Long-term radiostrontium interactions and transport through sediment

Environmental Science and Technology

Volumn 48, Issue 15, 2014, Pages 8919-8925

  Kaplan, Daniel I ^a   Miller, Todd J ^b   Diprete, David ^a   Powell, Brian A ^b  

^a SAVANNAH RIVER NATIONAL LABORATORY   (United States)

^b CLEMSON UNIVERSITY   (United States)

Author keywords

[No Author keywords available]

Indexed keywords

DESORPTION; GROUNDWATER; LYSIMETERS; SEDIMENTS; SOIL SURVEYS;

CONCENTRATION RATIO; DESORPTION TESTS; HIGH-LEVEL NUCLEAR WASTES; RADIOACTIVE STRONTIUM; RADIOLOGICAL CONTAMINANTS; SECONDARY AGING; SORPTION COEFFICIENTS; TRANSPORT MODELING;

SOIL TESTING;

STRONTIUM; STRONTIUM 85; STRONTIUM 90; CARBONIC ACID DERIVATIVE; GROUND WATER; RADIOACTIVE WASTE; SOIL; SOIL POLLUTANT; WATER POLLUTANT;

AGING; ARTICLE; CHEMICAL INTERACTION; CONTACT TIME; CONTROLLED STUDY; DESORPTION; IONIC STRENGTH; ISOTHERM; LIQUID; LYSIMETER; MEDICAL DEVICE; NUCLEAR WASTE; SEDIMENT; SOLID; STEADY STATE; STRONTIUM TRANSPORT; TIME; TRANSPORT AND BINDING PHENOMENA; ADSORPTION; ANALYSIS; CHEMICAL MODEL; CHEMISTRY; PH; RADIOACTIVE WASTE; SOIL; SOIL POLLUTANT; WATER POLLUTANT;

ADSORPTION; CARBONATES; GEOLOGIC SEDIMENTS; GROUNDWATER; HYDROGEN-ION CONCENTRATION; MODELS, CHEMICAL; RADIOACTIVE WASTE; SOIL; SOIL POLLUTANTS, RADIOACTIVE; STRONTIUM; STRONTIUM RADIOISOTOPES; WATER POLLUTANTS, RADIOACTIVE;

EID: 84905660147     PISSN: 0013936X     EISSN: 15205851     Source Type: Journal    
DOI: 10.1021/es5021108     Document Type: Article

References (32)

