Principle of Photocatalysis and Design of Active Photocatalysts

New and Future Developments in Catalysis: Solar Photocatalysis

Volumn , Issue , 2013, Pages 121-144

  Ohtani, B ^a  

^a HOKKAIDO UNIVERSITY   (Japan)

Author keywords

[No Author keywords available]

Indexed keywords

EID: 84904372007     PISSN: None     EISSN: None     Source Type: Book    
DOI: 10.1016/B978-0-444-53872-7.00006-6     Document Type: Chapter

References (61)

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57. + pairs:).
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59. Some reports on photocatalytic reaction stated that the time-course curve obeys the first-order rate law and that the rate of reaction changes following Langmuir-type adsorption behavior (so-called "Langmuir-Hinshelwood mechanism") when the substrate concentration is changed, though these two facts are incompatible. A possible situation is that a double reciprocal plot of rate and substrate concentration (Figure 5.7a) is linear but that the line passes through the origin, suggesting that the rate is proportional to the substrate concentration.
60. Similar action spectrum analysis of photoinduced degradation of Rhodamine B with a cadmium sulfide suspension has been reported by Watanabe et al. They pointed out a similar dye-sensitization mechanism: T. Watanabe, T. Takizawa, K. Honda, J. Phys. Chem. 81 (1977) 1845. Photocatalytic reaction of MB in aerated titania suspensions was reported in 1937 by a Japanese photochemist: M. Horio, Nihon Gakujutsu Kyokai Hokoku 12 (1937) 204 (in Japanese). As far as the author knows, this is the first report on titania photocatalysis.
61. It was proved that tungsten(VI) oxide produces a negligible amount of hydrogen from an aqueous solution containing electron donors such as methanol even when loaded with platinum, and this is consistent with the assumption of platinum-catalyzed multiple-electron transfer to oxygen.