrode performance for ethanol oxidation J. Power Sources 196 2011 159 163
3. C. Xu, L. Cheng, P. Shen, and Y. Liu Methanol and ethanol electrooxidation on Pt and Pd supported on carbon microspheres in alkaline media.Electrochem Electrochem. Commun. 9 2007 997 1001
4. C. Bianchini, and P.K. Shen Palladium-based electrocatalysts for alcohol oxidation in half cells and in direct alcohol fuel cells Chem. Rev. 109 2009 4183 4206
5. Q. He, W. Chen, S. Mukerjee, S. Chen, and F. Laufek Carbon-supported PdM (M = Au and Sn) nanocatalysts for the electrooxidation of ethanol in high pH media J. Power Sources 187 2009 298 304
6. C.-H. Cui, J.-W. Yu, H.-H. Li, M.-R. Gao, H.-W. Liang, and S.-H. Yu Remarkable enhancement of electrocatalytic activity by tuning the interface of Pd-Au bimetallic nanoparticle tubes ACS Nano 5 2011 4211 4218
7. Y.-Y. Feng, Z.-H. Liu, Y. Xu, P. Wang, W.-H. Wang, and D.-S. Kong Highly active PdAu alloy catalysts for ethanol electro-oxidation J. Power Sources 232 2013 99 105
8. M. Nie, H. Tang, Z. Wei, S.P. Jiang, and P.K. Shen Highly efficient AuPd-WC/C electrocatalyst for ethanol oxidation Electrochem. Commun. 9 2007 2375 2379
9. F. Cheng, X. Dai, H. Wang, S.P. Jiang, M. Zhang, and C. Xu Synergistic effect of Pd-Au bimetallic surfaces in Au-covered Pd nanowires studied for ethanol oxidation Electrochim. Acta 55 2010 2295 2298
10. S.W. Kang, Y.W. Lee, M. Kim, J.W. Hong, and S.W. Han One-pot synthesis of carbon-supported dendritic Pd-Au nanoalloys for electrocatalytic ethanol oxidation Chem. -Asian J. 6 2011 909 913
11. C. Zhu, S. Guo, and S. Dong PdM (M = Pt, Au) bimetallic alloy nanowires with enhanced electrocatalytic activity for electro-oxidation of small molecules Adv. Mater. 24 2012 2326 2331
12. Z. Huang, H. Zhou, C. Li, F. Zeng, C. Fu, and Y. Kuang Preparation of well-dispersed PdAu bimetallic nanoparticles on reduced graphene oxide sheets with excellent electrochemical activity for ethanol oxidation in alkaline media J. Mater. Chem. 22 2012 1781 1785
13. Y.W. Lee, M. Kim, Y. Kim, S.W. Kang, J.-H. Lee, and S.W. Han Synthesis and electrocatalytic activity of Au-Pd alloy nanodendrites for ethanol oxidation J. Phys. Chem. C 114 2010 7689 7693
14. J.B. Xu, T.S. Zhao, S.Y. Shen, and Y.S. Li Stabilization of the palladium electrocatalyst with alloyed gold for ethanol oxidation Int. J. Hydrogen Energy 35 2010 6490 6500
15. G. Zhang, Y. Wang, X. Wang, Y. Chen, Y. Zhou, Y. Tang, L. Lu, J. Bao, and T. Lu Preparation of Pd-Au/C catalysts with different alloying degree and their electrocatalytic performance for formic acid oxidation Appl. Catal. B-Environ. 102 2011 614 619
16. Y. Suo, and I.M. Hsing Synthesis of bimetallic PdAu nanoparticles for formic acid oxidation Electrochim. Acta 56 2011 2174 2183
17. Y.-H. Qin, Y. Jiang, D.-F. Niu, X.-S. Zhang, X.-G. Zhou, L. Niu, and W.-K. Yuan Carbon nanofiber supported bimetallic PdAu nanoparticles for formic acid electrooxidation J. Power Sources 215 2012 130 134
18. G. Chen, M. Liao, B. Yu, Y. Li, D. Wang, G. You, C.-J. Zhong, and B.H. Chen Pt decorated PdAu/C nanocatalysts with ultralow Pt loading for formic acid electrooxidation Int. J. Hydrogen Energy 37 2012 9959 9966
19. F. Ren, H. Wang, C. Zhai, M. Zhu, R. Yue, Y. Du, P. Yang, J. Xu, and W. Lu Clean method for the synthesis of reduced graphene oxide-supported PtPd alloys with high electrocatalytic activity for ethanol oxidation in alkaline medium ACS Appl. Mater. Interfaces 6 2014 3607 3614
20. Y.-H. Qin, H.-H. Yang, X.-S. Zhang, P. Li, X.-G. Zhou, L. Niu, and W.-K. Yuan Electrophoretic deposition of network-like carbon nanofibers as a palladium catalyst support for ethanol oxidation in alkaline media Carbon 48 2010 3323 3329
21. Z.X. Liang, T.S. Zhao, J.B. Xu, and L.D. Zhu Mechanism study of the ethanol oxidation reaction on palladium in alkaline media Electrochim. Acta 54 2009 2203 2208
22. W. Hong, J. Wang, and E. Wang Facile synthesis of highly active PdAu nanowire networks as self-supported electrocatalyst for ethanol electrooxidation ACS Appl. Mater. Interfaces 6 2014 9481 9487
23. L.Y. Chen, N. Chen, Y. Hou, Z.C. Wang, S.H. Lv, T. Fujita, J.H. Jiang, A. Hirata, and M.W. Chen Geometrically controlled nanoporous PdAu bimetallic catalysts with tunable Pd/Au Ratio for direct ethanol fuel cells ACS Catal. 3 2013 1220 1230
24. J. Hernández, J. Solla-Gullón, E. Herrero, A. Aldaz, and J.M. Feliu Methanol oxidation on gold nanoparticles in alkaline media: unusual electrocatalytic activity Electrochim. Acta 52 2006 1662 1669
25. R.N. Singh, A. Singh, and Anindita Electrocatalytic activity of binary and ternary composite films of Pd, MWCNT, and Ni for ethanol electro-oxidation in alkaline solutions Carbon 47 2009 271 278
26. 2nanotube arrays supported Pd nanoparticles for ethanol electrooxidation in alkaline media Electrochim. Acta 106 2013 372 377
27. L.A. Kibler, A.M. El-Aziz, R. Hoyer, and D.M. Kolb Tuning reaction rates by lateral strain in a palladium monolayer Angew. Chem. Int. Ed. 44 2005 2080 2084
28. X.-M. Wang, and Y.-Y. Xia Synthesis, characterization and catalytic activity of an ultrafine Pd/C catalyst for formic acid electrooxidation Electrochim. Acta 54 2009 7525 7530