1. Faure, G. and Powell, J. L. Strontium Isotope Geology; Springer-Verlag: Berlin, Germany, 1972.
2. Environmental characteristics of EPA, NRC, and DOE sites contaminated with radioactive substances; EPA 402-R-93-011; U.S. Environmental Protection Agency: Washington, DC, 1993.
3. Riley, R. G. and Zachara, M. M.; Chemical Contaminants on DOE Lands and Selection of Contaminants Mixtures for Subsurface Science Research; DOE/ER-0547T DOE: Washington, DC, 1992.
4. d, Values. Vol. 1: The Kd Model, Methods of Measurement, and Application of Chemical Reaction Codes EPA 402-R-99-004A; Office of Air and Radiation, Office of Solid Waste and Emergency Response; U.S. Environmental Protection Agency: Washington, DC, 1999.
5. Dyer, A.; Chow, J. K. K.; Umar, I. M. The uptake of caesium and strontium radioisotopes onto clays J. Mater. Chem. 2000, 10, 2734-2740
6. Stevenson, F. J.; Fitch, A., Chemistry of complexation metal ions with soil solution organics. In Interactions of Soil Minerals with Natural Organics and Microbes, Huang, P. M.; Schnitzer, M., Eds.; Soil Science Society of America, Inc.: Madison, WI, 1986; pp 29-56.
7. 3H), and uranium; EPA 402-R-99 - 004; U.S. Environmental Protection Agency: Washington, DC, 1999.
8. Ames, L. L.; Rai, D. Radionuclide interactions with soil and rock media. Vol. 1: Processes influencing radionuclide mobility and retention, element chemistry and geochemistry, and conclusions and evaluation; EPA 520/6-78-007A; U.S. Environmental Protection Agency: Washington DC, 1978.
9. Bartl, U.; Czurda, K. A. Migration and retention phenomena of radionuclides in clay-barrier systems Appl. Clay Sci. 1991, 6 (3) 195-214
10. Czurda, K. A.; Rashidchi, A. A. Migration of radionuclides (Sr-90, Cs-137) in clays from the Austrian Molasse Appl. Clay Sci. 1987, 2 (2) 129-143
11. Brady, P. V.; Papenguth, H. W.; Lucero, D. A. Adsorption/desorption of strontium on calcite Mineral. Mag. 1998, 62A, 225-226
12. Schulz, R. K.; Riedel, H. H. Effect of aging on fixation of strontium-90 by soils Soil Sci. 1961, 91, 262-264
13. Wiklander, L. Uptake, adsorption and leaching of radiostrontium in a lysimeter experiment Soil Sci. 1964, 97, 168-172
14. Roberts, H., Jr.; Menzel, R. G. Availability of exchangeable and nonexchangeable strongium-90 to plants J. Agric. Food Chem. 1961, 9, 95-98
15. Taylor, A. W. Strontium retention in acid soils of the North Carolina Coastal Plain Soil Sci. 1968, 106, 440-0447
16. Cerling, T. E.; Spalding, B. P. Distribution and relationship of radionuclides to streambed gravels in a small watershed Environ. Geol. 1982, 4, 99-116
17. Capo, R. C.; Stewart, B. W.; Chadwick, O. A. Strontium isotopes as tracers of ecosystem processes: theory and methods Geoderma 1998, 82 (1-3) 197-225
18. Jantzen, C. M.; Kaplan, D. I.; Bibler, N. E.; Peeler, D. K.; Plodinec, M. J. Performance of a buried radioactive high level waste (HLW) glass after 24 years J. Nucl. Mater. 2008, 378 (3) 244-256
19. Demirkanli, D. I.; Molz, F. J.; Kaplan, D. I.; Fjeld, R. A.; Serkiz, S. M. A fully transient model for long-term plutonium transport in the Savannah River Site vadose zone: Plant water uptake Vadose Zone J. 2008, 7, 1099-1109
20. Sims, D. J.; Andrews, W. S.; Creber, D. A. M. Diffusion coefficients for uranium, cesium, and strontium in unsaturated prairie soil J. Radioanal. Nucl. Chem. 2008, 277, 143-147
21. Du Laing, G.; Rinklebe, J.; Vandecasteele, B.; Meers, E.; Tack, F. M. G. Trace metal behaviour in estuarine and riverine floodplain soils and sediments: A review Sci. Total Environ. 2009, 407 (13) 3972-3985
22. Sposito, G. Chemical Equilibria and Kinetics in Soils; Oxford University Press: New York, 1994.
23. Sparks, D. L., Kinetics and mechanisms of chemical reactions at the soil mineral/water interface. In Soil Physical Chemistry, 2 nd ed.; Sparks, D. L., Ed.; CRC Press, LLC: Boca Raton, FL, 1999; pp 135-192.
24. Guiherme, L. R. G.; Anderson, S. J., Copper sorption kinetics and sorption hysteresis in two oxide-rich soils (Oxisols): Effect of phophate pretreatment. In Adsorption of Metals by Geomedia; Jenne, E. A., Ed.; Academic Press Ltd: London, 1998; pp 210-229.
25. Demirkanli, D. I.; Molz, F. J.; Kaplan, D. I.; Fjeld, R. A. Soil-root interactions controlling upward plutonium transport in variably saturated soils Vadose Zone J. 2009, 8 (3) 574-585
26. Kaplan, D. I.; Demirkanli, D. I.; Gumapas, L.; Powell, B. A.; Fjeld, R. A.; Molz, F. J.; Serkiz, S. M. 11-Year field study of Pu migration from Pu III, IV, and VI sources Environ. Sci. Technol. 2006, 40 (2) 443-448
27. Kaplan, D. I.; Powell, B. A.; Gumapas, L.; Coates, J. T.; Fjeld, R. A.; Diprete, D. P. Influence of pH on plutonium desorption/solubilization from sediment Environ. Sci. Technol. 2006, 40 (19) 5937-5942
28. Choppin, G. R. Actinide speciation in aquatic systems Mar. Chem. 2006, 99, 83-92
29. Powell, B. A.; Kaplan, D. I.; Serkez, S. M.; Coates, J.; Fjeld, R. A. Pu(V) transport through southeastern soils-an evaluation of a conceptual model of surface-mediated reduction to Pu(IV) J. Environ. Radioact. 2014, 131, 47-56
30. Harris, W.; White, N. X-ray diffraction techniques for soil mineral identification. In Methods of Soil Analysis. Part 5. Mineralogical Methods; Ulery, A. L.; Drees, L. R., Eds.; Soil Society of America, Inc: Madison, WI, 2007; pp 81-117.
31. Nelson, D. W.; Sommers, L. E. Total carbon, organic carbon, and organic matter. In Methods of Soil Analysis. Part 3. Chemical Methods; Sparks, D. L., Ed.; Soil Science Society of America, Inc: Madison, WI, 1996; pp 961-1010.
32. Leoppert, R. H.; Inskeep, W. P. Iron. In Methods of Soil Analysis. Part 3. Chemical Methods; Sparks, D. L., Ed.; Soil Science Society of America, Inc: Madison, WI, 1996; pp 639-664.